21 research outputs found

    Onset of the nonlinear dielectric response of glasses in the two-level system model

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    We have calculated the real part χ\chi' of the nonlinear dielectric susceptibility of amorphous insulators in the kHz range, by using the two-level system model and a nonperturbative numerical quantum approach. At low temperature TT, it is first shown that the standard two-level model should lead to a \textit{decrease} of χ\chi' when the measuring field EE is raised, since raising EE increases the population of the upper level and induces Rabi oscillations canceling the ones induced from the ground level. This predicted EE-induced decrease of χ\chi' is at \textit{odds} with experiments. However, a \textit{good agreement} with low-frequency experimental nonlinear data is achieved if, in our fully quantum simulations, interactions between defects are taken into account by a new relaxation rate whose efficiency increases as E\sqrt{E}, as was proposed recently by Burin \textit{et al.} (Phys. Rev. Lett. {\bf 86}, 5616 (2001)). In this approach, the behavior of χ\chi' at low TT is mainly explained by the efficiency of this new relaxation channel. This new relaxation rate could be further tested since it is shown that it should lead: \textit{i)} to a completely new nonlinear behavior for samples whose thickness is 10\simeq 10 nm; \textit{ii)} to a decrease of nonequilibrium effects when EE is increased.Comment: latex Sept02.tex, 5 files, 4 figures, 17 pages, submitted to Eur. Phys. J. B. Text change

    Dielectric constant of glasses: first observation of a two-dimensional behavior

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    The 1kHz real part χ\chi' of the dielectric constant of a structural glass was measured at low temperature TT down to 14 mK. Reducing the sample thickness hh to 10 nm suppresses the usual minimum of χ\chi' for measuring fields E<.5E<.5 MV/m. This contradicts the Two Level System (TLS) model but is well accounted for by including TLS-TLS interactions where excitations delocalize between TLS's through a EE-induced mechanism recently designed: for small hh's this interaction is reduced, which explains the two-dimensional behavior of χ(T)\chi'(T). Hence, interactions play a key role in standard thick samples.Comment: latex finesse3.tex, 5 files, 4 figures, 4 pages [SPEC-S02/050], submitted to Phys. Rev. Let

    Pairing interactions and pairing mechanism in high temperature copper oxide superconductors

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    The polaron binding energy E_{p} in undoped parent cuprates has been determined to be about 1.0 eV from the unconventional oxygen-isotope effect on the antiferromagnetic ordering temperature. The deduced value of E_{p} is in quantitative agreement with that estimated from independent optical data and that estimated theoretically from the measured dielectric constants. The substantial oxygen-isotope effect on the in-plane supercarrier mass observed in optimally doped cuprates suggests that polarons are bound into the Cooper pairs. We also identify the phonon modes that are strongly coupled to conduction electrons from the angle-resolved photoemission spectroscopy, tunneling spectra, and optical data. We consistently show that there is a very strong electron-phonon coupling feature at a phonon energy of about 20 meV along the antinodal direction and that this coupling becomes weaker towards the diagonal direction. We further show that high-temperature superconductivity in cuprates is caused by strong electron-phonon coupling, polaronic effect, and significant coupling with 2 eV Cu-O charge transfer fluctuation.Comment: 11 pages, 7 figure

    Electrodynamic response of MgB2 sintered pellets and thin films

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    We present a study of the electrodynamic response of MgB2 pellets and thin film samples exhibiting critical temperatures ranging between 26 and 38 K. We have performed accurate measurements of the surface impedance ZS =RS+iXS as a function of the temperature and of the magnitude of the electromagnetic field. The temperature variation and the field dependence of ZS was measured by a dielectric resonator cavity technique in the microwave region. In particular, the temperature variation of the magnetic penetration depth was also determined in the RF region by a single coil mutual inductance method. In the case of the films, for T<TC/2 a clear exponential behavior of the penetration depth is observed, which can be explained by a simple BCS s-wave model with a reduced value of the energy gap. On the contrary, pellets show no evidence of saturation, and the experimental results strictly follow a quadratic dependence down to the lowest temperatures. This behavior can be induced by the presence of metallic Mg inclusions that may locally depress the gap. The analysis of the field dependence of the surface impedance in the microwave region confirms that the electrodynamic response of MgB2 is dominated by different sources of dissipation, depending on the sample history, likely to be ascribed to the predominance of grain boundaries or normal regions on its surface.Comment: To appear as a chapter in "Studies of High Temperature Superconductors", Vol. 41, A.V. Narlikar ed., Nova Sci. Publ., New York. (submitted October 5, 2001). 21 pages, 16 figure

