112 research outputs found
Superconducting Gap Structure of kappa-(BEDT-TTF)2Cu(NCS)2 Probed by Thermal Conductivity Tensor
The thermal conductivity of organic superconductor kappa-(BEDT-TTF)2Cu(NCS)2
(Tc =10.4 K) has been studied in a magnetic field rotating within the 2D
superconducting planes with high alignment precision. At low temperatures (T <
0.5 K), a clear fourfold symmetry in the angular variation, which is
characteristic of a d-wave superconducting gap with nodes along the directions
rotated 45 degrees relative to the b and c axes of the crystal, was resolved.
The determined nodal structure is inconsistent with recent theoretical
predictions of superconductivity induced by the antiferromagnetic spin
fluctuation.Comment: 5 pages, 4 figures, to be published in Phys. Rev. Let
Magnetic Field-Induced Superconductor-Insulator-Metal Transition in an Organic Conductor: An Infrared Magneto-Optical Imaging Spectroscopy
The magnetic field-induced superconductor-insulator-metal transition (SIMT)
in partially deuterated -(BEDT-TTF)Cu[N(CN)]Br, which is just
on the Mott boundary, has been observed using the infrared magneto-optical
imaging spectroscopy. The infrared reflectivity image on the sample surface
revealed that the metallic (or superconducting) and insulating phases coexist
and they have different magnetic field dependences. One of the magnetic field
dependence is SIMT that appeared on part of the sample surface. The SIMT was
concluded to originate from the balance of the inhomogenity in the sample
itself and the disorder of the ethylene end groups resulting from fast cooling.Comment: 5 pages, 5 figures, to appear in Phys. Rev.
Dynamical mean field study of the Mott transition in the half-filled Hubbard model on a triangular lattice
We employ dynamical mean field theory (DMFT) with a Quantum Monte Carlo (QMC)
atomic solver to investigate the finite temperature Mott transition in the
Hubbard model with the nearest neighbor hopping on a triangular lattice at
half-filling. We estimate the value of the critical interaction to be in units of the hopping amplitude through the evolution of the
magnetic moment, spectral function, internal energy and specific heat as the
interaction and temperature are varied. This work also presents a
comparison between DMFT and finite size determinant Quantum Monte Carlo (DQMC)
and a discussion of the advantages and limitations of both methods.Comment: 7 pages, 5 figure
C NMR observation of a nonmagnetic charge-ordered state in the organic conductor -(ET)Hg(SCN)Cl
We investigated the local magnetism of the organic conductor,
-(ET)Hg(SCN)Cl, with a quasi-triangular lattice of weakly
dimerized molecules through C NMR spectroscopy. The NMR spectra and
nuclear relaxation show that charge disproportionation occurs, associated with
the metal-insulator transition at 31 K. The relaxation rate indicates that the
paramagnetic spins in the insulating phase undergo a transition into a
spin-singlet ground state with the emergence of orphan spins, a possible
valence-bond-glass state. The present results are in high contrast to the
spin-cluster paramagnetism of the electric dipole-liquid candidate,
--(ET)Hg(SCN)Br, having nearly identical material
parameters. This fact indicates that these two systems are on the verge between
distinct phases in both charge and spin degrees of freedom; a spin-singlet
charge-ordered state versus a spin-active Mott insulating state, competing with
each other on a triangular lattice of dimerized sites
Frustrated Spin System in theta-(BEDT-TTF)_2RbZn(SCN)_4
The origin of the spin gap behavior in the low-temperature dimerized phase of
theta-(BEDT-TTF)_2RbZn(SCN)_4 has been theoretically studied based on the
Hartree-Fock approximation for the on-site Coulomb interaction at absolute
zero. Calculations show that, in the parameter region considered to be relevant
to this compound, antiferromagnetic ordering is stabilized between dimers
consisting of pairs of molecules coupled with the largest transfer integral.
Based on this result an effective localized spin 1/2 model is constructed which
indicates the existence of the frustration among spins. This frustration may
result in the formation of spin gap.Comment: 4 pages, 5 figures, to be published in J. Phys. Soc. Jpn. 67 (1998)
no.
