Non-conventional superconducting fluctuations in Ba(Fe1-xRhx)2As2 iron-based superconductors

We measured the static uniform spin susceptibility of Ba(Fe$_{1-x}$Rh$_x$)$_2$As$_2$ iron-based superconductors, over a broad range of doping ($0.041\leq x\leq 0.094$) and magnetic fields. At small fields ($H \le$ 1 kOe) we observed, above the transition temperature $T_c$, the occurrence of precursor diamagnetism, which is not ascribable to the Ginzburg-Landau theory. On the contrary, our data fit a phase fluctuation model, which has been used to interpret a similar phenomenology occurring in the high-$T_c$ cuprate superconductors. On the other hand, in presence of strong fields the unconventional fluctuating diamagnetism is suppressed, whereas 3D fluctuations are found, in agreement with literature

Chapter The Cultural Heritage of Tomorrow: Should we Put a Limit to the Influence that New Technologies Have on Culture and Design?

undefine

Tunneling splitting of magnetic levels in Fe8 detected by 1H NMR cross relaxation

Measurements of proton NMR and the spin lattice relaxation rate 1/T1 in the octanuclear iron (III) cluster [Fe8(N3C6H15)6O2(OH)12][Br8 9H2O], in short Fe8, have been performed at 1.5 K in a powder sample aligned along the main anisotropy z axis, as a function of a transverse magnetic field (i.e., perpendicular to the main easy axis z). A big enhancement of 1/T1 is observed over a wide range of fields (2.5-5 T), which can be attributed to the tunneling dynamics; in fact, when the tunneling splitting of the pairwise degenerate m=+-10 states of the Fe8 molecule becomes equal to the proton Larmor frequency a very effective spin lattice relaxation channel for the nuclei is opened. The experimental results are explained satisfactorily by considering the distribution of tunneling splitting resulting from the distribution of the angles in the hard xy plane for the aligned powder, and the results of the direct diagonalization of the model Hamiltonian.Comment: J. Appl. Phys., in pres

Spin dynamics in molecular ring nanomagnets: Significant effect of acoustic phonons and magnetic anisotropies

The nuclear spin-lattice relaxation rate 1/T_1_ is calculated for magnetic ring clusters by fully diagonalizing their microscopic spin Hamiltonians. Whether the nearest-neighbor exchange interaction J is ferromagnetic or antiferromagnetic, 1/T_1_ versus temperature T in ring nanomagnets may be peaked at around k_B_T=|J| provided the lifetime broadening of discrete energy levels is in proportion to T^3^. Experimental findings for ferromagnetic and antiferromagnetic Cu^II^ rings are reproduced with crucial contributions of magnetic anisotropies as well as acoustic phonons.Comment: 5 pages with 5 figures embedded, to be published in J. Phys. Soc. Jpn. 75, No. 10 (2006