Long-range and short-range magnetic correlations, and microscopic origin of net magnetization in the spin-1 trimer chain compound CaNi3P4O14

Spin-spin correlations and microscopic origin of net magnetization in the spin-1 trimer chain compound CaNi3P4O14 have been investigated by powder neutron diffraction. The present study reveals a 3D long-range magnetic ordering below 16 K where the magnetic structure consists of ferromagnetic trimers that are coupled ferromagnetically along the spin-chain. The moment components along the a and c axes arrange antiferromagnetically. Our study establishes that the uncompensated moment components along the b axis result in a net magnetization per unit cell. The magnetic structure, determined in the present study, is in agreement with the results of recent first principles calculation; however, it is in contrast to a fascinating experimental prediction of ferrimagnetic ordering based on the periodicity of the exchange interactions in CaNi3P4O14. Our study also confirms the presence of broad diffuse magnetic scattering, due to 1D short-range spin-spin correlations, over a wide temperature range below ~50 K down to a temperature well below the Tc. Total neutron scattering analysis by the RMC method reveals that the dominating spin-spin correlation above Tc is ferromagnetic and along the b axis. The nearest neighbour spin-spin correlations along the a and c axes are found to be weakly antiferromagnetic. The nature of the trimer spin structure of the short-range state is similar to that of the 3D long-range ordered state. The present investigation of microscopic nature of the magnetic ground state also explains the condition required for the 1/3 magnetization plateau to be observed in the trimer spin-chains. In spite of the S=1 trimer chain system, the present compound CaNi3P4O14 is found to be a good realization of 3D magnet below the Tc=16 K with full ordered moment values of ~2 mu_B/Ni2+ (1.98 and 1.96 mu_B/Ni2+ for two Ni sites, respectively) at 1.5 K.Comment: 10 pages, 8 figure

Widespread HCN maser emission in carbon-rich evolved stars

Context. HCN is a major constituent of the circumstellar envelopes of carbon-rich evolved stars, and rotational lines from within its vibrationally excited states probe parts of these regions closest to the stellar surface. A number of such lines are known to show maser action. Historically, in one of them, the 177 GHz $J=2\rightarrow1$ line in the $l$-doubled bending mode has been found to show relatively strong maser action, with results only published for a single object, the archetypical high-mass loss asymptotic giant branch (AGB) star IRC+10216. Aims. To examine how common 177 GHz HCN maser emission is, we conducted an exploratory survey for this line toward a select sample of carbon-rich asymptotic giant branch stars that are observable from the southern hemisphere. Methods. We used the Atacama Pathfinder Experiment 12 meter submillimeter Telescope (APEX) equipped with a new receiver to simultaneously observe three $J=2\rightarrow1$ HCN rotational transitions, the $(0,1^{{1}_{\rm c}},0)$ and $(0,1^{{1}_{\rm d}},0)$ $l$-doublet components, and the line from the (0,0,0) ground state. Results. The $(0,1^{{1}_{\rm c}},0)$ maser line is detected toward 11 of 13 observed sources, which all show emission in the (0,0,0) transition. In most of the sources, the peak intensity of the $(0,1^{{1}_{\rm c}},0)$ line rivals that of the (0,0,0) line; in two sources, it is even stronger. Except for the object with the highest mass-loss rate, IRC+10216, the $(0,1^{{1}_{\rm c}},0)$ line covers a smaller velocity range than the (0,0,0) line. Conclusions. Maser emission in the 177 GHz $J=2\rightarrow1$ $(0,1^{{1}_{\rm c}},0)$ line of HCN appears to be common in carbon-rich AGB stars. (Abbreviated)Comment: 12 pages (including appendix), 3 figures / Astronomy & Astrophysics (in press

^25Mg NMR study of the MgB_2 superconductor

^25Mg NMR spectra and nuclear spin-lattice relaxation time, T_1, have been measured in polycrystalline ^25MgB_2 with a superconducting transition temperature T_c = 39.0 K in zero magnetic field. From the first order and second order quadrupole perturbed NMR spectrum a quadrupole coupling frequency nu_Q = 222(1.5) kHz is obtained. T_1T = 1090(50) sK and Knight shift K_c = 242(4) ppm are temperature independent in the normal conducting phase. The ^25Mg Korringa ratio equals to 0.95 which is very close to the ideal value of unity for s-electrons. The comparison of the experimental nu_Q, T_1T, and K_c with the corresponding values obtained by LDA calculations shows an excellent agreement for all three quantities.Comment: 4 pages including 4 eps-figures, revtex

