52 research outputs found

    t-J model of coupled Cu2_2O5_5 ladders in Sr14−x_{14-x}Cax_xCu24_{24}O41_{41}

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    Starting from the proper charge transfer model for Cu2_2O5_5 coupled ladders in Sr14−x_{14-x}Cax_xCu24_{24}O41_{41} we derive the low energy Hamiltonian for this system. It occurs that the widely used ladder t-J model is not sufficient and has to be supplemented by the Coulomb repulsion term between holes in the neighboring ladders. Furthermore, we show how a simple mean-field solution of the derived t-J model may explain the onset of the charge density wave with the odd period in Sr14−x_{14-x}Cax_xCu24_{24}O41_{41}.Comment: 8 pages, 4 figures, 2 table

    Quantum walk versus classical wave: Distinguishing ground states of quantum magnets by spacetime dynamics

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    We investigate wave packet spreading after a single spin flip in prototypical two-dimensional ferromagnetic and antiferromagnetic quantum spin systems. We find characteristic spatial magnon density profiles: While the ferromagnet shows a square-shaped pattern reflecting the underlying lattice structure, as exhibited by quantum walkers, the antiferromagnet shows a circular-shaped pattern which hides the lattice structure and instead resembles a classical wave pattern. We trace these fundamentally different behaviors back to the distinctly different magnon energy-momentum dispersion relations and also provide a real-space interpretation. Our findings point to opportunities for real-time, real-space imaging of quantum magnets both in materials science and in quantum simulators

    Dispersion of orbital excitations in 2D quantum antiferromagnets

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    We map the problem of the orbital excitation (orbiton) in a 2D antiferromagnetic and ferroorbital ground state onto a problem of a hole in 2D antiferromagnet. The orbiton turns out to be coupled to magnons and can only be mobile on a strongly renormalized scale by dressing with magnetic excitations. We show that this leads to a dispersion relation reflecting the two-site unit cell of the antiferromagnetic background, in contrast to the predictions based on a mean-field approximation and linear orbital-wave theory.Comment: 4 pages, 2 figures, submitted to SCES 2011 conference proceeding

    Possibility to realize spin-orbit-induced correlated physics in iridium fluorides

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    Recent theoretical predictions of "unprecedented proximity" of the electronic ground state of iridium fluorides to the SU(2) symmetric jeff=1/2j_{\mathrm{eff}}=1/2 limit, relevant for superconductivity in iridates, motivated us to investigate their crystal and electronic structure. To this aim, we performed high-resolution x-ray powder diffraction, Ir L3_3-edge resonant inelastic x-ray scattering, and quantum chemical calculations on Rb2_2[IrF6_6] and other iridium fluorides. Our results are consistent with the Mott insulating scenario predicted by Birol and Haule [Phys. Rev. Lett. 114, 096403 (2015)], but we observe a sizable deviation of the jeff=1/2j_{\mathrm{eff}}=1/2 state from the SU(2) symmetric limit. Interactions beyond the first coordination shell of iridium are negligible, hence the iridium fluorides do not show any magnetic ordering down to at least 20 K. A larger spin-orbit coupling in iridium fluorides compared to oxides is ascribed to a reduction of the degree of covalency, with consequences on the possibility to realize spin-orbit-induced strongly correlated physics in iridium fluorides

    Absence of Hole Confinement in Transition Metal Oxides with Orbital Degeneracy

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    We investigate the spectral properties of a hole moving in a two-dimensional Hubbard model for strongly correlated t_2g electrons. Although superexchange interactions are Ising-like, a quasi-one-dimensional coherent hole motion arises due to effective three-site terms. This mechanism is fundamentally different from the hole motion via quantum fluctuations in the conventional spin model with SU(2) symmetry. The orbital model describes also propagation of a hole in some e_g compounds, and we argue that orbital degeneracy alone does not lead to hole self-localization.Comment: 4 pages, 5 figure

    Directly characterizing the relative strength and momentum dependence of electron-phonon coupling using resonant inelastic x-ray scattering

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    The coupling between lattice and charge degrees of freedom in condensed matter materials is ubiquitous and can often result in interesting properties and ordered phases, including conventional superconductivity, charge density wave order, and metal-insulator transitions. Angle-resolved photoemission spectroscopy and both neutron and non-resonant x-ray scattering serve as effective probes for determining the behavior of appropriate, individual degrees of freedom -- the electronic structure and lattice excitation, or phonon dispersion, respectively. However, each provides less direct information about the mutual coupling between the degrees of freedom, usual through self-energy effects, which tend to renormalize and broaden spectral features precisely where the coupling is strong, impacting ones ability to quantitively characterize the coupling. Here we demonstrate that resonant inelastic x-ray scattering, or RIXS, can be an effective tool to directly determine the relative strength and momentum dependence of the electron-phonon coupling in condensed matter systems. Using a diagrammatic approach for an 8-band model of copper oxides, we study the contributions from the lowest order diagrams to the full RIXS intensity for a realistic scattering geometry, accounting for matrix element effects in the scattering cross-section as well as the momentum dependence of the electron-phonon coupling vertex. A detailed examination of these maps offers a unique perspective into the characteristics of electron-phonon coupling, which complements both neutron and non-resonant x-ray scattering, as well as Raman and infrared conductivity.Comment: 10 pages, 10 figure

    Micro integration of optical components for the fabrication of active optical cables

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    Optical interconnects have become very interesting for short reach data transfer. We examine a new concept for integration and miniaturization of such systems based on recent experiments. The application of these designs is an active optical cable. The advantages of the concept and the employed technologies are presented
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