604 research outputs found
Two-photon excitation and relaxation of the 3d-4d resonance in atomic Kr
Two-photon excitation of a single-photon forbidden Auger resonance has been observed and investigated using the intense extreme ultraviolet radiation from the free electron laser in Hamburg. At the wavelength 26.9 nm (46 eV) two photons promoted a 3d core electron to the outer 4d shell. The subsequent Auger decay, as well as several nonlinear above threshold ionization processes, were studied by electron spectroscopy. The experimental data are in excellent agreement with theoretical predictions and analysis of the underlying multiphoton processes
Time-dependent calculation of ionization in Potassium at mid-infrared wavelengths
We study the dynamics of the Potassium atom in the mid-infrared, high
intensity, short laser pulse regime. We ascertain numerical convergence by
comparing the results obtained by the direct expansion of the time-dependent
Schroedinger equation onto B-Splines, to those obtained by the eigenbasis
expansion method. We present ionization curves in the 12-, 13-, and 14-photon
ionization range for Potassium. The ionization curve of a scaled system, namely
Hydrogen starting from the 2s, is compared to the 12-photon results. In the
13-photon regime, a dynamic resonance is found and analyzed in some detail. The
results for all wavelengths and intensities, including Hydrogen, display a
clear plateau in the peak-heights of the low energy part of the Above Threshold
Ionization (ATI) spectrum, which scales with the ponderomotive energy Up, and
extends to 2.8 +- 0.5 Up.Comment: 15 two-column pages with 15 figures, 3 tables. Accepted for
publication in Phys. Rev A. Improved figures, language and punctuation, and
made minor corrections. We also added a comparison to the ADK theor
Non-Markovian dynamics in atom-laser outcoupling from a double-well Bose-Einstein condensate
We investigate the dynamics of a continuous atom laser based on the merging
of independently formed atomic condensates. In a first attempt to understand
the dynamics of the system, we consider two independent elongated Bose-Einstein
condensates which approach each other and focus on intermediate inter-trap
distances so that a two-mode model is well justified. In the framework of a
mean-field theory, we discuss the quasi steady-state population of the traps as
well as the energy distribution of the outcoupled atoms.Comment: 21 pages, 9 figure, to appear in J. Phys.
Quantum correlation of an optically controlled quantum system
A precise time-dependent control of a quantum system relies on an accurate
account of the quantum interference among the system, the control and the
environment. A diagrammatic technique has been recently developed to precisely
calculate this quantum correlation for a fast multimode coherent photon control
against slow relaxation, valid for both Markovian and non-Markovian systems. We
review this formalism in comparison with the existing approximate theories and
extend it to cases with controls by photon state other than the coherent state.Comment: 23 pages, 8 figure
Phase-Control of Photoabsorption in Optically Dense Media
We present a self-consistent theory, as well as an illustrative application
to a realistic system, of phase control of photoabsorption in an optically
dense medium. We demonstrate that, when propagation effects are taken into
consideration, the impact on phase control is significant. Independently of the
value of the initial phase difference between the two fields, over a short
scaled distance of propagation, the medium tends to settle the relative phase
so that it cancels the atomic excitation. In addition, we find some rather
unusual behavior for an optically thin layer.Comment: 5 pages, 3 figures, submitted to PR
Tunable photonic band gaps with coherently driven atoms in optical lattices
Optical lattice loaded with cold atoms can exhibit a tunable photonic band
gap for a weak probe field under the conditions of electromagnetically induced
transparency. This system possesses a number of advantageous properties,
including reduced relaxation of Raman coherence and the associated probe
absorption, and simultaneous enhancement of the index modulation and the
resulting reflectivity of the medium. This flexible system has a potential to
serve as a testbed of various designs for the linear and nonlinear photonic
band gap materials at a very low light level and can be employed for realizing
deterministic entanglement between weak quantum fields
Two-electron processes in multiple ionization under strong soft-x-ray radiation
In a combined experimental and theoretical study we have investigated the ionization of atomic argon upon irradiation with intense soft-x-ray pulses of 105 eV photon energy from the free-electron laser FLASH. The measured ion yields show charge states up to Ar7+. The comparison with the theoretical study of the underlying photoionization dynamics highlights the importance of excited states in general and of processes governed by electron correlation in particular, namely, ionization with excitation and shake-off, processes usually inaccessible by measurements of ionic yields only. The Ar7+ yield shows a clear deviation from the predictions of the commonly used model of sequential ionization via single-electron processes and the observed signal can only be explained by taking into account the full multiplet structure of the involved configurations and by inclusion of two-electron processes. The competing process of two-photon ionization from the ground state of Ar6+ is calculated to be orders of magnitude smaller
Non-Markovian Dynamics of Entanglement for Multipartite Systems
Entanglement dynamics for a couple of two-level atoms interacting with
independent structured reservoirs is studied using a non-perturbative approach.
It is shown that the revival of atom entanglement is not necessarily
accompanied by the sudden death of reservoir entanglement, and vice versa. In
fact, atom entanglement can revive before, simultaneously or even after the
disentanglement of reservoirs. Using a novel method based on the population
analysis for the excited atomic state, we present the quantitative criteria for
the revival and death phenomena. For giving a more physically intuitive
insight, the quasimode Hamiltonian method is applied. Our quantitative analysis
is helpful for the practical engineering of entanglement.Comment: 10 pages and 4 figure
Ionization dynamics in intense pulsed laser radiation. Effects of frequency chirping
Via a non-perturbative method we study the population dynamics and
photoelectron spectra of Cs atoms subject to intense chirped laser pulses, with
gaussian beams. We include above threshold ionization spectral peaks. The
frequency of the laser is near resonance with the 6s-7p transition. Dominant
couplings are included exactly, weaker ones accounted for perturbatively. We
calculate the relevant transition matrix elements, including spin-orbit
coupling. The pulse is taken to be a hyperbolic secant in time and the chirping
a hyperbolic tangent. This choice allows the equations of motions for the
probability amplitudes to be solved analytically as a series expansion in the
variable u=(tanh(pi t/tau)+1)/2, where tau is a measure of the pulse length. We
find that the chirping changes the ionization dynamics and the photoelectron
spectra noticeably, especially for longer pulses of the order of 10^4 a.u. The
peaks shift and change in height, and interference effects between the 7p
levels are enhanced or diminished according to the amount of chirping and its
sign. The integrated ionization probability is not strongly affected.Comment: Accepted by J. Phys. B; 18 pages, 17 figures. Latex, uses
ioplppt.sty, iopl10.sty and psfig.st
Effects of interatomic collisions on atom laser outcoupling
We present a computational approach to the outcoupling in a simple
one-dimensional atom laser model, the objective being to circumvent
mathematical difficulties arising from the breakdown of the Born and Markov
approximations. The approach relies on the discretization of the continuum
representing the reservoir of output modes, which allows the treatment of
arbitrary forms of outcoupling as well as the incorporation of non-linear terms
in the Hamiltonian, associated with interatomic collisions. By considering a
single-mode trapped condensate, we study the influence of elastic collisions
between trapped and free atoms on the quasi steady-state population of the
trap, as well as the energy distribution and the coherence of the outcoupled
atoms.Comment: 25 pages, 11 figures, to appear in J. Phys.
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