Energy Gaps and Kohn Anomalies in Elemental Superconductors

The momentum and temperature dependence of the lifetimes of acoustic phonons in the elemental superconductors Pb and Nb was determined by resonant spin-echo spectroscopy with neutrons. In both elements, the superconducting energy gap extracted from these measurements was found to converge with sharp anomalies originating from Fermi-surface nesting (Kohn anomalies) at low temperatures. The results indicate electron many-body correlations beyond the standard theoretical framework for conventional superconductivity. A possible mechanism is the interplay between superconductivity and spin- or charge-density-wave fluctuations, which may induce dynamical nesting of the Fermi surface

Arrays of Josephson junctions in an environment with vanishing impedance

The Hamiltonian operator for an unbiased array of Josephson junctions with gate voltages is constructed when only Cooper pair tunnelling and charging effects are taken into account. The supercurrent through the system and the pumped current induced by changing the gate voltages periodically are discussed with an emphasis on the inaccuracies in the Cooper pair pumping. Renormalisation of the Hamiltonian operator is used in order to reliably parametrise the effects due to inhomogeneity in the array and non-ideal gating sequences. The relatively simple model yields an explicit, testable prediction based on three experimentally motivated and determinable parameters.Comment: 13 pages, 9 figures, uses RevTeX and epsfig, Revised version, Better readability and some new result

Correlation between oxygen isotope effects on the transition temperature and the magnetic penetration depth in high-temperature superconductors close to optimal doping

The oxygen-isotope (^{16}O/^{18}O) effect (OIE) on the in-plane magnetic penetration depth \lambda_{ab}(0) in optimally-doped YBa_2Cu_3O_{7-\delta} and La_{1.85}Sr_{0.15}CuO_4, and in slightly underdoped YBa_2Cu_4O_8 and Y_{0.8}Pr_{0.2}Ba_2Cu_3O_{7-\delta} was studied by means of muon-spin rotation. A substantial OIE on \lambda_{ab}(0) with an OIE exponent \beta_O=-d\ln\lambda_{ab}(0)/d\ln M_O\approx - 0.2 (M_O is the mass of the oxygen isotope), and a small OIE on the transition temperature T_c with an OIE exponent \alpha_O=-d\ln T_{c}/d \ln M_O\simeq0.02 to 0.1 were observed. The observation of a substantial isotope effect on \lambda_{ab}(0), even in cuprates where the OIE on T_c is small, indicates that lattice effects play an important role in cuprate HTS.Comment: 6 pages, 4 figure

Stellar Associations and their Field East of LMC 4 in the Large Magellanic Cloud

We report about the stellar content and the luminosity and mass functions of three stellar associations and their field located on the north-east edge of the super-bubble LMC 4 in the Large Magellanic Cloud.Comment: To be appeared in the meeting Proceedings of ``Modes of Star Formation and the Origin of Field Populations'', Heidelberg, Germany, October 2000; to be published in the ASP Conference Series, edited by E. K. Grebel and W. Brandne

Collinear order in a frustrated three-dimensional spin-12\frac12 antiferromagnet Li2_2CuW2_2O8_8

Magnetic frustration in three dimensions (3D) manifests itself in the spin-$\frac12$ insulator Li$_2$CuW$_2$O$_8$. Density-functional band-structure calculations reveal a peculiar spin lattice built of triangular planes with frustrated interplane couplings. The saturation field of 29 T contrasts with the susceptibility maximum at 8.5 K and a relatively low N\'eel temperature $T_N\simeq 3.9$ K. Magnetic order below $T_N$ is collinear with the propagation vector $(0,\frac12,0)$ and an ordered moment of 0.65(4) $\mu_B$ according to neutron diffraction data. This reduced ordered moment together with the low maximum of the magnetic specific heat ($C^{\max}/R\simeq 0.35$) pinpoint strong magnetic frustration in 3D. Collinear magnetic order suggests that quantum fluctuations play crucial role in this system, where a non-collinear spiral state would be stabilized classically.Comment: published version with supplemental material merged into the tex