Optical spectroscopy of single quantum dots at tunable positive, neutral and negative charge states

We report on the observation of photoluminescence from positive, neutral and negative charge states of single semiconductor quantum dots. For this purpose we designed a structure enabling optical injection of a controlled unequal number of negative electrons and positive holes into an isolated InGaAs quantum dot embedded in a GaAs matrix. Thereby, we optically produced the charge states -3, -2, -1, 0, +1 and +2. The injected carriers form confined collective 'artificial atoms and molecules' states in the quantum dot. We resolve spectrally and temporally the photoluminescence from an optically excited quantum dot and use it to identify collective states, which contain charge of one type, coupled to few charges of the other type. These states can be viewed as the artificial analog of charged atoms such as H$^{-}$, H$^{-2}$, H$^{-3}$, and charged molecules such as H$_{2}^{+}$ and H$_{3}^{+2}$. Unlike higher dimensionality systems, where negative or positive charging always results in reduction of the emission energy due to electron-hole pair recombination, in our dots, negative charging reduces the emission energy, relative to the charge-neutral case, while positive charging increases it. Pseudopotential model calculations reveal that the enhanced spatial localization of the hole-wavefunction, relative to that of the electron in these dots, is the reason for this effect.Comment: 5 figure

Spontaneously Localized Photonic Modes Due to Disorder in the Dielectric Constant

We present the first experimental evidence for the existence of strongly localized photonic modes due to random two dimensional fluctuations in the dielectric constant. In one direction, the modes are trapped by ordered Bragg reflecting mirrors of a planar, one wavelength long, microcavity. In the cavity plane, they are localized by disorder, which is due to randomness in the position, composition and sizes of quantum dots located in the anti-node of the cavity. We extend the theory of disorder induced strong localization of electron states to optical modes and obtain quantitative agreement with the main experimental observations.Comment: 6 page

Radiative cascade from quantum dot metastable spin-blockaded biexciton

We detect a novel radiative cascade from a neutral semiconductor quantum dot. The cascade initiates from a metastable biexciton state in which the holes form a spin-triplet configuration, Pauli-blockaded from relaxation to the spin-singlet ground state. The triplet biexciton has two photon-phonon-photon decay paths. Unlike in the singlet-ground state biexciton radiative cascade, in which the two photons are co-linearly polarized, in the triplet biexciton cascade they are crosslinearly polarized. We measured the two-photon polarization density matrix and show that the phonon emitted when the intermediate exciton relaxes from excited to ground state, preserves the exciton's spin. The phonon, thus, does not carry with it any which-path information other than its energy. Nevertheless, entanglement distillation by spectral filtering was found to be rather ineffective for this cascade. This deficiency results from the opposite sign of the anisotropic electron-hole exchange interaction in the excited exciton relative to that in the ground exciton.Comment: 6 pages, 4 figure

Multi-Exciton Spectroscopy of a Single Self Assembled Quantum Dot

We apply low temperature confocal optical microscopy to spatially resolve, and spectroscopically study a single self assembled quantum dot. By comparing the emission spectra obtained at various excitation levels to a theoretical many body model, we show that: Single exciton radiative recombination is very weak. Sharp spectral lines are due to optical transitions between confined multiexcitonic states among which excitons thermalize within their lifetime. Once these few states are fully occupied, broad bands appear due to transitions between states which contain continuum electrons.Comment: 12 pages, 4 figures, submitted for publication on Jan,28 199

Polarization sensitive spectroscopy of charged Quantum Dots

We present an experimental and theoretical study of the polarized photoluminescence spectrum of single semiconductor quantum dots in various charge states. We compare our high resolution polarization sensitive spectral measurements with a new many-carrier theoretical model, which was developed for this purpose. The model considers both the isotropic and anisotropic exchange interactions between all participating electron-hole pairs. With this addition, we calculate both the energies and polarizations of all optical transitions between collective, quantum dot confined charge carrier states. We succeed in identifying most of the measured spectral lines. In particular, the lines resulting from singly-, doubly- and triply- negatively charged excitons and biexcitons. We demonstrate that lines emanating from evenly charged states are linearly polarized. Their polarization direction does not necessarily coincide with the traditional crystallographic direction. It depends on the shells of the single carriers, which participate in the recombination process.Comment: 11 pages, 9 figures. Revised versio

Quasiparticle properties of a coupled quantum wire electron-phonon system

We study leading-order many-body effects of longitudinal optical (LO) phonons on electronic properties of one-dimensional quantum wire systems. We calculate the quasiparticle properties of a weakly polar one dimensional electron gas in the presence of both electron-phonon and electron-electron interactions. The leading-order dynamical screening approximation (GW approximation) is used to obtain the electron self-energy, the quasiparticle spectral function, and the quasiparticle damping rate in our calculation by treating electrons and phonons on an equal footing. Our theory includes effects (within the random phase approximation) of Fermi statistics, Landau damping, plasmon-phonon mode coupling, phonon renormalization, dynamical screening, and impurity scattering. In general, electron-electron and electron-phonon many-body renormalization effects are found to be nonmultiplicative and nonadditive in our theoretical results for quasiparticle properties.Comment: 21 pages, Revtex, 12 figures enclose