1,962 research outputs found
MBE-grown ZnO-based nanostructures for electronics applications
Low-dimensional semiconductors have properties di erent from their bulk counterparts and are thus attractive components for future electronic devices. This thesis presents work on ZnO nanostructures and ZnO/ZnMgO nano-heterostructures grown by molecular beam epitaxy (MBE) for electronics applications. ZnO nanostructures are grown by gold-catalysed MBE. We show that the cut of sapphire used as a substrate determines the orientation of one-dimensional nanostructure growth. On C-plane sapphire we grow ZnO nanowires and on R-plane sapphire we grow ZnO nanobelts. The morphology of nanobelts is shown to depend on temperature with tapering reduced at higher temperatures. Field-e ect transistors based on ZnO nanobelts are fabricated to characterize the electronic properties of single nanobelts. ZnO/ZnMgO heterostructure nanowires and nanobelts are grown and characterized. We show abrupt ZnO/ZnMgO interfaces and demonstrate that the core-shell structures in nanowires increase the luminescence intensity of nanowires. Nanobelt heterostructures are characterized optically at both room temperature and cryogenic temperatures showing evidence of quantum con nement in these structures. Scanning transmission electron microscope cathodoluminescence (CL) is performed on single ZnO nanowires. We perform hyperspectral mapping of CL, in which a single nanowire is spatially mapped with full CL spectra collected at each spatial co-ordinate on the nanowire. We achieve record resolution for hyperspectral mapping and deconvolve full spectra into constituent components. This allows us to distinguish surface and defect peaks as well as CL from inter-band processes in ZnO. We perform proof-of-principle studies combining high quality RF superconducting circuits with epitaxial ZnO layers on single sapphire substrates. Such chips can be used for future experiments coupling mechanical degrees of freedom to superconducting qubits for quantum opto-mechanical experiments
Spin resonance linewidths of bismuth donors in silicon coupled to planar microresonators
Ensembles of bismuth donor spins in silicon are promising storage elements
for microwave quantum memories due to their long coherence times which exceed
seconds. Operating an efficient quantum memory requires achieving critical
coupling between the spin ensemble and a suitable high-quality factor resonator
-- this in turn requires a thorough understanding of the lineshapes for the
relevant spin resonance transitions, particularly considering the influence of
the resonator itself on line broadening. Here, we present pulsed electron spin
resonance measurements of ensembles of bismuth donors in natural silicon, above
which niobium superconducting resonators have been patterned. By studying spin
transitions across a range of frequencies and fields we identify distinct line
broadening mechanisms, and in particular those which can be suppressed by
operating at magnetic-field-insensitive `clock transitions'. Given the donor
concentrations and resonator used here, we measure a cooperativity
and based on our findings we discuss a route to achieve unit cooperativity, as
required for a quantum memory
Tunable Nb superconducting resonators based upon a Ne-FIB-fabricated constriction nanoSQUID
Hybrid superconducting--spin systems offer the potential to combine highly
coherent atomic quantum systems with the scalability of superconducting
circuits. To fully exploit this potential requires a high quality-factor
microwave resonator, tunable in frequency and able to operate at magnetic
fields optimal for the spin system. Such magnetic fields typically rule out
conventional Al-based Josephson junction devices that have previously been used
for tunable high- microwave resonators. The larger critical field of niobium
(Nb) allows microwave resonators with large field resilience to be fabricated.
