Large magnetic field-induced spectral weight enhancement of high-energy spin excitations in La1.88Sr0.12CuO4La_{1.88}Sr_{0.12}CuO_{4}

We report electronic Raman scattering experiments on a superconducting ${\rm La_{1.88}Sr_{0.12}CuO_{4}}$ single crystal in a magnetic field. At low temperatures, the spectral weight of the high-energy two-magnon peak increases linearly with field and is amplified by a factor of more than two at 14 T. The effect disappears at elevated temperatures and is not present in undoped ${\rm La_{2}CuO_{4}}$. This observation is discussed in terms of an electronically inhomogeneous state in which the field enhances the volume fraction of a phase with local antiferromagnetic order at the expense of the superconducting phase.Comment: to appear in PR

Spin-Wave Lifetimes Throughout the Brillouin Zone

We use a neutron spin-echo method with $\mu$eV resolution to determine the lifetimes of spin waves in the prototypical antiferromagnet MnF$_2$ over the entire Brillouin zone. A theory based on the interaction of magnons with longitudinal spin fluctuations provides an excellent, parameter-free description of the data, except at the lowest momenta and temperatures. This is surprising, given the prominence of alternative theories based on magnon-magnon interactions in the literature. The results and technique open up a new avenue for the investigation of fundamental concepts in magnetism. The technique also allows measurement of the lifetimes of other elementary excitations (such as lattice vibrations) throughout the Brillouin zone.Comment: 12 pages, 4 figure

Neutron spin-echo study of the critical dynamics of spin-5/2 antiferromagnets in two and three dimensions

We report a neutron spin-echo study of the critical dynamics in the $S=5/2$ antiferromagnets MnF$_2$ and Rb$_2$MnF$_4$ with three-dimensional (3D) and two-dimensional (2D) spin systems, respectively, in zero external field. Both compounds are Heisenberg antiferromagnets with a small uniaxial anisotropy resulting from dipolar spin-spin interactions, which leads to a crossover in the critical dynamics close to the N\'eel temperature, $T_N$. By taking advantage of the $\mu\text{eV}$ energy resolution of the spin-echo spectrometer, we have determined the dynamical critical exponents $z$ for both longitudinal and transverse fluctuations. In MnF$_2$, both the characteristic temperature for crossover from 3D Heisenberg to 3D Ising behavior and the exponents $z$ in both regimes are consistent with predictions from the dynamical scaling theory. The amplitude ratio of longitudinal and transverse fluctuations also agrees with predictions. In Rb$_2$MnF$_4$, the critical dynamics crosses over from the expected 2D Heisenberg behavior for $T\gg T_N$ to a scaling regime with exponent $z = 1.387(4)$, which has not been predicted by theory and may indicate the influence of long-range dipolar interactions

Coherent Modulation of the YBa2Cu3O6+x Atomic Structure by Displacive Stimulated Ionic Raman Scattering

We discuss the mechanism of coherent phonon generation by Stimulated Ionic Raman Scattering, a process different from conventional excitation with near visible optical pulses. Ionic Raman scattering is driven by anharmonic coupling between a directly excited infrared-active phonon mode and other Raman modes. We experimentally study the response of YBa2Cu3O6+x to the resonant excitation of apical oxygen motions at 20 THz by mid-infrared pulses, which has been shown in the past to enhance the interlayer superconducting coupling. We find coherent oscillations of four totally symmetric (Ag) Raman modes and make a critical assessment of the role of these oscillatory motions in the enhancement of superconductivity.Comment: 12 pages, 4 figure