1,340 research outputs found
Low-Energy Scale Excitations in the Spectral Function of Organic Monolayer Systems
Using high-resolution photoemission spectroscopy we demonstrate that the
electronic structure of several organic monolayer systems, in particular
1,4,5,8-naphthalene tetracarboxylic dianhydride and Copper-phtalocyanine on
Ag(111), is characterized by a peculiar excitation feature right at the Fermi
level. This feature displays a strong temperature dependence and is immediatly
connected to the binding energy of the molecular states, determined by the
coupling between the molecule and the substrate. At low temperatures, the
line-width of this feature, appearing on top of the partly occupied lowest
unoccupied molecular orbital of the free molecule, amounts to only
meV, representing an unusually small energy scale for electronic excitations in
these systems. We discuss possible origins, related e.g. to many-body
excitations in the organic-metal adsorbate system, in particular a generalized
Kondo scenario based on the single impurity Anderson model.Comment: 6 pages, 3 figures, accepted as PRB Rapid Communication
Echo of the Quantum Phase Transition of CeCuAu in XPS: Breakdown of Kondo Screening
We present an X-ray photoemission study of the heavy-fermion system
CeCuAu across the magnetic quantum phase transition of this
compound at temperatures above the single-ion Kondo temperature . In
dependence of the Au concentration we observe a sudden change of the
-occupation number and the core-hole potential at the
critical concentration . We interpret these findings in the framework
of the single-impurity Anderson model. Our results are in excellent agreement
with findings from earlier UPS measurements %\cite{klein08qpt} and provide
further information about the precursors of quantum criticality at elevated
temperatures.Comment: 5 pages, 3 figures; published version, references updated, minor
changes in wordin
High-temperature signatures of quantum criticality in heavy fermion systems
We propose a new criterion for distinguishing the Hertz-Millis (HM) and the
local quantum critical (LQC) mechanism in heavy fermion systems with a magnetic
quantum phase transition (QPT). The criterion is based on our finding that the
spin screening of Kondo ions can be completely suppressed by the RKKY coupling
to the surrounding magnetic ions even without magnetic ordering and that,
consequently, the signature of this suppression can be observed in
spectroscopic measurements above the magnetic ordering temperature. We apply
the criterion to high-resolution photoemission (UPS) measurements on
CeCuAu and conclude that the QPT in this system is dominated by
the LQC scenario.Comment: Inveted paper, International Conference on Magnetism, ICM 2009,
Karlsruhe. Published version, added discussions of the relevance of
Fermi-surface fluctuations and of a structural transition near the QC
Temperature dependence of the Kondo resonance and its satellites in CeCu_2Si_2
We present high-resolution photoemission spectroscopy studies on the Kondo
resonance of the strongly-correlated Ce system CeCuSi. Exploiting the
thermal broadening of the Fermi edge we analyze position, spectral weight, and
temperature dependence of the low-energy 4f spectral features, whose major
weight lies above the Fermi level . We also present theoretical
predictions based on the single-impurity Anderson model using an extended
non-crossing approximation (NCA), including all spin-orbit and crystal field
splittings of the 4f states. The excellent agreement between theory and
experiment provides strong evidence that the spectral properties of
CeCuSi can be described by single-impurity Kondo physics down to K.Comment: 4 pages, 3 figure
Structure and transport in multi-orbital Kondo systems
We consider Kondo impurity systems with multiple local orbitals, such as rare
earth ions in a metallic host or multi--level quantum dots coupled to metallic
leads. It is shown that the multiplet structure of the local orbitals leads to
multiple Kondo peaks above the Fermi energy , and to ``shadow'' peaks
below . We use a slave boson mean field theory, which recovers the strong
coupling Fermi liquid fixed point, to calculate the Kondo peak positions,
widths, and heights analytically at T=0, and NCA calculations to fit the
temperature dependence of high--resolution photoemission spectra of Ce
compounds. In addition, an approximate conductance quantization for transport
through multi--level quantum dots or single--atom transistors in the Kondo
regime due to a generalized Friedel sum rule is demonstrated.Comment: 4 pages, 3 figures. Invited article, 23rd International Conference on
Low Temperature Physics LT23, Hiroshima, Japan 200
Evidence of momentum dependent hybridization in Ce2Co0.8Si3.2
We studied the electronic structure of the Kondo lattice system Ce2Co0.8Si3.2
by angle-resolved photoemission spectroscopy (ARPES). The spectra obtained
below the coherence temperature consist of a Kondo resonance, its spin-orbit
partner and a number of dispersing bands. The quasiparticle weight related to
the Kondo peak depends strongly on Fermi vectors associated with bulk bands.
This indicates a highly anisotropic hybridization between conduction band and
4f electrons - V_{cf} in Ce2Co0.8Si3.2.Comment: 6 page
Sampling bias in systems with structural heterogeneity and limited internal diffusion
Complex systems research is becomingly increasingly data-driven, particularly
in the social and biological domains. Many of the systems from which sample
data are collected feature structural heterogeneity at the mesoscopic scale
(i.e. communities) and limited inter-community diffusion. Here we show that the
interplay between these two features can yield a significant bias in the global
characteristics inferred from the data. We present a general framework to
quantify this bias, and derive an explicit corrective factor for a wide class
of systems. Applying our analysis to a recent high-profile survey of conflict
mortality in Iraq suggests a significant overestimate of deaths
High Resolution Photoemission Study on Low-T_K Ce Systems: Kondo Resonance, Crystal Field Structures, and their Temperature Dependence
We present a high-resolution photoemission study on the strongly correlated
Ce-compounds CeCu_6, CeCu_2Si_2, CeRu_2Si_2, CeNi_2Ge_2, and CeSi_2. Using a
normalization procedure based on a division by the Fermi-Dirac distribution we
get access to the spectral density of states up to an energy of 5 k_BT above
the Fermi energy E_F. Thus we can resolve the Kondo resonance and the crystal
field (CF) fine-structure for different temperatures above and around the Kondo
temperature T_K. The CF peaks are identified with multiple Kondo resonances
within the multiorbital Anderson impurity model. Our theoretical 4f spectra,
calculated from an extended non-crossing approximation (NCA), describe
consistently the observed photoemission features and their temperature
dependence. By fitting the NCA spectra to the experimental data and
extrapolating the former to low temperatures, T_K can be extracted
quantitatively. The resulting values for T_K and the crystal field energies are
in excellent agreement with the results from bulk sensitive measurements, e.g.
inelastic neutron scattering.Comment: 16 two-column pages, 10 figure
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