Glassy dynamics in thin films of polystyrene

Glassy dynamics was investigated for thin films of atactic polystyrene by complex electric capacitance measurements using dielectric relaxation spectroscopy. During the isothermal aging process the real part of the electric capacitance increased with time, whereas the imaginary part decreased with time. It follows that the aging time dependences of real and imaginary parts of the electric capacitance were primarily associated with change in volume (film thickness) and dielectric permittivity, respectively. Further, dielectric permittivity showed memory and rejuvenation effects in a similar manner to those observed for poly(methyl methacrylate) thin films. On the other hand, volume did not show a strong rejuvenation effect.Comment: 7 pages, 7 figures. Phys. Rev. E (in press

A microscopic description of the aging dynamics: fluctuation-dissipation relations, effective temperature and heterogeneities

We consider the dynamics of a diluted mean-field spin glass model in the aging regime. The model presents a particularly rich heterogeneous behavior. In order to catch this behavior, we perform a **spin-by-spin analysis** for a **given disorder realization**. The results compare well with the outcome of a static calculation which uses the ``survey propagation'' algorithm of Mezard, Parisi, and Zecchina [Sciencexpress 10.1126/science.1073287 (2002)]. We thus confirm the connection between statics and dynamics at the level of single degrees of freedom. Moreover, working with single-site quantities, we can introduce a new response-vs-correlation plot, which clearly shows how heterogeneous degrees of freedom undergo coherent structural rearrangements. Finally we discuss the general scenario which emerges from our work and (possibly) applies to more realistic glassy models. Interestingly enough, some features of this scenario can be understood recurring to thermometric considerations.Comment: 4 pages, 5 figures (7 eps files

Fluctuation-Dissipation-Theorem violation during the formation of a colloidal-glass

The relationship between the conductivity and the polarization noise is measured in a gel as a function of frequency in the range $1Hz - 40Hz$. It is found that at the beginning of the transition from a fluid like sol to a solid like gel the fluctuation dissipation theorem is strongly violated. The amplitude and the persistence time of this violation are decreasing functions of frequency. At the lowest frequencies of the measuring range it persists for times which are about 5% of the time needed to form the gel. This phenomenology is quite close to the recent theoretical predictions done for the violation of the fluctuation dissipation theorem in glassy systems.Comment: 6 pages + 4 figure

Coarsening of Disordered Quantum Rotors under a Bias Voltage

We solve the dynamics of an ensemble of interacting rotors coupled to two leads at different chemical potential letting a current flow through the system and driving it out of equilibrium. We show that at low temperature the coarsening phase persists under the voltage drop up to a critical value of the applied potential that depends on the characteristics of the electron reservoirs. We discuss the properties of the critical surface in the temperature, voltage, strength of quantum fluctuations and coupling to the bath phase diagram. We analyze the coarsening regime finding, in particular, which features are essentially quantum mechanical and which are basically classical in nature. We demonstrate that the system evolves via the growth of a coherence length with the same time-dependence as in the classical limit, $R(t) \simeq t^{1/2}$ -- the scalar curvature driven universality class. We obtain the scaling function of the correlation function at late epochs in the coarsening regime and we prove that it coincides with the classical one once a prefactor that encodes the dependence on all the parameters is factorized. We derive a generic formula for the current flowing through the system and we show that, for this model, it rapidly approaches a constant that we compute.Comment: 53 pages, 12 figure

Correlation function and generalized master equation of arbitrary age

We study a two-state statistical process with a non-Poisson distribution of sojourn times. In accordance with earlier work, we find that this process is characterized by aging and we study three different ways to define the correlation function of arbitrary age of the corresponding dichotomous fluctuation based respectively on the Generalized Master Equation formalism, on a Liouville-like approach and on a trajectory perspective.Comment: 11 pages, 1figur

Aging, memory and rejuvenation: some lessons from simple models

Many recent experiments probed the off equilibrium dynamics of spin glasses and other glassy systems through temperature cycling protocols and observed memory and rejuvenation phenomena. Here we show through numerical simulations, using powerful algorithms, that such features can already be observed to some extent in simple models such as two dimensional ferromagnets. We critically discuss these results and review some aspects of the literature in the light of our findings.Comment: 10 pages, 8 figures. Contribution to the Proceedings of the Summerschool "Ageing and the glass transition", Luxembourg 14-25 Sept. 200

Multiple scaling regimes in simple aging models

We investigate aging in glassy systems based on a simple model, where a point in configuration space performs thermally activated jumps between the minima of a random energy landscape. The model allows us to show explicitly a subaging behavior and multiple scaling regimes for the correlation function. Both the exponents characterizing the scaling of the different relaxation times with the waiting time and those characterizing the asymptotic decay of the scaling functions are obtained analytically by invoking a `partial equilibrium' concept.Comment: 4 pages, 3 figure

Step-wise responses in mesoscopic glassy systems: a mean field approach

We study statistical properties of peculiar responses in glassy systems at mesoscopic scales based on a class of mean-field spin-glass models which exhibit 1 step replica symmetry breaking. Under variation of a generic external field, a finite-sized sample of such a system exhibits a series of step wise responses which can be regarded as a finger print of the sample. We study in detail the statistical properties of the step structures based on a low temperature expansion approach and a replica approach. The spacings between the steps vanish in the thermodynamic limit so that arbitrary small but finite variation of the field induce infinitely many level crossings in the thermodynamic limit leading to a static chaos effect which yields a self-averaging, smooth macroscopic response. We also note that there is a strong analogy between the problem of step-wise responses in glassy systems at mesoscopic scales and intermittency in turbulent flows due to shocks.Comment: 50 pages, 18 figures, revised versio

Growing correlations and aging of an elastic line in a random potential

We study the thermally assisted relaxation of a directed elastic line in a two dimensional quenched random potential by solving numerically the Edwards-Wilkinson equation and the Monte Carlo dynamics of a solid-on-solid lattice model. We show that the aging dynamics is governed by a growing correlation length displaying two regimes: an initial thermally dominated power-law growth which crosses over, at a static temperature-dependent correlation length $L_T \sim T^3$, to a logarithmic growth consistent with an algebraic growth of barriers. We present a scaling arguments to deal with the crossover-induced geometrical and dynamical effects. This analysis allows to explain why the results of most numerical studies so far have been described with effective power-laws and also permits to determine the observed anomalous temperature-dependence of the characteristic growth exponents. We argue that a similar mechanism should be at work in other disordered systems. We generalize the Family-Vicsek stationary scaling law to describe the roughness by incorporating the waiting-time dependence or age of the initial configuration. The analysis of the two-time linear response and correlation functions shows that a well-defined effective temperature exists in the power-law regime. Finally, we discuss the relevance of our results for the slow dynamics of vortex glasses in High-Tc superconductors.Comment: 18 pages, 15 figures, submitted for publicatio

Driven quantum coarsening

We study the driven dynamics of quantum coarsening. We analyze models of M-component rotors coupled to two electronic reservoirs at different chemical potentials that generate a current threading through the system. In the large M limit we derive the dynamical phase diagram as a function of temperature, strength of quantum fluctuations, voltage and coupling to the leads. We show that the slow relaxation in the ordering phase is universal. On large time and length scales the dynamics are analogous to stochastic classical ones, even for the quantum system driven out of equilibrium at zero temperature. We argue that our results apply to generic driven quantum coarsening.Comment: 4 pages, 3 figure