391 research outputs found
Circular dichroism in photoelectron angular distributions from two‐color (1+1) REMPI of NO
A detailed experimental and theoretical study of dichroic effects in photoelectron angular distributions is reported for (1+1), two‐color REMPI of NO via the A^ 2Σ^+, v=0 state. Optically aligned A state rotational levels are probed through ionization by circularly polarized light. Resultant photoelectron angular distributions exhibit significant left–right asymmetry, the phase and magnitude of which are shown to be related to the curvature of the excited state M_J distribution. Theoretical calculations involving a full ab initio treatment of the ionization dynamics result in circularly dichroic angular distribution (CDAD) parameters in good agreement with those derived experimentally. Additional effects including hyperfine depolarization and coherence are also discussed in relation to the observed CDAD data
Electrical coupling of neuro-ommatidial photoreceptor cells in the blowfly
A new method of microstimulation of the blowfly eye using corneal neutralization was applied to the 6 peripheral photoreceptor cells (R1-R6) connected to one neuro-ommatidium (and thus looking into the same direction), whilst the receptor potential of a dark-adapted photoreceptor cell was recorded by means of an intracellular microelectrode. Stimulation of the photoreceptor cells not impaled elicited responses in the recorded cell of about 20% of the response elicited when stimulating the recorded cell. This is probably caused by gap junctions recently found between the axon terminals of these cells. Stimulation of all 6 cells together yielded responses that were larger and longer than those obtained with stimulation of just the recorded cell, and intensity-response curves that deviated more strongly from linearity. Evidence is presented that the resistance of the axon terminal of the photoreceptor cells quickly drops in response to a light flash, depending on the light intensity. Incorporating the cable properties of the cell body and the axon, the resistance of the gap junctions, and the (adapting) terminal resistance, a theoretical model is presented that explains the measurements well. Finally, it is argued that the gap junctions between the photoreceptor cells may effectively uncouple the synaptic responses of the cells by counteracting the influence of field potentials.
The Final Chapter In The Saga Of YIG
The magnetic insulator Yttrium Iron Garnet can be grown with exceptional
quality, has a ferrimagnetic transition temperature of nearly 600 K, and is
used in microwave and spintronic devices that can operate at room temperature.
The most accurate prior measurements of the magnon spectrum date back nearly 40
years, but cover only 3 of the lowest energy modes out of 20 distinct magnon
branches. Here we have used time-of-flight inelastic neutron scattering to
measure the full magnon spectrum throughout the Brillouin zone. We find that
the existing model of the excitation spectrum, well known from an earlier work
titled "The Saga of YIG", fails to describe the optical magnon modes. Using a
very general spin Hamiltonian, we show that the magnetic interactions are both
longer-ranged and more complex than was previously understood. The results
provide the basis for accurate microscopic models of the finite temperature
magnetic properties of Yttrium Iron Garnet, necessary for next-generation
electronic devices.Comment: 10 pages, 3 figures, 4 supplementary figures, 1 table, 1
supplementary tabl
A multiphoton ionization study of the photodissociation dynamics of the S_2 state of CH_3ONO
Two‐color (1+1) REMPI (resonantly enhanced multiphoton ionization) photoelectron spectroscopy is used to probe the NO photofragments produced by the UV photodissociation of methyl nitrite, i.e., CH_3ONO+hν→CH_3ONO∗(S_2)→CH_3O⋅(X)+NO(X, v, J). The photofragments are produced in their ground electronic states but with high rotational and translational energy. NO fragment angular distributions, rotational state distributions, and spatial alignment are determined by photoion and photoelectron detection. The initial state alignment is obtained by the CDAD (circularly dichroic angular distribution) technique for the first time. CDAD measurements for rotational levels with 35.5≤J≤46.5 result in alignment parameters at the classical high‐J limit of A^(2)_0 =−0.4. This alignment is consistent with an ‘‘impulsive’’ dissociation mechanism in which photofragment recoil along the CH_3O–NO bond imparts substantial rotational angular momentum to the NO molecule resulting in a high‐J state distribution and preferential rotation in the plane of dissociation. These measurements clearly establish the utility of the CDAD method for probing chemical processes in which spatial alignment plays an important role. Photoion angular distributions are used to probe correlations between the CH_3ONO transition dipole moment, NO fragment velocity, and angular momentum. These correlations reveal additional details of the photolysis mechanism
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Enhancement of Intracellular Calcium Ion Mobilization by Moderately but Not Highly Positive Material Surface Charges
Electrostatic forces at the cell interface affect the nature of cell adhesion and function; but there is still limited knowledge about the impact of positive or negative surface charges on cell-material interactions in regenerative medicine. Titanium surfaces with a variety of zeta potentials between −90 mV and +50 mV were generated by functionalizing them with amino polymers, extracellular matrix proteins/peptide motifs and polyelectrolyte multilayers. A significant enhancement of intracellular calcium mobilization was achieved on surfaces with a moderately positive (+1 to +10 mV) compared with a negative zeta potential (−90 to −3 mV). Dramatic losses of cell activity (membrane integrity, viability, proliferation, calcium mobilization) were observed on surfaces with a highly positive zeta potential (+50 mV). This systematic study indicates that cells do not prefer positive charges in general, merely moderately positive ones. The cell behavior of MG-63s could be correlated with the materials’ zeta potential; but not with water contact angle or surface free energy. Our findings present new insights and provide an essential knowledge for future applications in dental and orthopedic surgery. © Copyright © 2020 Gruening, Neuber, Nestler, Lehnfeld, Dubs, Fricke, Schnabelrauch, Helm, Müller, Staehlke and Nebe
Quantum and Semiclassical Calculations of Cold Atom Collisions in Light Fields
We derive and apply an optical Bloch equation (OBE) model for describing
collisions of ground and excited laser cooled alkali atoms in the presence of
near-resonant light. Typically these collisions lead to loss of atoms from
traps. We compare the results obtained with a quantum mechanical complex
potential treatment, semiclassical Landau-Zener models with decay, and a
quantum time-dependent Monte-Carlo wave packet (MCWP) calculation. We formulate
the OBE method in both adiabatic and diabatic representations. We calculate the
laser intensity dependence of collision probabilities and find that the
adiabatic OBE results agree quantitatively with those of the MCWP calculation,
and qualitatively with the semiclassical Landau-Zener model with delayed decay,
but that the complex potential method or the traditional Landau-Zener model
fail in the saturation limit.Comment: 21 pages, RevTex, 7 eps figures embedded using psfig, see also
http://www.physics.helsinki.fi/~kasuomin
Circular dichroism in photoelectron angular distributions from two‐color (1+1) REMPI of NO
Biomanufacturing and testbed development for the continuous production of monoclonal antibodies
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