Proliferation resistances of Generation IV recycling facilities for nuclear fuel

Abstract The effects of global warming raise demands for reduced CO2 emissions, whereas at the same time the world's need for energy increases. With the aim to resolve some of the difficulties facing today's nuclear power, striving for safety, sustainability and waste minimization, a new generation of nuclear energy systems is being pursued: Generation IV. New reactor concepts and new nuclear facilities should be at least as resistant to diversion of nuclear material for weapons production, as were the previous ones. However, the emerging generation of nuclear power will give rise to new challenges to the international safeguards community, due to new and increased flows of nuclear material in the nuclear fuel cycle. Before a wide implementation of Generation IV nuclear power facilities takes place, there lies still an opportunity to formulate safeguards requirements for the next generation of nuclear energy systems. In this context, this thesis constitutes one contribution to the global efforts to make future nuclear energy systems increasingly resistant to nuclear material diversion attempts. This thesis comprises three papers, all of which concern safeguards and proliferation resistance in Generation IV nuclear energy systems and especially recycling facilities: In Paper I, proliferation resistances of three fuel cycles, comprising different reprocessing techniques, are investigated. The results highlight the importance of making group actinide extraction techniques commercial, due to the inherently less vulnerable isotopic and radiological properties of the materials in such processes. Paper II covers the schematic design and safeguards instrumentation of a Generation IV recycling facility. The identification of the safeguards needs of planned facilities can act as a guide towards the development of new instrumentation suitable for Generation IV nuclear energy systems. Finally, Paper III describes a mode of procedure for assessing proliferation resistance of a recycling facility for fast reactor fuel. The assessments may be used, as in this case, as an aid to maintain or increase the inherent proliferation resistance when performing facility design changes and upgrades

Nuclear safeguards evaluation and analysis techniques for application to nuclear fuel material in Generation IV nuclear energy systems

A new generation of nuclear energy systems called Generation IV is under development to ensure that nuclear power will be a safe, reliable and sustainable energy source for the future. This thesis addresses the challenge of making future nuclear energy systems increasingly resistant to nuclear material diversion attempts. Several tools have been developed for structured evaluation of a system's resistance to nuclear proliferation, in order to identify areas where nuclear energy systems are the most inherently vulnerable. In this thesis, the TOPS methodology has been applied to three different fuel cycles involving a fast reactor with fuel recycling and fuel fabrication capabilities. The recycling facility, where the fuel is dissolved and undergoes chemical separation, is identified as being particularly vulnerable. Nondestructive measurements for verification of fuel assemblies in the receipt area of the recycling facility are essential, since it is the last opportunity to verify intact fuel items. Moreover, iterative evaluation of proliferation resistance by using two different assessment methodologies – TOPS and PR&PP – as suggested in this thesis, may act as an aid in facility design and for proposing safeguards implementation. Based on the identified need to measure irradiated fuel assemblies prior to dissolution in the recycling facility, new methods used for analyzing gamma-ray spectroscopy data using multivariate analysis methods have been investigated. Fuel parameters of modeled nuclear fuel have been determined without any reliance on operator-declared data. Nonlinear classifiers, e.g. support vector machines (SVM), have successfully been used for discrimination between uranium oxide fuels and mixed oxide fuels. Cooling time, burnup and initial fissile content have been determined using decision tree and SVM regression. The results are promising and indicate that the nuclear safeguards regime may benefit from using multivariate techniques for data analysis. It must be emphasized, however, that experimental verification of the multivariate analysis techniques is necessary

Magnetic Monopole Searches : with AMANDA and other detectors

Magnetic monopoles are hypothetical particles carrying isolated magnetic charges, analogous to electrically charged particles. They have never been observed in experiments, but there are theoretical indications that they might exist. Several experiments have been carried out over the years in order to detect monopoles, or to set upper limits on their abundance in the Universe. In this work, underlying theory of the properties of magnetic monopoles is presented, together with some of the experiments performed in the past, the present and the future. Emphasis is put on AMANDA and other Cherenkov neutrino telescopes. Results of the described experimental searches are summarized

