93 research outputs found
Spin-phonon coupled modes in the incommensurate phases of doped CuGeO
The doping effect of the folded phonon mode at 98 cm was investigated
on the Si-doped CuGeO by magneto-optical measurements in far-infrared (FIR)
region under high magnetic field. The folded phonon mode at 98 cm
appears not only in the dimerized (D) phase but also in the
dimerized-anitiferromagnetic (DAF) phase on the doped CuGeO. The splitting
was observed in the incommensurate (IC) phase and the antiferromagnetically
ordered incommensurate (IAF) phase above . The split-off branches exhibit
different field dependence from that of the pure CuGeO in the vicinity of
, and the discrepancy in the IAF phase is larger than that in the IC
phase. It is caused by the interaction between the solitons and the impurities.Comment: 7 pages, 4 figures, resubmitted to Phys. Rev.
Magnetic and Dielectric Properties in Multiferroic Cu3Mo2O9 under High Magnetic Fields
The magnetic and dielectric properties under high magnetic fields are studied
in the single crystal of Cu3Mo2O9. This multiferroic compound has distorted
tetrahedral spin chains. The effects of the quasi-one dimensionality and the
geometrical spin frustration are expected to appear simultaneously. We measure
the magnetoelectric current and the differential magnetization under the pulsed
magnetic field up to 74 T. We also measure the electric polarization versus the
electric field curve/loop under the static field up to 23 T. Dielectric
properties change at the magnetic fields where the magnetization jumps are
observed in the magnetization curve. Moreover, the magnetization plateaus are
found at high magnetic fields.Comment: 6 pages, 3 figures, in press in JPS Conf. Proc. as a part of SCES2013
Proceeding
Spin gap behavior and charge ordering in \alpha^{\prime}-NaV_2O_5 probed by light scattering
We present a detailed analysis of light scattering experiments performed on
the quarter-filled spin ladder compound -NaVO for
the temperature range 5 KT300 K. This system undergoes a phase
transition into a singlet ground state at T=34 K accompanied by the formation
of a super structure. For T34 K several new modes were detected. Three of
these modes are identified as magnetic bound states. Experimental evidence for
charge ordering on the V sites is detected as an anomalous shift and splitting
of a V-O vibration at 422 cm for temperatures above 34 K. The smooth and
crossover-like onset of this ordering at T= 80 K is accompanied by
pretransitional fluctuations both in magnetic and phononic Raman scattering. It
resembles the effect of stripe order on the super structure intensities in
LaNiO.Comment: 36 pages, 11 figures, accepted for publication in PRB (sept.99
Lattice vibrations of alpha'-NaV_2O_5 in the low-temperature phase. Magnetic bound states?
We report high resolution polarized infrared studies of the quarter-filled
spin ladder compound alpha'-NaV_2O_5 as a function of temperature (5K <= T <=
300K). Numerous new modes were detected below the temperature T_c=34K of the
phase transition into a charge ordered nonmagnetic state accompanied by a
lattice dimerization. We analyse the Brillouin zone (BZ) folding due to lattice
dimerization at T_c and show that some peculiarities of the low-temperature
vibrational spectrum come from quadruplets folded from the BZ point (1/2, 1/2,
1/4). We discuss an earlier interpretation of the 70, 107, and 133cm-1 modes as
magnetic bound states and propose the alternative interpretation as folded
phonon modes strongly interacting with charge and spin excitations.Comment: 15 pages, 13 Postscript figure
Raman Scattering in the Inorganic Spin-Peierls System alpha'-Na_{1-delta}V_2O_5
We have studied the spin-Peierls (SP) transition in alpha'-Na_{1-delta}V_2O_5
(delta = 0, 0.01 and 0.1) by means of Raman scattering. At room temperature, we
observe six A_1 and three A_2 phonon modes and a broad Raman band. Below
T_{SP}several new peaks and a new broad band appear. The new peak at 62 cm^{-1}
originates from the SP-gap excitation. The new peak at 128 cm^{-1} and the new
broad band between 130 and 400 cm^{-1} come from two magnetic excitations. The
new peaks at 102, 646 and 944 cm^{-1} are assigned to the folded phonon modes
and their Na^+-ion deficiency dependence shows that the defect of Na^+ ion
suppresses the SPtransition. The polarized Raman spectra below T_{SP} suggest
