47 research outputs found
Charge ordering and chemical potential shift in LaSrNiO studied by photoemission spectroscopy
We have studied the chemical potential shift in LaSrNiO and
the charge ordering transition in LaSrNiO by
photoemission spectroscopy. The result shows a large ( 1 eV/hole)
downward shift of the chemical potential with hole doping in the high-doping
regime ( 0.33) while the shift is suppressed in the low-doping
regime ( 0.33). This suppression is attributed to a
segregation of doped holes on a microscopic scale when the hole concentration
is lower than . In the sample, the
photoemission intensity at the chemical potential vanishes below the charge
ordering transition temperature 240 K.Comment: 5 pages, 4 figure
Chemical Potential Shift in NdCeCuO: Contrasting Behaviors of the Electron- and Hole-Doped Cuprates
We have studied the chemical potential shift in the electron-doped
superconductor NdCeCuO by precise measurements of
core-level photoemission spectra. The result shows that the chemical potential
monotonously increases with electron doping, quite differently from
LaSrCuO, where the shift is suppressed in the underdoped
region.
If the suppression of the shift in LaSrCuO is attributed
to strong stripe fluctuations, the monotonous increase of the chemical
potential is consistent with the absence of stripe fluctuations in
NdCeCuO. The chemical potential jump between
NdCuO and LaCuO is found to be much smaller than the
optical band gaps.Comment: 4 pages, 5 figure
Charge Stripes and Antiferromagnetism in Insulating Nickelates and Superconducting Cuprates
Neutron and X-ray scattering studies have provided strong evidence for
coupled spatial modulations of charge and spin densities in layered nickelates
and cuprates. The accumulated results for La(2-x)Sr(x)NiO(4+d) are consistent
with the strongly-modulated topological-stripe concept. Clues from Nd-doped
La(2-x)Sr(x)CuO(4) suggest similar behavior for the cuprates. The experimental
results are summarized, and features that conflict with an interpretation based
on a Fermi-surface instability are emphasized. A rationalization for the
differences in transport properties between the cuprates and nickelates is
given.Comment: 10pp., uses elsart.sty, 3 eps figures embedded with psfig; for
proceedings of Spectroscopies in Novel Superconductors '97, J. Phys. Chem.
Solid
Distribution of spectral weight in a system with disordered stripes
The ``band-structure'' of a disordered stripe array is computed and compared,
at a qualitative level, to angle resolved photoemission experiments on the
cuprate high temperature superconductors. The low-energy states are found to be
strongly localized transverse to the stripe direction, so the electron dynamics
is strictly one-dimensional (along the stripe). Despite this, aspects of the
two dimensional band-structure Fermi surface are still vividly apparent.Comment: 10 pages, 11 figure
DDW Order and its Role in the Phase Diagram of Extended Hubbard Models
We show in a mean-field calculation that phase diagrams remarkably similar to
those recently proposed for the cuprates arise in simple microscopic models of
interacting electrons near half-filling. The models are extended Hubbard models
with nearest neighbor interaction and correlated hopping. The underdoped region
of the phase diagram features density-wave (DDW) order. In a
certain regime of temperature and doping, DDW order coexists with
antiferromagnetic (AF) order. For larger doping, it coexists with
superconductivity (DSC). While phase diagrams of this form
are robust, they are not inevitable. For other reasonable values of the
coupling constants, drastically different phase diagrams are obtained. We
comment on implications for the cuprates.Comment: 7 pages, 3 figure
Magnetotransport in the Normal State of La1.85Sr0.15Cu(1-y)Zn(y)O4 Films
We have studied the magnetotransport properties in the normal state for a
series of La1.85Sr0.15Cu(1-y)Zn(y)O4 films with values of y, between 0 and
0.12. A variable degree of compressive or tensile strain results from the
lattice mismatch between the substrate and the film, and affects the transport
properties differently from the influence of the zinc impurities. In
particular, the orbital magnetoresistance (OMR) varies with y but is
strain-independent. The relations for the resistivity and the Hall angle and
the proportionality between the OMR and tan^2 theta are followed about 70 K. We
have been able to separate the strain and impurity effects by rewriting the
above relations, where each term is strain-independent and depends on y only.