    Magnetic field effect on the dielectric constant of glasses: Evidence of disorder within tunneling barriers

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    The magnetic field dependence of the low frequency dielectric constant ere_r(H) of a structural glass a - SiO2 + xCyHz was studied from 400 mK to 50 mK and for H up to 3T. Measurement of both the real and the imaginary parts of ere_r is used to eliminate the difficult question of keeping constant the temperature of the sample while increasing H: a non-zero ere_r(H) dependence is reported in the same range as that one very recently reported on multicomponent glasses. In addition to the recently proposed explanation based on interactions, the reported ere_r(H) is interpreted quantitatively as a consequence of the disorder lying within the nanometric barriers of the elementary tunneling systems of the glass.Comment: latex Bcorrige1.tex, 5 files, 4 figures, 7 pages [SPEC-S02/009

    Granularity-induced gapless superconductivity in NbN films: evidence of thermal phase fluctuations

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    Using a single coil mutual inductance technique, we measure the low temperature dependence of the magnetic penetration depth in superconducting NbN films prepared with similar critical temperatures around 16 K but with different microstructures. Only (100) epitaxial and weakly granular (100) textured films display the characteristic exponential dependence of conventional BCS s-wave superconductors. More granular (111) textured films exhibit a linear dependence, indicating a gapless state in spite of the s-wave gap. This result is quantitatively explained by a model of thermal phase fluctuations favored by the granular structure.Comment: 10 pages, 4 figures, to appear in Phys. Rev.

    Effect of Nuclear Quadrupole Interaction on the Relaxation in Amorphous Solids

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    Recently it has been experimentally demonstrated that certain glasses display an unexpected magnetic field dependence of the dielectric constant. In particular, the echo technique experiments have shown that the echo amplitude depends on the magnetic field. The analysis of these experiments results in the conclusion that the effect seems to be related to the nuclear degrees of freedom of tunneling systems. The interactions of a nuclear quadrupole electrical moment with the crystal field and of a nuclear magnetic moment with magnetic field transform the two-level tunneling systems inherent in amorphous dielectrics into many-level tunneling systems. The fact that these features show up at temperatures T<100mKT<100mK, where the properties of amorphous materials are governed by the long-range R3R^{-3} interaction between tunneling systems, suggests that this interaction is responsible for the magnetic field dependent relaxation. We have developed a theory of many-body relaxation in an ensemble of interacting many-level tunneling systems and show that the relaxation rate is controlled by the magnetic field. The results obtained correlate with the available experimental data. Our approach strongly supports the idea that the nuclear quadrupole interaction is just the key for understanding the unusual behavior of glasses in a magnetic field.Comment: 18 pages, 9 figure

    Penetration of Josephson vortices and measurement of the c-axis penetration depth in Bi2Sr2CaCu2O8+δBi_{2}Sr_{2}CaCu_{2}O_{8+\delta}: Interplay of Josephson coupling, surface barrier and defects

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    The first penetration field H_{J}(T) of Josephson vortices is measured through the onset of microwave absorption in the locked state, in slightly overdoped Bi2Sr2CaCu2O8+δ\rm{Bi_{2}Sr_{2}CaCu_{2}O_{8+\delta}} single crystals (T_{c} ~ 84 K). The magnitude of H_{J}(T) is too large to be accounted for by the first thermodynamic critical field H_{c1}(T). We discuss the possibility of a Bean-Livingston barrier, also supported by irreversible behavior upon flux exit, and the role of defects, which relates H_{J}(T) to the c-axis penetration depth λc(T)\lambda_{c}(T). The temperature dependence of the latter, determined by a cavity perturbation technique and a theoretical estimate of the defect-limited penetration field are used to deduce from H_{J}(T) the absolute value of λc(0)=(35±15)μm\lambda_{c}(0)=(35 \pm 15) \mu m.Comment: 9 pages, 6 figure
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