Proliferation resistances of Generation IV recycling facilities for nuclear fuel

The effects of global warming raise demands for reduced CO2 emissions, whereas at the same time the world’s need for energy increases. With the aim to resolve some of the difficulties facing today’s nuclear power, striving for safety, sustainability and waste minimization, a new generation of nuclear energy systems is being pursued: Generation IV. New reactor concepts and new nuclear facilities should be at least as resistant to diversion of nuclear material for weapons production, as were the previous ones. However, the emerging generation of nuclear power will give rise to new challenges to the international safeguards community, due to new and increased flows of nuclear material in the nuclear fuel cycle. Before a wide implementation of Generation IV nuclear power facilities takes place, there lies still an opportunity to formulate safeguards requirements for the next generation of nuclear energy systems. In this context, this thesis constitutes one contribution to the global efforts to make future nuclear energy systems increasingly resistant to nuclear material diversion attempts. This thesis comprises three papers, all of which concern safeguards and proliferation resistance in Generation IV nuclear energy systems and especially recycling facilities: In Paper I, proliferation resistances of three fuel cycles, comprising different reprocessing techniques, are investigated. The results highlight the importance of making group actinide extraction techniques commercial, due to the inherently less vulnerable isotopic and radiological properties of the materials in such processes. Paper II covers the schematic design and safeguards instrumentation of a Generation IV recycling facility. The identification of the safeguards needs of planned facilities can act as a guide towards the development of new instrumentation suitable for Generation IV nuclear energy systems. Finally, Paper III describes a mode of procedure for assessing proliferation resistance of a recycling facility for fast reactor fuel. The assessments may be used, as in this case, as an aid to maintain or increase the inherent proliferation resistance when performing facility design changes and upgrades

Nuclear safeguards evaluation and analysis techniques for application to nuclear fuel material in Generation IV nuclear energy systems

A new generation of nuclear energy systems called Generation IV is under development to ensure that nuclear power will be a safe, reliable and sustainable energy source for the future. This thesis addresses the challenge of making future nuclear energy systems increasingly resistant to nuclear material diversion attempts. Several tools have been developed for structured evaluation of a system's resistance to nuclear proliferation, in order to identify areas where nuclear energy systems are the most inherently vulnerable. In this thesis, the TOPS methodology has been applied to three different fuel cycles involving a fast reactor with fuel recycling and fuel fabrication capabilities. The recycling facility, where the fuel is dissolved and undergoes chemical separation, is identified as being particularly vulnerable. Nondestructive measurements for verification of fuel assemblies in the receipt area of the recycling facility are essential, since it is the last opportunity to verify intact fuel items. Moreover, iterative evaluation of proliferation resistance by using two different assessment methodologies – TOPS and PR&PP – as suggested in this thesis, may act as an aid in facility design and for proposing safeguards implementation. Based on the identified need to measure irradiated fuel assemblies prior to dissolution in the recycling facility, new methods used for analyzing gamma-ray spectroscopy data using multivariate analysis methods have been investigated. Fuel parameters of modeled nuclear fuel have been determined without any reliance on operator-declared data. Nonlinear classifiers, e.g. support vector machines (SVM), have successfully been used for discrimination between uranium oxide fuels and mixed oxide fuels. Cooling time, burnup and initial fissile content have been determined using decision tree and SVM regression. The results are promising and indicate that the nuclear safeguards regime may benefit from using multivariate techniques for data analysis. It must be emphasized, however, that experimental verification of the multivariate analysis techniques is necessary

Safeguards Licensing Aspects of a Future Generation IV Demonstration Facility : A Case Study

