Polarization and relaxation of radon

Investigations of the polarization and relaxation of $^{209}$Rn by spin exchange with laser optically pumped rubidium are reported. On the order of one million atoms per shot were collected in coated and uncoated glass cells. Gamma-ray anisotropies were measured as a signal of the alignment (second order moment of the polarization) resulting from the combination of polarization and quadrupole relaxation at the cell walls. The temperature dependence over the range 130$^\circ$C to 220$^\circ$C shows the anisotropies increasing with increasing temperature as the ratio of the spin exchange polarization rate to the wall relaxation rate increases faster than the rubidium polarization decreases. Polarization relaxation rates for coated and uncoated cells are presented. In addition, improved limits on the multipole mixing ratios of some of the main gamma-ray transitions have been extracted. These results are promising for electric dipole moment measurements of octupole-deformed $^{223}$Rn and other isotopes, provided sufficient quantities of the rare isotopes can be produced.Comment: 4 pages, 4 figure

Polarization and relaxation of ^209Rn

The study of the nuclear polarization of radon is motivated by the expected large enhancement of sensitivity to a CP-violating electric dipole moment (EDM) in isotopes with octupole deformation or vibrational strength. In preparation for EDM measurements, the polarization of radon by spin exchange with laser-polarized alkali metals is studied. The measurement of the alignment of 209Rn using HPGe detectors to observe the resulting anisotropy in the 337 and 745 keV gamma rays emitted following electron-capture decay of 209Rn to 209At is demonstrated. Radon is polarized via spin-exchange collisions with rubidium atoms in an uncoated Pyrex optical pumping cell. Anisotropy measurements at several temperatures are used to study polarization and relaxation