1,110 research outputs found
Evolution of the dipole polarizability in the stable tin isotope chain
The dipole polarizability of stable even-mass tin isotopes
112,114,116,118,120,124 was extracted from inelastic proton scattering
experiments at 295 MeV under very forward angles performed at RCNP. Predictions
from energy density functionals cannot account for the present data and the
polarizability of 208Pb simultaneously. The evolution of the polarizabilities
in neighboring isotopes indicates a kink at 120Sn while all model results show
a nearly linear increase with mass number after inclusion of pairing
corrections.Comment: 10 pages, 6 figures, submitted to Phys. Lett.
Theory of Raman Scattering from Orbital Excitations in Manganese Oxides
We present a theory of the Raman scattering from the orbital wave excitations
in manganese oxides. Two excitation processes of the Raman scattering are
proposed. The Raman scattering cross section is formulated by using the
pseudospin operator for orbital degree of freedom in a Mn ion. The Raman
spectra from the orbital wave excitations are calculated and their implications
in the recent experimental results reported in LaMnO are discussed.Comment: 10 pages, 7 figure
Templated Synthesis of Peptide Nucleic Acids via Sequence-Selective Base-Filling Reactions
The templated synthesis of nucleic acids has previously been achieved through the backbone ligation of preformed nucleotide monomers or oligomers. In contrast, here we demonstrate templated nucleic acid synthesis using a base-filling approach in which individual bases are added to abasic sites of a peptide nucleic acid (PNA). Because nucleobase substrates in this approach are not self-reactive, a base-filling approach may reduce the formation of nontemplated reaction products. Using either reductive amination or amine acylation chemistries, we observed efficient and selective addition of each of the four nucleobases to an abasic site in the middle of the PNA strand. We also describe the addition of single nucleobases to the end of a PNA strand through base filling, as well as the tandem addition of two bases to the middle of the PNA strand. These findings represent an experimental foundation for nonenzymatic information transfer through base filling.Chemistry and Chemical Biolog
Spin Wave Instability of Itinerant Ferromagnet
We show variationally that instability of the ferromagnetic state in the
Hubbard model is largely controlled by softening of a long-wavelength spin-wave
excitation, except in the over-doped strong-coupling region where the
individual-particle excitation becomes unstable first. A similar conclusion is
drawn also for the double exchange ferromagnet. Generally the spin-wave
instability may be regarded as a precursor of the metal-insulator transition.Comment: 11 pages, 8 figure
Spatial Structure of Spin Polarons in the t-J Model
The deformation of the quantum Neel state induced by a spin polaron is
analyzed in a slave fermion approach. Our method is based on the selfconsistent
Born approximation for Green's and the wave function for the quasiparticle. The
results of various spin-correlation functions relative to the position of the
moving hole are discussed and shown to agree with those available from small
cluster calculations. Antiferromagnetic correlations in the direct neighborhood
of the hole are reduced, but they remain antiferromagnetic even for J as small
as 0.1 t. These correlation functions exhibit dipolar distortions in the spin
structure, which sensitively depend on the momentum of the quasiparticle. Their
asymptotic decay with the distance from the hole is governed by power laws, yet
the spectral weight of the quasiparticles does not vanish.Comment: 12 pages, 2 postscipt files with figures; uses REVTeX, to be
published in Phys. Rev. B, Feb. 199
Double Degeneracy and Jahn-Teller Effects in CMR Perovskites
Jahn-Teller (JT) electron-phonon coupling effects in the colossal
magnetoresistance perovskite compounds are investigated.
Electron-electron correlations between two degenerate Mn orbitals are
studied in the Gutzwiller approximation. The static JT distortion and
antiadiabatic polaron effects are studied in a modified Lang-Firsov
approximation. We find that (i) the electron or hole character of the charge
carrier depends on the static JT distortion, and (ii) due to the two-component
nature of the JT coupling, fluctuations in the JT distortion direction
contribute to the charge transport in similar fashion as the local spins.Comment: 11 RevTeX pages. 3 Figures available upon request. submitted to Phys.
rev. B (Rapid Communications
Cluster diagonalization in systematically expanded Hilbert spaces: application to models of correlated electrons
A method of cluster diagonalization in a systematically expanded Hilbert
space is described. We discuss some applications of this procedure to models of
high-T_c superconductors, like the t - J and one and three bands Hubbard models
in two dimensions. The results obtained with this method are compared against
results obtained with other techniques dealing with truncated Hilbert spaces.
