104 research outputs found
Fingerprinting the magnetic behavior of antiferromagnetic nanostructures using remanent magnetization curves
Antiferromagnetic (AF) nanostructures from Co3O4, CoO and Cr2O3 were prepared
by the nanocasting method and were characterized magnetometrically. The field
and temperature dependent magnetization data suggests that the nanostructures
consist of a core-shell structure. The core behaves as a regular
antiferromagnet and the shell as a two-dimensional diluted antiferromagnet in a
field (2d DAFF) as previously shown on Co3O4 nanowires [Benitez et al., Phys.
Rev. Lett. 101, 097206 (2008)]. Here we present a more general picture on three
different material systems, i.e. Co3O4, CoO and Cr2O3. In particular we
consider the thermoremanent (TRM) and the isothermoremanent (IRM) magnetization
curves as "fingerprints" in order to identify the irreversible magnetization
contribution originating from the shells. The TRM/IRM fingerprints are compared
to those of superparamagnetic systems, superspin glasses and 3d DAFFs. We
demonstrate that TRM/IRM vs. H plots are generally useful fingerprints to
identify irreversible magnetization contributions encountered in particular in
nanomagnets.Comment: submitted to PR
The interparticle interaction and crossover in critical lines on field-temperature plane in PrSrMnO nanoparticles
The magnetic properties and the effects of interparticle interaction on it
have been studied in nanoparticles of half doped PrSrMnO.
Three samples consisting of nanoparticles of different average particle sizes
are synthesized to render the variation in interparticle interaction. Though
all the samples crystallize in the same structure to that of their bulk
compound, the low temperature ferromagnetic-antiferromagnetic transition, which
is present in bulk compound, is not evident in the nanoparticles. Linear as
well as nonlinear ac susceptibility coupled with dc magnetic measurements have
shown the superparamagnetic behavior of these nanoparticles where the blocking
temperature increases with the increasing particle size. Presence of
interparticle interaction is confirmed from the temperature variation of
coercive field and the analysis of frequency dependent ac susceptibility. We
have identified the nature of this interaction to be of dipolar type, and show
that its strength decreases with the increasing particle size. The effect of
this dipolar interaction on magnetic properties is intriguing as the compounds
exhibit crossover from de Almeida-Thouless to Gabay-Toulouse like critical
lines on field-temperature plane above their respective interaction field. In
agreement with theoretical prediction, we infer that this crossover is induced
by the unidirectional anisotropy arising from interparticle interaction, and
this is confirmed from the presence of exchange bias phenomenon.Comment: To appear in Phys. Rev.
A Novel Dielectric Anomaly in Cuprates and Nickelates: Signature of an Electronic Glassy State
The low-frequency dielectric response of hole-doped insulators
La_{2}Cu_{1-x}Li_{x}O_{4} and La_{2-x}Sr_{x}NiO_{4} shows a large dielectric
constant \epsilon ^{'} at high temperature and a step-like drop by a factor of
100 at a material-dependent low temperature T_{f}. T_{f} increases with
frequency and the dielectric response shows universal scaling in a Cole-Cole
plot, suggesting that a charge glass state is realized both in the cuprates and
in the nickelates.Comment: 5 pages, 4 figure
Ordering in a spin glass under applied magnetic field
Torque, torque relaxation, and magnetization measurements on a AuFe spin
glass sample are reported. The experiments carried out up to 7 T show a
transverse irreversibility line in the (H,T) plane up to high applied fields,
and a distinct strong longitudinal irreversibility line at lower fields. The
data demonstrate for that this type of sample, a Heisenberg spin glass with
moderately strong anisotropy, the spin glass ordered state survives under high
applied fields in contrast to predictions of certain "droplet" type scaling
models. The overall phase diagram closely ressembles those of mean field or
chiral models, which both have replica symmetry breaking transitions.Comment: 4 pages, 3 figures, accepted for PR
Spinless impurities in high Tc cuprates: Kondo-like behavior
We compare the effects of in-plane non magnetic Li and Zn
impurities on the normal state of high-T cuprates. Y NMR shows that the
extra hole introduced by Li is not localized in its vicinity. The Tc depression
and induced moments on near neighbour Cu sites of Zn or Li are found identical.
