91 research outputs found
Non-trivial Surface-band Dispersion on Bi(111)
We performed angle-resolved photoelectron spectroscopy of the Bi(111) surface
to demonstrate that this surface support edge states of non-trivial topology.
Along the -direction of the surface Brillouin zone, a
surface-state band disperses from the projected bulk valence bands at
to the conduction bands at continuously, indicating
the non-trivial topological order of three-dimensional Bi bands. We ascribe
this finding to the absence of band inversion at the point of the bulk Bi
Brillouin zone. According to our analysis, a modification of tight-binding
parameters can account for the non-trivial band structure of Bi without any
other significant change on other physical properties.Comment: 13 pages, 4 figures. This manuscript has been accepted in New Journal
of Physic
Origin of the different electronic structure of Rh- and Ru-doped Sr2IrO4
One way to induce insulator to metal transitions in the spin-orbit Mott
insulator Sr2IrO4 is to substitute iridium with transition metals (Ru, Rh).
However, this creates intriguing inhomogeneous metallic states, which cannot be
described by a simple doping effect. We detail the electronic structure of the
Ru-doped case with angle-resolved photoemission and show that, contrary to Rh,
it cannot be connected to the undoped case by a rigid shift. We further
identify bands below coexisting with the metallic ones that we assign to
non-bonding Ir sites. We rationalize the differences between Rh and Ru by a
different hybridization with oxygen, which mediates the coupling to Ir and
sensitively affects the effective doping. We argue that the spin-orbit coupling
does not control neither the charge transfer nor the transition threshold
First direct observation of a nearly ideal graphene band structure
Angle-resolved photoemission and X-ray diffraction experiments show that
multilayer epitaxial graphene grown on the SiC(000-1) surface is a new form of
carbon that is composed of effectively isolated graphene sheets. The unique
rotational stacking of these films cause adjacent graphene layers to
electronically decouple leading to a set of nearly independent linearly
dispersing bands (Dirac cones) at the graphene K-point. Each cone corresponds
to an individual macro-scale graphene sheet in a multilayer stack where
AB-stacked sheets can be considered as low density faults.Comment: 5 pages, 4 figure
Symmetry of the Fermi surface and evolution of the electronic structure across the paramagnetic-helimagnetic transition in MnSi/Si(111)
MnSi has been extensively studied for five decades, nonetheless detailed
information on the Fermi surface (FS) symmetry is still lacking. This missed
information prevented from a comprehensive understanding the nature of the
magnetic interaction in this material. Here, by performing angle-resolved
photoemission spectroscopy on high-quality MnSi films epitaxially grown on
Si(111), we unveil the FS symmetry and the evolution of the electronic
structure across the paramagnetic-helimagnetic transition at T 40 K,
along with the appearance of sharp quasiparticle emission below T. The
shape of the resulting FS is found to fulfill robust nesting effects. These
effects can be at the origin of strong magnetic fluctuations not accounted for
by state-of-art quasiparticle self-consistent GW approximation. From this
perspective, the unforeseen quasiparticle damping detected in the paramagnetic
phase and relaxing only below T, along with the persistence of the d-bands
splitting well above T, at odds with a simple Stoner model for itinerant
magnetism, open the search for exotic magnetic interactions favored by FS
nesting and affecting the quasiparticles lifetime
Large area molybdenum disulphide-epitaxial graphene vertical Van der Waals heterostructures
International audienceTwo-dimensional layered transition metal dichalcogenides (TMDCs) show great potential for optoelectronic devices due to their electronic and optical properties. A metal-semiconductor interface, as epitaxial graphene - molybdenum disulfide (MoS2), is of great interest from the standpoint of fundamental science, as it constitutes an outstanding platform to investigate the interlayer interaction in van der Waals heterostructures. Here, we study large area MoS2-graphene-heterostructures formed by direct transfer of chemical-vapor deposited MoS2 layer onto epitaxial graphene/SiC. We show that via a direct transfer, which minimizes interface contamination, we can obtain high quality and homogeneous van der Waals heterostructures. Angle-resolved photoemission spectroscopy (ARPES) measurements combined with Density Functional Theory (DFT) calculations show that the transition from indirect to direct bandgap in monolayer MoS2 is maintained in these heterostructures due to the weak van der Waals interaction with epitaxial graphene. A downshift of the Raman 2D band of the graphene, an up shift of the A1g peak of MoS2 and a significant photoluminescence quenching are observed for both monolayer and bilayer MoS2 as a result of charge transfer from MoS2 to epitaxial graphene under illumination. Our work provides a possible route to modify the thin film TDMCs photoluminescence properties via substrate engineering for future device design
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