We also find that changes in the lattice constants give rise to closely the
same fractional changes in other terms of the equation.The OMR is more strongly
supressed by the addition of impurities than tan^2 theta. We conclude that the
relaxation ratethat governs Hall effect is not the same as for the
magnetoresistance. We also suggest a correspondence between the transport
properties and the opening of the pseudogap at a temperature which changes when
the La-sr ratio changes, but does not change with the addition of the zinc
impurities
Stability of metallic stripes in the extended one-band Hubbard model
Based on an unrestricted Gutzwiller approximation (GA) we investigate the
stripe orientation and periodicity in an extended one-band Hubbard model. A
negative ratio between next-nearest and nearest neighbor hopping t'/t, as
appropriate for cuprates, favors partially filled (metallic) stripes for both
vertical and diagonal configurations. At around optimal doping diagonal
stripes, site centered (SC) and bond centered (BC) vertical stripes become
degenerate suggesting strong lateral and orientational fluctuations. We find
that within the GA the resulting phase diagram is in agreement with experiment
whereas it is not in the Hartree-Fock approximation due to a strong
overestimation of the stripe filling. Results are in agreement with previous
calculations within the three-band Hubbard model but with the role of SC and BC
stripes interchanged.Comment: 10 pages, 8 figure
Theory of Kondo lattices and its application to high-temperature superconductivity and pseudo-gaps in cuprate oxides
A theory of Kondo lattices is developed for the t-J model on a square
lattice. The spin susceptibility is described in a form consistent with a
physical picture of Kondo lattices: Local spin fluctuations at different sites
interact with each other by a bare intersite exchange interaction, which is
mainly composed of two terms such as the superexchange interaction, which
arises from the virtual exchange of spin-channel pair excitations of electrons
across the Mott-Hubbard gap, and an exchange interaction arising from that of
Gutzwiller's quasi-particles. The bare exchange interaction is enhanced by
intersite spin fluctuations developed because of itself. The enhanced exchange
interaction is responsible for the development of superconducting fluctuations
as well as the Cooper pairing between Gutzwiller's quasi-particles. On the
basis of the microscopic theory, we develop a phenomenological theory of
low-temperature superconductivity and pseudo-gaps in the under-doped region as
well as high-temperature superconductivity in the optimal-doped region.
Anisotropic pseudo-gaps open mainly because of d\gamma-wave superconducting
low-energy fluctuations: Quasi-particle spectra around (\pm\pi/a,0) and
(0,\pm\pi/a), with a the lattice constant, or X points at the chemical
potential are swept away by strong inelastic scatterings, and quasi-particles
are well defined only around (\pm\pi/2a,\pm\pi/2a) on the Fermi surface or
line. As temperatures decrease in the vicinity of superconducting critical
temperatures, pseudo-gaps become smaller and the well-defined region is
extending toward X points. The condensation of d\gamma-wave Cooper pairs
eventually occurs at low enough temperatures when the pair breaking by
inelastic scatterings becomes small enough.Comment: 15 pages, 14 figure
Pentagonal nanowires: a first-principles study of atomic and electronic structure
We performed an extensive first-principles study of nanowires in various
pentagonal structures by using pseudopotential plane wave method within the
density functional theory. Our results show that nanowires of different types
of elements, such as alkali, simple, transition and noble metals and inert gas
atoms, have a stable structure made from staggered pentagons with a linear
chain perpendicular to the planes of the pentagons and passing through their
centers. This structure exhibits bond angles close to those in the icosahedral
structure. However, silicon is found to be energetically more favorable in the
eclipsed pentagonal structure. These quasi one dimensional pentagonal nanowires
have higher cohesive energies than many other one dimensional structures and
hence may be realized experimentally. The effect of magnetic state are examined
by spin-polarized calculations. The origin of the stability are discussed by
examining optimized structural parameters, charge density and electronic band
structure, and by using analysis based on the empirical Lennard-Jones type
interaction. Electronic band structure of pentagonal wires of different
elements are discussed and their effects on quantum ballistic conductance are
mentioned. It is found that the pentagonal wire of silicon exhibits metallic
band structure.Comment: 4 figures, accepted for publication in Phys. Rev.
Spectral functions, Fermi surface and pseudogap in the t-J model
Spectral functions within the generalized t-J model as relevant to cuprates
are analyzed using the method of equations of motion for projected fermion
operators. In the evaluation of the self energy the decoupling of spin and
single-particle fluctuations is performed. It is shown that in an undoped
antiferromagnet (AFM) the method reproduces the selfconsistent Born
approximation. For finite doping with short range AFM order the approximation
evolves into a paramagnon contribution which retains large incoherent
contribution in the hole part of the spectral function as well as the
hole-pocket-like Fermi surface at low doping. On the other hand, the
contribution of (longitudinal) spin fluctuations, with the coupling mostly
determined predominantly by J and next-neighbor hopping t', is essential for
the emergence of the pseudogap. The latter shows at low doping in the effective
truncation of the large Fermi surface, reduced electron density of states and
at the same time quasiparticle density of states at the Fermi level.Comment: RevTex, 13 pages, 11 figures (5 color