Are all maximally entangled states pure?

We study if all maximally entangled states are pure through several entanglement monotones. In the bipartite case, we find that the same conditions which lead to the uniqueness of the entropy of entanglement as a measure of entanglement, exclude the existence of maximally mixed entangled states. In the multipartite scenario, our conclusions allow us to generalize the idea of monogamy of entanglement: we establish the \textit{polygamy of entanglement}, expressing that if a general state is maximally entangled with respect to some kind of multipartite entanglement, then it is necessarily factorized of any other system.Comment: 5 pages, 1 figure. Proof of theorem 3 corrected e new results concerning the asymptotic regime include

Separable approximation for mixed states of composite quantum systems

We describe a purely algebraic method for finding the best separable approximation to a mixed state of a composite 2x2 quantum system, consisting of a decomposition of the state into a linear combination of a mixed separable part and a pure entangled one. We prove that, in a generic case, the weight of the pure part in the decomposition equals the concurrence of the state.Comment: 13 pages, no figures; minor changes; accepted for publication in PR

Reflections upon separability and distillability

We present an abstract formulation of the so-called Innsbruck-Hannover programme that investigates quantum correlations and entanglement in terms of convex sets. We present a unified description of optimal decompositions of quantum states and the optimization of witness operators that detect whether a given state belongs to a given convex set. We illustrate the abstract formulation with several examples, and discuss relations between optimal entanglement witnesses and n-copy non-distillable states with non-positive partial transpose.Comment: 12 pages, 7 figures, proceedings of the ESF QIT Conference Gdansk, July 2001, submitted to special issue of J. Mod. Op

Schmidt balls around the identity

Robustness measures as introduced by Vidal and Tarrach [PRA, 59, 141-155] quantify the extent to which entangled states remain entangled under mixing. Analogously, we introduce here the Schmidt robustness and the random Schmidt robustness. The latter notion is closely related to the construction of Schmidt balls around the identity. We analyse the situation for pure states and provide non-trivial upper and lower bounds. Upper bounds to the random Schmidt-2 robustness allow us to construct a particularly simple distillability criterion. We present two conjectures, the first one is related to the radius of inner balls around the identity in the convex set of Schmidt number n-states. We also conjecture a class of optimal Schmidt witnesses for pure states.Comment: 7 pages, 1 figur

Two-Photon Oxygen Sensing with Quantum Dot-Porphyrin Conjugates

Supramolecular assemblies of a quantum dot (QD) associated to palladium(II) porphyrins have been developed to detect oxygen (pO2) in organic solvents. Palladium porphyrins are sensitive in the 0–160 torr range, making them ideal phosphors for in vivo biological oxygen quantification. Porphyrins with meso pyridyl substituents bind to the surface of the QD to produce self–assembled nanosensors. Appreciable overlap between QD emission and porphyrin absorption features results in efficient Förster resonance energy transfer (FRET) for signal transduction in these sensors. The QD serves as a photon antenna, enhancing porphyrin emission under both one– and two–photon excitation, demonstrating that QD–palladium porphyrin conjugates may be used for oxygen sensing over physiological oxygen ranges.Chemistry and Chemical Biolog

Micelle-Encapsulated Quantum Dot-Porphyrin Assemblies as

Micelles have been employed to encapsulate the supramolecular assembly of quantum dots with palladium(II) porphyrins for the quantification of O₂ levels in aqueous media and in vivo. Förster resonance energy transfer from the quantum dot (QD) to the palladium porphyrin provides a means for signal transduction under both one- and two-photon excitation. The palladium porphyrins are sensitive to O₂ concentrations in the range of 0–160 Torr. The micelle-encapsulated QD-porphyrin assemblies have been employed for in vivo multiphoton imaging and lifetime-based oxygen measurements in mice with chronic dorsal skinfold chambers or cranial windows. Our results establish the utility of the QD-micelle approach for in vivo biological sensing applications.National Cancer Institute (U.S.) (R01- CA126642)International Society for Neurochemistry (W911NF-07-D-0004)United States. Dept. of Energy. Office of Basic Energy Sciences (DE-SC0009758

Separability in 2xN composite quantum systems

We analyze the separability properties of density operators supported on \C^2\otimes \C^N whose partial transposes are positive operators. We show that if the rank of $\rho$ equals N then it is separable, and that bound entangled states have rank larger than N. We also give a separability criterion for a generic density operator such that the sum of its rank and the one of its partial transpose does not exceed 3N. If it exceeds this number we show that one can subtract product vectors until decreasing it to 3N, while keeping the positivity of $\rho$ and its partial transpose. This automatically gives us a sufficient criterion for separability for general density operators. We also prove that all density operators that remain invariant after partial transposition with respect to the first system are separable.Comment: Extended version of quant-ph/9903012 with new results. 11 page

Separable approximations of density matrices of composite quantum systems

We investigate optimal separable approximations (decompositions) of states rho of bipartite quantum systems A and B of arbitrary dimensions MxN following the lines of Ref. [M. Lewenstein and A. Sanpera, Phys. Rev. Lett. 80, 2261 (1998)]. Such approximations allow to represent in an optimal way any density operator as a sum of a separable state and an entangled state of a certain form. For two qubit systems (M=N=2) the best separable approximation has a form of a mixture of a separable state and a projector onto a pure entangled state. We formulate a necessary condition that the pure state in the best separable approximation is not maximally entangled. We demonstrate that the weight of the entangled state in the best separable approximation in arbitrary dimensions provides a good entanglement measure. We prove in general for arbitrary M and N that the best separable approximation corresponds to a mixture of a separable and an entangled state which are both unique. We develop also a theory of optimal separable approximations for states with positive partial transpose (PPT states). Such approximations allow to decompose any density operator with positive partial transpose as a sum of a separable state and an entangled PPT state. We discuss procedures of constructing such decompositions.Comment: 12 pages, 2 figure

Separability and entanglement in 2x2xN composite quantum systems

We investigate separability and entanglement of mixed states in ${\cal C}^2\otimes{\cal C}^2\otimes{\cal C}^N$ three party quantum systems. We show that all states with positive partial transposes that have rank $\le N$ are separable. For the 3 qubit case (N=2) we prove that all states $\rho$ that have positive partial transposes and rank 3 are separable. We provide also constructive separability checks for the states $\rho$ that have the sum of the rank of $\rho$ and the ranks of partial transposes with respect to all subsystems smaller than 15N-1.Comment: Finally corrected file submitted. Numerous misprints and small errors corrected, better versions of constructive separability checks included, updated and extended reference