274 research outputs found
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Optically detected magnetic resonance studies on {pi}-conjugate polymers and novel carbon allotropes
This report describes the following: introduction to photoluminescence detected magnetic resonance (PLDMR); introduction to {pi}-conjugated systems; PLDMR measurements on poly(p-phenylene)-type ladder polymers; PLMDR measurements on poly(p-phenylene ethylene); and PLDMR measurements on C{sub 70}, polythiophene, poly(p-phenylene vinylene) and Dan-40. Appendices to this report describe: Operation of ODMR (optically detected magnetic resonance) spectrometer; ODMR system parameters; and Special purpose circuitry
Reversible and Irreversible Interactions of Poly(3-hexylthiophene) with Oxygen Studied by Spin-Sensitive Methods
Understanding of degradation mechanisms in polymer:fullerene
bulk-heterojunctions on the microscopic level aimed at improving their
intrinsic stability is crucial for the breakthrough of organic photovoltaics.
These materials are vulnerable to exposure to light and/or oxygen, hence they
involve electronic excitations. To unambiguously probe the excited states of
various multiplicities and their reactions with oxygen, we applied combined
magneto-optical methods based on multifrequency (9 and 275 GHz) electron
paramagnetic resonance (EPR), photoluminescence (PL), and PL-detected magnetic
resonance (PLDMR) to the conjugated polymer poly(3-hexylthiophene) (P3HT) and
polymer:fullerene bulk heterojunctions (P3HT:PCBM; PCBM =
[6,6]-phenyl-C61-butyric acid methyl ester). We identified two distinct
photochemical reaction routes, one being fully reversible and related to the
formation of polymer:oxygen charge transfer complexes, the other one,
irreversible, being related to the formation of singlet oxygen under
participation of bound triplet excitons on the polymer chain. With respect to
the blends, we discuss the protective effect of the methanofullerenes on the
conjugated polymer bypassing the triplet exciton generation
Abstract Interpretation of Indexed Grammars.
Indexed grammars are a generalization of context-free grammars and recognize a proper subset of context-sensitive languages. The class of languages recognized by indexed grammars are called indexed languages and they correspond to the languages recognized by nested stack automata. For example indexed grammars can recognize the language {a^n b^n c^n | n > = 1} which is not context-free, but they cannot recognize {(ab^n)^n) | n >= 1} which is context-sensitive. Indexed grammars identify a set of languages that are more expressive than context-free languages, while having decidability results that lie in between the ones of context-free and context-sensitive languages. In this work we study indexed grammars in order to formalize the relation between indexed languages and the other classes of languages in the Chomsky hierarchy. To this end, we provide a fixpoint characterization of the languages recognized by an indexed grammar and we study possible ways to abstract, in the abstract interpretation sense, these languages and their grammars into context-free and regular languages
“This is proof”? Forensic evidence and ambiguous material culture at Treblinka extermination camp
In recent years, a forensic archaeological project at Treblinka extermination camp has uncovered significance evidence relating to the mass murder that took place there. A number of questions emerged regarding the provenance and origins of objects discovered as part of this work, and why they had remained undiscovered for over seventy years. These discoveries led to an opportunity to confirm and challenge the history of the extermination camp, and demands (from the public) to view the objects. This paper will outline how archaeologists and artists came together to reflect on these issues, whilst simultaneously providing access to the new findings
The construction of viewpoint aspect: the imperfective revisited
This paper argues for a constructionist approach to viewpoint Aspect by exploring the idea that it does not exert any altering force on the situation-aspect properties of predicates. The proposal is developed by analyzing the syntax and semantics of the imperfective, which has been attributed a coercer role in the literature as a de-telicizer and de-stativizer in the progressive, and as a de-eventivizer in the so-called ability (or attitudinal) and habitual readings. This paper proposes a unified semantics for the imperfective, preserving the properties of eventualities throughout the derivation. The paper argues that the semantics of viewpoint aspect is encoded in a series of functional heads containing interval-ordering predicates and quantifiers. This richer structure allows us to account for a greater amount of phenomena, such as the perfective nature of the individual instantiations of the event within a habitual construction or the nonculminating reading of perfective accomplishments in Spanish. This paper hypothesizes that nonculminating accomplishments have an underlying structure corresponding to the perfective progressive. As a consequence, the progressive becomes disentangled from imperfectivity and is given a novel analysis. The proposed syntax is argued to have a corresponding explicit morphology in languages such as Spanish and a nondifferentiating one in languages such as English; however, the syntax-semantics underlying both of these languages is argued to be the same
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