946 research outputs found
Stark effect of excitons in individual air-suspended carbon nanotubes
We investigate electric-field induced redshifts of photoluminescence from
individual single-walled carbon nanotubes. The shifts scale quadratically with
field, while measurements with different excitation powers and energies show
that effects from heating and relaxation pathways are small. We attribute the
shifts to the Stark effect, and characterize nanotubes with different
chiralities. By taking into account exciton binding energies for air-suspended
tubes, we find that theoretical predictions are in quantitative agreement.Comment: 4 pages, 3 figure
Spontaneous exciton dissociation in carbon nanotubes
Simultaneous photoluminescence and photocurrent measurements on individual
single-walled carbon nanotubes reveal spontaneous dissociation of excitons into
free electron-hole pairs. Correlation of luminescence intensity and
photocurrent shows that a significant fraction of excitons are dissociating
during their relaxation into the lowest exciton state. Furthermore, the
combination of optical and electrical signals also allows for extraction of the
absorption cross section and the oscillator strength. Our observations explain
the reasons for photoconductivity measurements in single-walled carbon
nanotubes being straightforward despite the large exciton binding energies.Comment: 4 pages, 3 figure
Gate-controlled generation of optical pulse trains using individual carbon nanotubes
We report on optical pulse-train generation from individual air-suspended
carbon nanotubes under an application of square-wave gate voltages.
Electrostatically-induced carrier accummulation quenches photoluminescence,
while a voltage sign reversal purges those carriers, resetting the nanotubes to
become luminescent temporarily. Frequency domain measurements reveal
photoluminescence recovery with characteristic frequencies that increase with
excitation laser power, showing that photoexcited carriers quench the emission
in a self-limiting manner. Time-resolved measurements directly confirm the
presence of an optical pulse train sychronized to the gate voltage signal, and
flexible control over pulse timing and duration is demonstrated.Comment: 4 pages, 4 figure
Lack of antigen-specific tissue remodeling in mice deficient in the macrophage galactose-type calcium-type lectin 1/CD301a.
Macrophage galactose-type C-type lectins (MGLs), which were recently named CD301, have 2 homologues in mice: MGL1 and MGL2. MGLs are expressed on macrophages and immature dendritic cells. The persistent presence of granulation tissue induced by a protein antigen was observed in wild-type mice but not in mice lacking an endogenous, macrophage-specific, galactose-type calcium-type lectin 1 (MGL1) in an air pouch model. The anti-MGL1 antibody suppressed the granulation tissue formation in wild-type mice. A large number of cells, present only in the pouch of MGL1-deficient mice, were not myeloid or lymphoid lineage cells and the number significantly declined after administration of interleukin 1 alpha (IL-1alpha) into the pouch of MGL1-deficient mice. Furthermore, granulation tissue was restored by this treatment and the cells obtained from the pouch of MGL1-deficient mice were incorporated into the granulation tissue when injected with IL-1alpha. Taken together, MGL1 expressed on a specific subpopulation of macrophages that secrete IL-1alpha was proposed to regulate specific cellular interactions crucial to granulation tissue formation
Stark effect of excitons in individual air-suspended carbon nanotubes
We investigate electric-field induced redshifts of photoluminescence from individual single-walled carbon nanotubes. The shifts scale quadratically with field, while measurements with different excitation powers and energies show that effects from heating and relaxation pathways are small. We attribute the shifts to the Stark effect and characterize nanotubes with different chiralities. By taking into account exciton binding energies for air-suspended tubes, we find that theoretical predictions are in quantitative agreement
Spontaneous Exciton Dissociation in Carbon Nanotubes
Simultaneous photoluminescence and photocurrent measurements on individual single-walled carbon nanotubes reveal spontaneous dissociation of excitons into free electron-hole pairs. The correlation of luminescence intensity and photocurrent shows that a significant fraction of excitons are dissociating before recombination. Furthermore, the combination of optical and electrical signals also allows for extraction of the absorption cross section and the oscillator strength. Our observations explain the reasons why photoconductivity measurements in single-walled carbon nanotubes are straightforward despite the large exciton binding energies
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