These universal effects of spinless impurities establish the major influence of
the spin perturbation with respect to the charge defect. The susceptibility of
the induced moment measured by Li NMR displays a 1/(T+Theta) behavior. Theta
increases with doping up to about 200 K in the overdoped regime. We attribute
this to a "Kondo like" effect.Comment: To appear in Phys.Rev.Lett. (22 nov. 99) Minor modifications compared
to previous version. 8 pages (4 pages for text + 4 figures
Aging in a topological spin glass
We have examined the nonconventional spin glass phase of the 2-dimensional
kagome antiferromagnet (H_3 O) Fe_3 (SO_4)_2 (OH)_6 by means of ac and dc
magnetic measurements. The frequency dependence of the ac susceptibility peak
is characteristic of a critical slowing down at Tg ~ 18K. At fixed temperature
below Tg, aging effects are found which obey the same scaling law as in spin
glasses or polymers. However, in clear contrast with conventional spin glasses,
aging is remarkably insensitive to temperature changes. This particular type of
dynamics is discussed in relation with theoretical predictions for highly
frustrated non-disordered systems.Comment: 4 pages, 4 figure
Phase Separation and the Low-Field Bulk Magnetic Properties of Pr0.7Ca0.3MnO3
We present a detailed magnetic study of the perovskite manganite
Pr0.7Ca0.3MnO3 at low temperatures including magnetization and a.c.
susceptibility measurements. The data appear to exclude a conventional spin
glass phase at low fields, suggesting instead the presence of correlated
ferromagnetic clusters embedded in a charge-ordered matrix. We examine the
growth of the ferromagnetic clusters with increasing magnetic field as they
expand to occupy almost the entire sample at H ~ 0.5 T. Since this is well
below the field required to induce a metallic state, our results point to the
existence of a field-induced ferromagnetic insulating state in this material.Comment: 15 pages with figures, submitted to Physical Review
Mean-field theory of temperature cycling experiments in spin-glasses
We study analytically the effect of temperature cyclings in mean-field
spin-glasses. In accordance with real experiments, we obtain a strong
reinitialization of the dynamics on decreasing the temperature combined with
memory effects when the original high temperature is restored. The same
calculation applied to mean-field models of structural glasses shows no such
reinitialization, again in accordance with experiments. In this context, we
derive some relations between experimentally accessible quantities and propose
new experimental protocols. Finally, we briefly discuss the effect of field
cyclings during isothermal aging.Comment: Some misprints corrected, references updated, final version to apper
in PR
Real spin glasses relax slowly in the shade of hierarchical trees
The Parisi solution of the mean-field spin glass has been widely accepted and
celebrated. Its marginal stability in 3d and its complexity however raised the
question of its relevance to real spin glasses. This paper gives a short
overview of the important experimental results which could be understood within
the mean-field solution. The existence of a true phase transition and the
particular behaviour of the susceptibility below the freezing temperature,
predicted by the theory, are clearly confirmed by the experimental results. The
behaviour of the complex order parameter and of the Fluctuation Dissipation
ratio are in good agreement with results of spontaneous noise measurements. The
very particular ultrametric symmetry, the key feature of the theory, provided
us with a simple description of the rejuvenation and memory effects observed in
experiment. Finally, going a step beyond mean-field, the paper shortly
discusses new analyses in terms of correlated domains characterized by their
length scales, as well as new experiments on superspin glasses which compare
well with recent theoretical simulations.Comment: To appear in the proceedings of "Wandering with Curiosity in Complex
Landscapes", a scientific conference in honour of Giorgio Parisi for his 60th
birthday, Roma, September 8-10 2008 (submitted for the special issue of the
Journal of Statistical Physics, 2009
The pseudo‐brookite spin‐glass system studied by means of muon spin relaxation
Zero-field muon spin relaxation (µSR) experiments have been performed on the spin glass Fe1.75Ti1.25O5. Above the spin-glass temperature of 44 K a distinct exponential µSR rate (¿) is observed, while below Tg a square-root exponential decay occurs, indicating fast spin fluctuations. Near 8 K, a maximum in ¿ is indicative of transverse spin ordering. The low ¿ values and the sharp ¿ peak at Tg are very promising for the study of spin freezing models like the Vogel–Fulcher law or the power law
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