Here, we demonstrate how constriction-type weak links, patterned in parallel
into the central conductor of a Nb coplanar resonator using a neon focused ion
beam (FIB), can be used to implement a frequency-tunable resonator. We study
transmission through two such devices and show how they realise high quality
factor, tunable, field resilient devices which hold promise for future
applications coupling to spin systems
Coherent spin dynamics of rare-earth doped crystals in the high-cooperativity regime
Rare-earth doped crystals have long coherence times and the potential to
provide quantum interfaces between microwave and optical photons. Such
applications benefit from a high cooperativity between the spin ensemble and a
microwave cavity -- this motivates an increase in the rare earth ion
concentration which in turn impacts the spin coherence lifetime. We measure
spin dynamics of two rare-earth spin species, Nd and Yb doped into
YSiO, coupled to a planar microwave resonator in the high
cooperativity regime, in the temperature range 1.2 K to 14 mK. We identify
relevant decoherence mechanisms including instantaneous diffusion arising from
resonant spins and temperature-dependent spectral diffusion from impurity
electron and nuclear spins in the environment. We explore two methods to
mitigate the effects of spectral diffusion in the Yb system in the
low-temperature limit, first, using magnetic fields of up to 1 T to suppress
impurity spin dynamics and, second, using transitions with low effective
g-factors to reduce sensitivity to such dynamics. Finally, we demonstrate how
the `clock transition' present in the Yb system at zero field can be
used to increase coherence times up to ms.Comment: 8 pages, 5 figure
Random-access quantum memory using chirped pulse phase encoding
Quantum memories capable of faithfully storing and recalling quantum states
on-demand are powerful ingredients in bulding quantum networks
[arXiv:0806.4195] and quantum information processors [arXiv:1109.3743]. As in
conventional computing, key attributes of such memories are high storage
density and, crucially, random access, or the ability to read from or write to
an arbitrarily chosen register. However, achieving such random access with
quantum memories [arXiv:1904.09643] in a dense, hardware-efficient manner
remains a challenge, for example requiring dedicated cavities per qubit
[arXiv:1109.3743] or pulsed field gradients [arXiv:0908.0101]. Here we
introduce a protocol using chirped pulses to encode qubits within an ensemble
of quantum two-level systems, offering both random access and naturally
supporting dynamical decoupling to enhance the memory lifetime. We demonstrate
the protocol in the microwave regime using donor spins in silicon coupled to a
superconducting cavity, storing up to four multi-photon microwave pulses and
retrieving them on-demand up to 2~ms later. A further advantage is the natural
suppression of superradiant echo emission, which we show is critical when
approaching unit cooperativity. This approach offers the potential for
microwave random access quantum memories with lifetimes exceeding seconds
[arXiv:1301.6567, arXiv:2005.09275], while the chirped pulse phase encoding
could also be applied in the optical regime to enhance quantum repeaters and
networks
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Strain in heterogeneous quantum devices with atomic layer deposition
Abstract: We investigated the use of dielectric layers produced by atomic layer deposition (ALD) as an approach to strain mitigation in composite silicon/superconductor devices operating at cryogenic temperatures. We show that the addition of an ALD layer acts to reduce the strain of spins closest to silicon/superconductor interface where strain is highest. We show that appropriately biasing our devices at the hyperfine clock transition of bismuth donors in silicon, we can remove strain broadening and that the addition of ALD layers left T 2 (or temporal inhomogeneities) unchanged in these natural silicon devices
Probing spin dynamics of ultra-thin van der Waals magnets via photon-magnon coupling
Layered van der Waals (vdW) magnets can maintain a magnetic order even down to the single-layer regime and hold promise for integrated spintronic devices. While the magnetic ground state of vdW magnets was extensively studied, key parameters of spin dynamics, like the Gilbert damping, crucial for designing ultra-fast spintronic devices, remains largely unexplored. Despite recent studies by optical excitation and detection, achieving spin wave control with microwaves is highly desirable, as modern integrated information technologies predominantly are operated with these. The intrinsically small numbers of spins, however, poses a major challenge to this. Here, we present a hybrid approach to detect spin dynamics mediated by photon-magnon coupling between high-Q superconducting resonators and ultra-thin flakes of Cr2Ge2Te6 (CGT) as thin as 11 nm. We test and benchmark our technique with 23 individual CGT flakes and extract an upper limit for the Gilbert damping parameter. These results are crucial in designing on-chip integrated circuits using vdW magnets and offer prospects for probing spin dynamics of monolayer vdW magnets
AMR, stability and higher accuracy
Efforts to achieve better accuracy in numerical relativity have so far
focused either on implementing second order accurate adaptive mesh refinement
or on defining higher order accurate differences and update schemes. Here, we
argue for the combination, that is a higher order accurate adaptive scheme.
This combines the power that adaptive gridding techniques provide to resolve
fine scales (in addition to a more efficient use of resources) together with
the higher accuracy furnished by higher order schemes when the solution is
adequately resolved. To define a convenient higher order adaptive mesh
refinement scheme, we discuss a few different modifications of the standard,
second order accurate approach of Berger and Oliger. Applying each of these
methods to a simple model problem, we find these options have unstable modes.
However, a novel approach to dealing with the grid boundaries introduced by the
adaptivity appears stable and quite promising for the use of high order
operators within an adaptive framework
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