The relation between this method of diagonalization in a reduced Hilbert space,
and perturbation theory and variational techniques is also discussed.Comment: 26 pages + 12 figures, available upon request, LATEX, preprint
ORNL/CCIP/93/
Grain boundary effects on magnetotransport in bi-epitaxial films of LaSrMnO
The low field magnetotransport of LaSrMnO (LSMO) films
grown on SrTiO substrates has been investigated. A high qualtity LSMO film
exhibits anisotropic magnetoresistance (AMR) and a peak in the
magnetoresistance close to the Curie temperature of LSMO. Bi-epitaxial films
prepared using a seed layer of MgO and a buffer layer of CeO display a
resistance dominated by grain boundaries. One film was prepared with seed and
buffer layers intact, while a second sample was prepared as a 2D square array
of grain boundaries. These films exhibit i) a low temperature tail in the low
field magnetoresistance; ii) a magnetoconductance with a constant high field
slope; and iii) a comparably large AMR effect. A model based on a two-step
tunneling process, including spin-flip tunneling, is discussed and shown to be
consistent with the experimental findings of the bi-epitaxial films.Comment: REVTeX style; 14 pages, 9 figures. Figure 1 included in jpeg format
(zdf1.jpg); the eps was huge. Accepted to Phys. Rev.
Vicinal Surface with Langmuir Adsorption: A Decorated Restricted Solid-on-solid Model
We study the vicinal surface of the restricted solid-on-solid model coupled
with the Langmuir adsorbates which we regard as two-dimensional lattice gas
without lateral interaction. The effect of the vapor pressure of the adsorbates
in the environmental phase is taken into consideration through the chemical
potential. We calculate the surface free energy , the adsorption coverage
, the step tension , and the step stiffness by
the transfer matrix method combined with the density-matrix algorithm. Detailed
step-density-dependence of and is obtained. We draw the roughening
transition curve in the plane of the temperature and the chemical potential of
adsorbates. We find the multi-reentrant roughening transition accompanying the
inverse roughening phenomena. We also find quasi-reentrant behavior in the step
tension.Comment: 7 pages, 12 figures (png format), RevTeX 3.1, submitted to Phys. Rev.
Immunotoxin-Mediated Tract Targeting in the Primate Brain: Selective Elimination of the Cortico-Subthalamic “Hyperdirect” Pathway
Using a neuron-specific retrograde gene-transfer vector (NeuRet vector), we established immunotoxin (IT)-mediated tract targeting in the primate brain that allows ablation of a neuronal population constituting a particular pathway. Here, we attempted selective removal of the cortico-subthalamic “hyperdirect” pathway. In conjunction with the direct and indirect pathways, the hyperdirect pathway plays a crucial role in motor information processing in the basal ganglia. This pathway links the motor-related areas of the frontal lobe directly to the subthalamic nucleus (STN) without relay at the striatum. After electrical stimulation in the motor-related areas such as the supplementary motor area (SMA), triphasic responses consisting of an early excitation, an inhibition, and a late excitation are usually detected in the internal segment of the globus pallidus (GPi). Several lines of pharmacophysiological evidence suggest that the early excitation may be derived from the hyperdirect pathway. In the present study, the NeuRet vector expressing human interleukin-2 receptor α-subunit was injected into the STN of macaque monkeys. Then, IT injections were made into the SMA. In these monkeys, single-neuron activity in the GPi was recorded in response to the SMA stimulation. We found that the early excitation was largely reduced, with neither the inhibition nor the late excitation affected. The spontaneous firing rate and pattern of GPi neurons remained unchanged. This indicates that IT-mediated tract targeting successfully eliminated the hyperdirect pathway selectively from the basal ganglia circuitry without affecting spontaneous activity of STN neurons. The electrophysiological finding was confirmed with anatomical data obtained from retrograde and anterograde neural tracings. The present results define that the cortically-driven early excitation in GPi neurons is mediated by the hyperdirect pathway. The IT-mediated tract targeting technique will provide us with novel strategies for elucidating various neural network functions
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