49 research outputs found

    Pressure Evolution of Magnetism in URhGa

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    In this paper, we report the results of an ambient and high pressure study of a 5f-electron ferromagnet URhGa. The work is focused on measurements of magnetic and thermodynamic properties of a single crystal sample and on the construction of the p-T phase diagram. Diamond anvil cells were employed to measure the magnetization and electrical resistivity pressures up to ~ 9 GPa. At ambient pressure, URhGa exhibits collinear ferromagnetic ordering of uranium magnetic moments {\mu}U ~ 1.1 {\mu}B (at 2 K) aligned along the c-axis of the hexagonal crystal structure below the Curie temperature TC = 41K. With the application of pressure up to 5GPa the ordering temperature TC initially increases whereas the saturated moment slightly decreases. The rather unexpected evolution is put in the context of the UTX family of compounds.Comment: arXiv admin note: text overlap with arXiv:1611.0327

    Pressure dependence of magneto-structural properties of Co-doped off-stoichiometric Ni2MnGa alloys

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    A strong effect of pressure on magnetization and paramagnetic moment of the Co-doped Mn-rich Ni 50-x Co x Mn 25+y Ga 25-y (x = 5,7,9 and y = 5,6,7,8) Heusler alloys is presented and compared with very weak pressure sensitivity of magnetization of the stoichiometric Ni 2 MnGa alloy. The effects of both, the pressure and the magnetic field, on temperature of the structural martensitic transition in the alloys are discussed with a use of the Clausius-Clapeyron relations. An analysis of pressure and field effects provides a possibility to evaluate structural and magnetic parts of latent heat of the martensitic transitions in the studied alloys. The Curie temperature of martensite phase of the Co-rich alloys is not affected by pressure

    Antiferromagnetic order in (Lu0.8Ce0.2)2Fe17 and Lu2Fe16.5Ru0.5: High pressure study

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    International audienceThe antiferromagnetic state observed in Lu2Fe17 at elevated temperatures is stabilized down to the ground state in (Lu0.8Ce0.2)2Fe17 and Lu2Fe16.5Ru0.5. The Néel temperature TN decreases from 274 K in Lu2Fe17 to 247 and 208 K in (Lu0.8Ce0.2)2Fe17 and Lu2Fe16.5Ru0.5, respectively. Both compounds exhibit the easy-plane type of magnetic anisotropy and a metamagnetic transition at fields below 1 T. External pressure pushes the transition toward a higher field and reduces the magnetization as well as TN to 234 and 185 K for (Lu0.8Ce0.2)2Fe17 and Lu2Fe16.5Ru0.5, respectively, under pressure 0.8 GPa. The pressure and the substitution effects can be understood in terms of exchange interaction varying strongly with changes in the lattice parameter c for (Lu0.8Ce0.2)2Fe17, while for Lu2Fe16.5Ru0.5, the change in magnetic structure occurs due to the weakening of the positive exchange interaction as a result of the reduction in the Fe magnetic moments at 12 k sites

    Magnetocaloric Effect in Materials with the First Order Transitions - Direct Measurements

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    The results of direct measurements of the magneto-caloric characteristics Δ TadT_{ad} and the indirect determination of Δ SmS_{m} of pure Gd around the Curie temperature and of the FeMnP0.45As0.55FeMnP_{0.45}As_{0.55} and Ni45Co5Mn31Ga19Ni_{45}Co_5Mn_{31}Ga_{19} intermetallics in the vicinity of the first order magnetic and structural phase transitions are presented and discussed. A pronounced temperature and field dependence of the first order transitions in the studied materials manifests restrictions applying these materials in magnetic refrigeration techniques. An effective use of the Ericsson and the Brayton refrigeration cycles with FeMnP0.45As0.55FeMnP_{0.45}As_{0.55} in the role of a refrigerant is discussed

    Spin disordered resistivity of the Heusler Ni₂MnGa-based alloys

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    Electrical resistivity of the selected Heusler off-stoichiometric (NiCo)₂Mn(GaIn) alloys was studied in a wide range of temperature and magnetic field. A step-like change of resistivity (Δρ ≈24 μΩcm) was detected in the off-stoichiometric Ni_{1.85}Mn_{1.21}Ga_{0.94} alloy at temperature of martensitic structural transition. This Δρ is much more significant than one in the stoichiometric Ni₂MnGa alloy. In the case of the off-stoichiometric (NiCo)₂Mn(GaIn) alloys, an enormous change of resistivity, Δρ ≈ 200 μΩcm, accompanies the structural transition. Simultaneously, the maximum of the spin disordered resistivity ρ_{sd}(T) of austenite phase of the alloys is slightly dependent on composition of the alloy and vary from ≈30 μΩcm up to ≈45 μΩcm, in good agreement with theoretical calculations. Due to high sensitivity of the structural transition temperature of the alloys to magnetic field, the very pronounced magnetoresistance effects have been observed in the studied alloys
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