Generation IV (Gen IV) is a developing new generation of nuclear power reactors which is foreseen to bring about a safer and more sustainable production of nuclear power. A Swedish research program called GENIUS aims at developing the Gen IV technology, with emphasis on lead-cooled fast reactors. The present work is part of the GENIUS project, and deals with safeguards aspects for an envisioned future 100 MW Gen IV demonstration facility including storage and reprocessing plant. Also, the safeguards licensing aspects for the facilities have been investigated and results thereof are presented. As a basis for the study, the changed usage and handling of nuclear fuel, as compared to that of today, have been examined in order to determine how today's safeguards measures can be modified and extended to meet the needs of the demonstration facility. Safeguards approaches have been considered for within and between each unit at the demonstration facility, with the main focus on system aspects rather than proposing safeguards instrumentation on a detailed level. The proposed safeguards approach include the implementation of well-tried measures that are used at currently existing nuclear facilities as well as suggestions for new procedures. The former include, among others, regular inventory verifications, containment and surveillance measures as well as non-destructive and destructive measurements of nuclear materials. The traditional approaches may be improved and supplemented by modern techniques and approaches such as nuclear forensics, safeguards-by-design and improved on-line monitoring of streams of nuclear material. The safeguards approach for the demonstration facility should be outlined early in the licensing process, such that the facility units can be designed in a way that allows for implementation of adequate safeguards measures with minimal intrusion on the regular activities. For operating a nuclear facility in Sweden, two separate permits are required. A license application for a new facility shall be handed both to the Swedish Radiation Safety Authority and to the environmental court, which in parallel prepare for decisions according to the Nuclear Activities Act and the Environmental Code, respectively. In terms of the Swedish legislation, there are no fundamental differences between Gen IV facilities and currently existing plants. However, comprehensive investigations and evaluations would be required in order to license new Gen IV facilities

Magnetic Monopole Searches : with AMANDA and other detectors

Magnetic monopoles are hypothetical particles carrying isolated magnetic charges, analogous to electrically charged particles. They have never been observed in experiments, but there are theoretical indications that they might exist. Several experiments have been carried out over the years in order to detect monopoles, or to set upper limits on their abundance in the Universe. In this work, underlying theory of the properties of magnetic monopoles is presented, together with some of the experiments performed in the past, the present and the future. Emphasis is put on AMANDA and other Cherenkov neutrino telescopes. Results of the described experimental searches are summarized

Safeguards Licensing Aspects of a Future Generation IV Demonstration Facility : A Case Study

Generation IV (Gen IV) is a developing new generation of nuclear power reactors which is foreseen to bring about a safer and more sustainable production of nuclear power. A Swedish research program called GENIUS aims at developing the Gen IV technology, with emphasis on lead-cooled fast reactors. The present work is part of the GENIUS project, and deals with safeguards aspects for an envisioned future 100 MW Gen IV demonstration facility including storage and reprocessing plant. Also, the safeguards licensing aspects for the facilities have been investigated and results thereof are presented. As a basis for the study, the changed usage and handling of nuclear fuel, as compared to that of today, have been examined in order to determine how today's safeguards measures can be modified and extended to meet the needs of the demonstration facility. Safeguards approaches have been considered for within and between each unit at the demonstration facility, with the main focus on system aspects rather than proposing safeguards instrumentation on a detailed level. The proposed safeguards approach include the implementation of well-tried measures that are used at currently existing nuclear facilities as well as suggestions for new procedures. The former include, among others, regular inventory verifications, containment and surveillance measures as well as non-destructive and destructive measurements of nuclear materials. The traditional approaches may be improved and supplemented by modern techniques and approaches such as nuclear forensics, safeguards-by-design and improved on-line monitoring of streams of nuclear material. The safeguards approach for the demonstration facility should be outlined early in the licensing process, such that the facility units can be designed in a way that allows for implementation of adequate safeguards measures with minimal intrusion on the regular activities. For operating a nuclear facility in Sweden, two separate permits are required. A license application for a new facility shall be handed both to the Swedish Radiation Safety Authority and to the environmental court, which in parallel prepare for decisions according to the Nuclear Activities Act and the Environmental Code, respectively. In terms of the Swedish legislation, there are no fundamental differences between Gen IV facilities and currently existing plants. However, comprehensive investigations and evaluations would be required in order to license new Gen IV facilities