that the possible crystal symmetry is C_s^2(Pn) or C_1^1(P1). The asymmetric
lineshape of the 531-cm^{-1} peak superimposed on the electronic Raman band
from the d-d transition around 600 cm^{-1} is interpreted in terms of the Fano
resonance between the electronic continuous band and the phonon with a finite
lifetime. The defects of the Na^+ ions reduce the Fano effect because the life
time of the phonon and the phonon-continuum interaction are decreased.Comment: 24 pages, 10 Postscript figures,uses jpsj.sty and epsf.sty. in press
in J. Phys. Soc. Jp
Low-Lying Magnetic Excitation of the Shastry-Sutherland Model
By using perturbation calculation and numerical diagonalization, low-energy
spin dynamics of the Shastry-Sutherland model is investigated paying particular
attention to the two-particle coherent motion. In addition to spin-singlet- and
triplet bound states, we find novel branches of coherent motion of a bound
quintet pair, which are usually unstable because of repulsion. Unusual
dispersion observed in neutron-scattering measurements are explained by the
present theory. The importance of the effects of phonon is also pointed out.Comment: 4 pages, 6 figures combined into 1 PSfile. Final version to appear in
Phys.Rev.Lett. (Jan. 2000
Dynamics in the dimerised and high field incommensurate phase of CuGeO
Temperature (\ K) and magnetic field (\ T) dependent far
infrared absorption spectroscopy on the spin-Peierls coumpound CuGeO\ has
revealed several new absorption processes in both the dimerised and high field
phase of CuGeO. These results are discussed in terms of the modulation of
the CuGeO\ structure. At low fields this is the well known spin-Peierls
dimerisation. At high fields the data strongly suggests a field dependent
incommensurate modulation of the lattice as well as of the spin structure.Comment: 12 pages (revtex), 2 figures (eps), csh selfextracting .uu file, To
appear in PRB-Rapid Com
Folded modes in the infrared spectra of the spin-Peierls phase of CuGeO_3
Polarized far-infrared transmittance spectra of CuGeO_3 single crystals were
measured at different temperatures (6K < T < 300K). Two spectral lines, at
284.2 cm-1 in E||c polarization and at 311.7 cm-1 in E||b polarization, appear
at the temperature of the spin-Peierls transition and grow in intensity with
decreasing temperature. Both of them are, most probably, folded modes of the
dimerized lattice. We discuss a possible role of the spin-phonon interaction in
the formation of the 311.7 cm-1 feature.Comment: 4 pages, 5 figures, 1 table; Submitted to Phys.Rev.B Second revision.
Figures and text were slightly change
Charge Order Driven spin-Peierls Transition in NaV2O5
We conclude from 23Na and 51V NMR measurements in NaxV2O5(x=0.996) a charge
ordering transition starting at T=37 K and preceding the lattice distortion and
the formation of a spin gap Delta=106 K at Tc=34.7 K. Above Tc, only a single
Na site is observed in agreement with the Pmmn space group of this first
1/4-filled ladder system. Below Tc=34.7 K, this line evolves into eight
distinct 23Na quadrupolar split lines, which evidences a lattice distortion
with, at least, a doubling of the unit cell in the (a,b) plane. A model for
this unique transition implying both charge density wave and spin-Peierls order
is discussed.Comment: 4 pages, 3 figures, submitted to Phys. Rev. Let
Reexamination of the microscopic couplings of the quasi one-dimensional antiferromagnet CuGeO_3
Experimental data for the magnetic susceptibility and magnetostriction of
CuGeO_3 are analyzed within a one-dimensional antiferromagnetic model with
nearest ({J_1}) and next-nearest neighbour interactions ({J_2}). We show that
the ratio of the exchange constants in the antiferromagnetic chains of CuGeO_3
amounts to = 0.354(0.01), i.e. it is significantly larger than
the critical value for the formation of a spontaneous gap in the magnetic
excitation spectrum without lattice dimerization. The susceptibility data are
reproduced by our numerical results over the temperature range from 20K to 950K
to a high degree of accuracy for and .
The pressure dependence of the exchange constants is estimated from
magnetostriction data. Furthermore, the specific heat data are checked on
consistency against the calculated entropy of the above model.Comment: 9 pages, REVTEX, 5 figure
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