Evolution of Quantum Discord and its Stability in Two-Qubit NMR Systems

We investigate evolution of quantum correlations in ensembles of two-qubit nuclear spin systems via nuclear magnetic resonance techniques. We use discord as a measure of quantum correlations and the Werner state as an explicit example. We first introduce different ways of measuring discord and geometric discord in two-qubit systems and then describe the following experimental studies: (a) We quantitatively measure discord for Werner-like states prepared using an entangling pulse sequence. An initial thermal state with zero discord is gradually and periodically transformed into a mixed state with maximum discord. The experimental and simulated behavior of rise and fall of discord agree fairly well. (b) We examine the efficiency of dynamical decoupling sequences in preserving quantum correlations. In our experimental setup, the dynamical decoupling sequences preserved the traceless parts of the density matrices at high fidelity. But they could not maintain the purity of the quantum states and so were unable to keep the discord from decaying. (c) We observe the evolution of discord for a singlet-triplet mixed state during a radio-frequency spin-lock. A simple relaxation model describes the evolution of discord, and the accompanying evolution of fidelity of the long-lived singlet state, reasonably well.Comment: 9 pages, 7 figures, Phys. Rev. A (in press

Techniques for the realization of ultrareliable spaceborne computers Interim scientific report

Error-free ultrareliable spaceborne computer

Phase space spinor amplitudes for spin 1/2 systems

The concept of phase space amplitudes for systems with continuous degrees of freedom is generalized to finite-dimensional spin systems. Complex amplitudes are obtained on both a sphere and a finite lattice, in each case enabling a more fundamental description of pure spin states than that previously given by Wigner functions. In each case the Wigner function can be expressed as the star product of the amplitude and its conjugate, so providing a generalized Born interpretation of amplitudes that emphasizes their more fundamental status. The ordinary product of the amplitude and its conjugate produces a (generalized) spin Husimi function. The case of spin-\half is treated in detail, and it is shown that phase space amplitudes on the sphere transform correctly as spinors under under rotations, despite their expression in terms of spherical harmonics. Spin amplitudes on a lattice are also found to transform as spinors. Applications are given to the phase space description of state superposition, and to the evolution in phase space of the state of a spin-\half magnetic dipole in a time-dependent magnetic field.Comment: 19 pages, added new results, fixed typo

Storing entanglement of nuclear spins via Uhrig Dynamical Decoupling

Stroboscopic spin flips have already been shown to prolong the coherence times of quantum systems under noisy environments. Uhrig's dynamical decoupling scheme provides an optimal sequence for a quantum system interacting with a dephasing bath. Several experimental demonstrations have already verified the efficiency of such dynamical decoupling schemes in preserving single qubit coherences. In this work we describe the experimental study of Uhrig's dynamical decoupling in preserving two-qubit entangled states using an ensemble of spin-1/2 nuclear pairs in solution state. We find that the performance of odd-order Uhrig sequences in preserving entanglement is superior to both even-order Uhrig sequences and periodic spin-flip sequences. We also find that there exists an optimal length of the Uhrig sequence at which the decoherence time gets boosted from a few seconds to about 30 seconds.Comment: 6 pages, 7 figure

Tungsten resonance integrals and Doppler coefficients Third quarterly report, Jan. - Mar. 1966

Reactivities, Doppler coefficients, and resonance integrals for tungsten isotope

Quantum information processing using strongly-dipolar coupled nuclear spins

Dipolar coupled homonuclear spins present challenging, yet useful systems for quantum information processing. In such systems, eigenbasis of the system Hamiltonian is the appropriate computational basis and coherent control can be achieved by specially designed strongly modulating pulses. In this letter we describe the first experimental implementation of the quantum algorithm for numerical gradient estimation on the eigenbasis of a four spin system.Comment: 5 pages, 5 figures, Accepted in PR

A First Principles Theory of Nuclear Magnetic Resonance J-Coupling in solid-state systems

A method to calculate NMR J-coupling constants from first principles in extended systems is presented. It is based on density functional theory and is formulated within a planewave-pseudopotential framework. The all-electron properties are recovered using the projector augmented wave approach. The method is validated by comparison with existing quantum chemical calculations of solution-state systems and with experimental data. The approach has been applied to verify measured J-coupling in a silicophosphate structure, Si5O(PO4)6Comment: 9 page

High Order Coherent Control Sequences of Finite-Width Pulses

The performance of sequences of designed pulses of finite length $\tau$ is analyzed for a bath of spins and it is compared with that of sequences of ideal, instantaneous pulses. The degree of the design of the pulse strongly affects the performance of the sequences. Non-equidistant, adapted sequences of pulses, which equal instantaneous ones up to $\mathcal{O}(\tau^3)$, outperform equidistant or concatenated sequences. Moreover, they do so at low energy cost which grows only logarithmically with the number of pulses, in contrast to standard pulses with linear growth.Comment: 6 pages, 5 figures, new figures, published versio

Quantum Zeno dynamics of a field in a cavity

We analyze the quantum Zeno dynamics that takes place when a field stored in a cavity undergoes frequent interactions with atoms. We show that repeated measurements or unitary operations performed on the atoms probing the field state confine the evolution to tailored subspaces of the total Hilbert space. This confinement leads to non-trivial field evolutions and to the generation of interesting non-classical states, including mesoscopic field state superpositions. We elucidate the main features of the quantum Zeno mechanism in the context of a state-of-the-art cavity quantum electrodynamics experiment. A plethora of effects is investigated, from state manipulations by phase space tweezers to nearly arbitrary state synthesis. We analyze in details the practical implementation of this dynamics and assess its robustness by numerical simulations including realistic experimental imperfections. We comment on the various perspectives opened by this proposal