Nuclear safeguards evaluation and analysis techniques for application to nuclear fuel material in Generation IV nuclear energy systems

A new generation of nuclear energy systems called Generation IV is under development to ensure that nuclear power will be a safe, reliable and sustainable energy source for the future. This thesis addresses the challenge of making future nuclear energy systems increasingly resistant to nuclear material diversion attempts. Several tools have been developed for structured evaluation of a system's resistance to nuclear proliferation, in order to identify areas where nuclear energy systems are the most inherently vulnerable. In this thesis, the TOPS methodology has been applied to three different fuel cycles involving a fast reactor with fuel recycling and fuel fabrication capabilities. The recycling facility, where the fuel is dissolved and undergoes chemical separation, is identified as being particularly vulnerable. Nondestructive measurements for verification of fuel assemblies in the receipt area of the recycling facility are essential, since it is the last opportunity to verify intact fuel items. Moreover, iterative evaluation of proliferation resistance by using two different assessment methodologies – TOPS and PR&PP – as suggested in this thesis, may act as an aid in facility design and for proposing safeguards implementation. Based on the identified need to measure irradiated fuel assemblies prior to dissolution in the recycling facility, new methods used for analyzing gamma-ray spectroscopy data using multivariate analysis methods have been investigated. Fuel parameters of modeled nuclear fuel have been determined without any reliance on operator-declared data. Nonlinear classifiers, e.g. support vector machines (SVM), have successfully been used for discrimination between uranium oxide fuels and mixed oxide fuels. Cooling time, burnup and initial fissile content have been determined using decision tree and SVM regression. The results are promising and indicate that the nuclear safeguards regime may benefit from using multivariate techniques for data analysis. It must be emphasized, however, that experimental verification of the multivariate analysis techniques is necessary

Safeguards Licensing Aspects of a Future Generation IV Demonstration Facility : A Case Study

Generation IV (Gen IV) is a developing new generation of nuclear power reactors which is foreseen to bring about a safer and more sustainable production of nuclear power. A Swedish research program called GENIUS aims at developing the Gen IV technology, with emphasis on lead-cooled fast reactors. The present work is part of the GENIUS project, and deals with safeguards aspects for an envisioned future 100 MW Gen IV demonstration facility including storage and reprocessing plant. Also, the safeguards licensing aspects for the facilities have been investigated and results thereof are presented. As a basis for the study, the changed usage and handling of nuclear fuel, as compared to that of today, have been examined in order to determine how today's safeguards measures can be modified and extended to meet the needs of the demonstration facility. Safeguards approaches have been considered for within and between each unit at the demonstration facility, with the main focus on system aspects rather than proposing safeguards instrumentation on a detailed level. The proposed safeguards approach include the implementation of well-tried measures that are used at currently existing nuclear facilities as well as suggestions for new procedures. The former include, among others, regular inventory verifications, containment and surveillance measures as well as non-destructive and destructive measurements of nuclear materials. The traditional approaches may be improved and supplemented by modern techniques and approaches such as nuclear forensics, safeguards-by-design and improved on-line monitoring of streams of nuclear material. The safeguards approach for the demonstration facility should be outlined early in the licensing process, such that the facility units can be designed in a way that allows for implementation of adequate safeguards measures with minimal intrusion on the regular activities. For operating a nuclear facility in Sweden, two separate permits are required. A license application for a new facility shall be handed both to the Swedish Radiation Safety Authority and to the environmental court, which in parallel prepare for decisions according to the Nuclear Activities Act and the Environmental Code, respectively. In terms of the Swedish legislation, there are no fundamental differences between Gen IV facilities and currently existing plants. However, comprehensive investigations and evaluations would be required in order to license new Gen IV facilities