684 research outputs found
Astrocytes in the entorhinal cortex show early atrophy in a triple transgenic animal model of Alzheimer's disease
Structure formation in binary colloids
A theoretical study of the structure formation observed very recently [Phys.
Rev. Lett. 90, 128303 (2003)] in binary colloids is presented. In our model
solely the dipole-dipole interaction of the particles is considered,
electrohidrodynamic effects are excluded. Based on molecular dynamics
simulations and analytic calculations we show that the total concentration of
the particles, the relative concentration and the relative dipole moment of the
components determine the structure of the colloid. At low concentrations the
kinetic aggregation of particles results in fractal structures which show a
crossover behavior when increasing the concentration. At high concentration
various lattice structures are obtained in a good agreement with experiments.Comment: revtex, 4 pages, figures available from authors due to size problem
High-resolution Ce 3d-edge resonant photoemission study of CeNi_2
Resonant photoemission (RPES) at the Ce 3d -> 4f threshold has been performed
for alpha-like compound CeNi_2 with extremely high energy resolution (full
width at half maximum < 0.2 eV) to obtain bulk-sensitive 4f spectral weight.
The on-resonance spectrum shows a sharp resolution-limited peak near the Fermi
energy which can be assigned to the tail of the Kondo resonance. However, the
spin-orbit side band around 0.3 eV binding energy corresponding to the f_{7/2}
peak is washed out, in contrast to the RPES spectrum at the Ce 3d -> 4f RPES
threshold. This is interpreted as due to the different surface sensitivity, and
the bulk-sensitive Ce 3d -> 4f RPES spectra are found to be consistent with
other electron spectroscopy and low energy properties for alpha-like
Ce-transition metal compounds, thus resolves controversy on the interpretation
of Ce compound photoemission. The 4f spectral weight over the whole valence
band can also be fitted fairly well with the Gunnarsson-Schoenhammer
calculation of the single impurity Anderson model, although the detailed
features show some dependence on the hybridization band shape and (possibly) Ce
5d emissions.Comment: 4 pages, 3 figur
The transition from the adiabatic to the sudden limit in core level photoemission: A model study of a localized system
We consider core electron photoemission in a localized system, where there is
a charge transfer excitation. The system is modelled by three electron levels,
one core level and two outer levels. The model has a Coulomb interaction
between these levels and the continuum states into which the core electron is
emitted. The model is simple enough to allow an exact numerical solution, and
with a separable potential an analytic solution. We calculate the ratio
r(omega) between the weights of the satellite and the main peak as a function
of the photon energy omega. The transition from the adiabatic to the sudden
limit takes place for quite small photoelectron kinetic energies. For such
small energies, the variation of the dipole matrix element is substantial and
described by the energy scale Ed. Without the coupling to the photoelectron,
the corresponding ratio r0(omega) is determined by Ed and the satellite
excitation energy dE. When the interaction potential with the continuum states
is introduced, a new energy scale Es=1/(2Rs^2) enters, where Rs is a length
scale of the interaction potential. At threshold there is typically a (weak)
constructive interference between intrinsic and extrinsic contributions, and
the ratio r(omega)/r0(omega) is larger than its limiting value for large omega.
The interference becomes small or weakly destructive for photoelectron energies
of the order Es. For larger energies r(omega)/r0(omega) therefore typically has
a weak undershoot. If this undershoot is neglected, r(omega)/r0(omega) reaches
its limiting value on the energy scale Es.Comment: 18 pages, latex2e, 13 eps figure
Electronic structure of NiS_{1-x}Se_x
We investigate the electronic structure of the metallic NiSSe
system using various electron spectroscopic techniques. The band structure
results do not describe the details of the spectral features in the
experimental spectrum, even for this paramagnetic metallic phase. However, a
parameterized many-body multi-band model is found to be successful in
describing the Ni~2 core level and valence band, within the same model. The
asymmetric line shape as well as the weak intensity feature in the Ni~2 core
level spectrum has been ascribed to extrinsic loss processes in the system. The
presence of satellite features in the valence band spectrum shows the existence
of the lower Hubbard band, deep inside the metallic regime, consistent
with the predictions of the dynamical mean field theory.Comment: To be published in Physical Review B, 18 pages and 5 figure
Angle-resolved photoemission study of USb2: the 5f band structure
Single crystal antiferromagnetic USb2 was studied at 15K by angle-resolved
photoemission with an overall energy resolution of 24 meV. The measurements
unambiguously show the dispersion of extremely narrow bands situated near the
Fermi level. The peak at the Fermi level represents the narrowest feature
observed in 5f-electron photoemission to date. The natural linewidth of the
feature just below the Fermi level is not greater than 10 meV. Normal emission
data indicate a three dimensional aspect to the electronic structure of this
layered material.Comment: 22 pages including figure
Temperature-Dependent Pseudogaps in Colossal Magnetoresistive Oxides
Direct electronic structure measurements of a variety of the colossal
magnetoresistive oxides show the presence of a pseudogap at the Fermi energy
E_F which drastically suppresses the electron spectral function at E_F. The
pseudogap is a strong function of the layer number of the samples (sample
dimensionality) and is strongly temperature dependent, with the changes
beginning at the ferromagnetic transition temperature T_c. These trends are
consistent with the major transport trends of the CMR oxides, implying a direct
relationship between the pseudogap and transport, including the "colossal"
conductivity changes which occur across T_c. The k-dependence of the
temperature-dependent effects indicate that the pseudogap observed in these
compounds is not due to the extrinsic effects proposed by Joynt.Comment: 5 pages, 6 figures, submitted to Phys. Rev.
Bulk-sensitive photoemission spectroscopy of A_2FeMoO_6 double perovskites (A=Sr, Ba)
Electronic structures of Sr_2FeMoO_6 (SFMO) and Ba_2FeMoO_6 (BFMO) double
perovskites have been investigated using the Fe 2p->3d resonant photoemission
spectroscopy (PES) and the Cooper minimum in the Mo 4d photoionization cross
section. The states close to the Fermi level are found to have strongly mixed
Mo-Fe t_{2g} character, suggesting that the Fe valence is far from pure 3+. The
Fe 2p_{3/2} XAS spectra indicate the mixed-valent Fe^{3+}-Fe^{2+}
configurations, and the larger Fe^{2+} component for BFMO than for SFMO,
suggesting a kind of double exchange interaction. The valence-band PES spectra
reveal good agreement with the LSDA+U calculation.Comment: 4 pages, 3 figure
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