Anisotropic charge dynamics in the quantum spin-liquid candidate -(BEDT-TTF)Cu(CN)
We have in detail characterized the anisotropic charge response of the dimer
Mott insulator -(BEDT-TTF)\-Cu(CN) by dc conductivity, Hall
effect and dielectric spectroscopy. At room temperature the Hall coefficient is
positive and close to the value expected from stoichiometry; the temperature
behavior follows the dc resistivity . Within the planes the dc
conductivity is well described by variable-range hopping in two dimensions;
this model, however, fails for the out-of-plane direction. An unusually broad
in-plane dielectric relaxation is detected below about 60 K; it slows down much
faster than the dc conductivity following an Arrhenius law. At around 17 K we
can identify a pronounced dielectric anomaly concomitantly with anomalous
features in the mean relaxation time and spectral broadening. The out-of-plane
relaxation, on the other hand, shows a much weaker dielectric anomaly; it
closely follows the temperature behavior of the respective dc resistivity. At
lower temperatures, the dielectric constant becomes smaller both within and
perpendicular to the planes; also the relaxation levels off. The observed
behavior bears features of relaxor-like ferroelectricity. Because
heterogeneities impede its long-range development, only a weak tunneling-like
dynamics persists at low temperatures. We suggest that the random potential and
domain structure gradually emerge due to the coupling to the anion network.Comment: 14 pages, 13 figure
Multiple Superconducting Phases in New Heavy Fermion Superconductor PrOs4Sb12
The superconducting gap structure of recently discovered heavy fermion
superconductor PrOs4Sb12 was investigated by using thermal transport
measurements in magnetic field rotated relative to the crystal axes. We
demonstrate that a novel change in the symmetry of the superconducting gap
function occurs deep inside the superconducting state, giving a clear
indication of the presence of two distinct superconducting phases with twofold
and fourfold symmetries. We infer that the gap functions in both phases have a
point node singularity, in contrast to the familiar line node singularity
observed in almost all unconventional superconductors.Comment: 4 Pages, 4 Figure
Phase Diagram of -(BEDT-TTF)ICl under High Pressure Based on the First-Principles Electronic Structure
We present a theoretical study on the superconductivity of
-(BEDT-TTF)ICl at 14.2 K under a high hydrostatic
pressure recently found, which is the highest among organic superconductors. In
the present work, we study an effective model using the fluctuation-exchange
(FLEX) approximation based on the results of first-principles calculation. In
the obtained phase diagram, the superconductivity with -like symmetry
is realized next to the antiferromagnetic phase, as a result of the
one-dimensional to two-dimensional crossover driven by the pressure.Comment: 4 pages, 3 figures. accepted for publication in J. Phys. Soc. Jpn.
errors correcte
Dynamic Exponent of t-J and t-J-W Model
Drude weight of optical conductivity is calculated at zero temperature by
exact diagonalization for the two-dimensional t-J model with the two-particle
term, . For the ordinary t-J model with =0, the scaling of the Drude
weight for small doping concentration is
obtained, which indicates anomalous dynamic exponent =4 of the Mott
transition. When is switched on, the dynamic exponent recovers its
conventional value =2. This corresponds to an incoherent-to-coherent
transition associated with the switching of the two-particle transfer.Comment: LaTeX, JPSJ-style, 4 pages, 5 eps files, to appear in J. Phys. Soc.
Jpn. vol.67, No.6 (1998
NMR Evidence for Antiferromagnetic Transition in the Single-Component Molecular Conductor, [Au(tmdt)_{2}] at 110 K
We present the results of a ^{1}H NMR study of the single-component molecular
conductor, [Au(tmdt)_{2}].
A steep increase in the NMR line width and a peak formation of the nuclear
spin-lattice relaxation rate, 1/T_{1}, were observed at around 110 K.
This behavior provides clear and microscopic evidences for a magnetic phase
transition at considerably high temperature among organic conductors.
The observed variation in 1/T_{1} with respect to temperature indicates the
highly correlated nature of the metallic phase.Comment: 5pages, 6figures to be published in J. Phys. Soc. Jp
- …