Vacuum-Stimulated Raman Scattering based on Adiabatic Passage in a High-Finesse Optical Cavity

We report on the first observation of stimulated Raman scattering from a Lambda-type three-level atom, where the stimulation is realized by the vacuum field of a high-finesse optical cavity. The scheme produces one intracavity photon by means of an adiabatic passage technique based on a counter-intuitive interaction sequence between pump laser and cavity field. This photon leaves the cavity through the less-reflecting mirror. The emission rate shows a characteristic dependence on the cavity and pump detuning, and the observed spectra have a sub-natural linewidth. The results are in excellent agreement with numerical simulations.Comment: 4 pages, 5 figure

Quantum Beat of Two Single Photons

The interference of two single photons impinging on a beam splitter is measured in a time-resolved manner. Using long photons of different frequencies emitted from an atom-cavity system, a quantum beat with a visibility close to 100% is observed in the correlation between the photodetections at the output ports of the beam splitter. The time dependence of the beat amplitude reflects the coherence properties of the photons. Most remarkably, simultaneous photodetections are never observed, so that a temporal filter allows one to obtain perfect two-photon coalescence even for non-perfect photons.Comment: 4 pages, 3 figure

Entanglement and purity of single- and two-photon states

Whereas single- and two-photon wave packets are usually treated as pure states, in practice they will be mixed. We study how entanglement created with mixed photon wave packets is degraded. We find in particular that the entanglement of a delocalized single-photon state of the electro-magnetic field is determined simply by its purity. We also discuss entanglement for two-photon mixed states, as well as the influence of a vacuum component.Comment: 11 pages, 10 figures, 1 debuting autho

Detecting drift of quantum sources: not the de Finetti theorem

We propose and analyze a method to detect and characterize the drift of a nonstationary quantum source. It generalizes a standard measurement for detecting phase diffusion of laser fields to quantum systems of arbitrary Hilbert space dimension, qubits in particular. We distinguish diffusive and systematic drifts, and examine how quickly one can determine that a source is drifting. We show that for single-photon wavepackets our measurement is implemented by the Hong-Ou-Mandel effect.Comment: 5 pages, 2 figure

Characterization of single photons using two-photon interference

Adiabatic passage techniques allow the generation of single photons which are very long compared to the typical detector time resolution. Therefore the detection time of a photon can be measured within the duration of the single-photon wavepacket. As a consequence, two-photon interference can be investigated in a time-resolved manner, i.e., the coincidence rate can be measured as a function of the time between photodetections. The theoretical analysis shows that this method not only gives information about the duration of single photons, but also about their coherence time. Here we discuss how to use this method for a spectral or temporal characterization of a single-photon source.Comment: 17 pages, 12 figure

Counter-Intuitive Vacuum-Stimulated Raman Scattering

Vacuum-stimulated Raman scattering in strongly coupled atom-cavity systems allows one to generate free-running single photon pulses on demand. Most properties of the emitted photons are well defined, provided spontaneous emission processes do not contribute. Therefore, electronic excitation of the atom must not occur, which is assured for a system adiabatically following a dark state during the photon-generation process. We experimentally investigate the conditions that must be met for adiabatic following in a time-of-flight driven system, with atoms passing through a cavity and a pump beam oriented transverse to the cavity axis. From our results, we infer the optimal intensity and relative pump-beam position with respect to the cavity axis.Comment: 4 pages, 4 figure