1,668 research outputs found

    Transfer of spectral weight across the gap of Sr2IrO4 induced by La doping

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    We study with Angle Resolved PhotoElectron Spectroscopy (ARPES) the evolution of the electronic structure of Sr2IrO4, when holes or electrons are introduced, through Rh or La substitutions. At low dopings, the added carriers occupy the first available states, at bottom or top of the gap, revealing an anisotropic gap of 0.7eV in good agreement with STM measurements. At further doping, we observe a reduction of the gap and a transfer of spectral weight across the gap, although the quasiparticle weight remains very small. We discuss the origin of the in-gap spectral weight as a local distribution of gap values

    Short small-polaron lifetime in the mixed-valence perovskite Cs2_2Au2_2I6_6 from high-pressure pump-probe experiments

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    We study the ultrafast phonon response of mixed-valence perovskite Cs2_2Au2_2I6_6 using pump-probe spectroscopy under high-pressure in a diamond anvil cell. We observed a remarkable softening and broadening of the Au - I stretching phonon mode with both applied pressure and photoexcitation. Using a double-pump scheme we measured a lifetime of the charge transfer excitation into single valence Au2+^{2+} of less than 4 ps, which is an indication of the local character of the Au2+^{2+} excitation. Furthermore, the strong similarity between the pressure and fluence dependence of the phonon softening shows that the inter-valence charge transfer plays an important role in the structural transition.Comment: 4 pages, 4 figure

    Characterizing Polytobacco Use Trajectories and Their Associations With Substance Use and Mental Health Across Mid-Adolescence.

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    Background:Polytobacco product use is suspected to be common, dynamic across time, and increase risk for adverse behavioral outcomes. We statistically modeled characteristic types of polytobacco use trajectories during mid-adolescence and tested their prospective association with substance use and mental health problems. Methods:Adolescents (N = 3393) in Los Angeles, CA, were surveyed semiannually from 9th to 11th grade. Past 6-month combustible cigarette, e-cigarette, or hookah use (yes/no) over four assessments were analyzed using parallel growth mixture modeling to identify a parsimonious set of polytobacco use trajectories. A tobacco product use trajectory group was used to predict substance use and mental health at the fifth assessment. Results:Three profiles were identified: (1) tobacco nonusers (N = 2291, 67.5%) with the lowest use prevalence (<3%) of all products across all timepoints; (2) polyproduct users (N = 920, 27.1%) with moderate use prevalence of each product (8-35%) that escalated for combustible cigarettes but decreased for e-cigarettes and hookah across time; and (3) chronic polyproduct users (N = 182, 5.4%) with high prevalence of each product use (38-86%) that escalated for combustible cigarettes and e-cigarettes. Nonusers, polyproduct users, and chronic polyproduct users reported successively higher alcohol, marijuana, and illicit drug use and ADHD at the final follow-up, respectively. Both tobacco using groups (vs. nonusers) reported greater odds of depression and anxiety at the final follow-up but did not differ from each other. Conclusions:Adolescent polytobacco use may involve a common moderate risk trajectory and a less common high-risk chronic trajectory. Both trajectories predict substance use and mental health symptomology. Implications:Variation in use and co-use of combustible cigarette, e-cigarette, and hookah use in mid-adolescence can be parsimoniously characterized by a small set common trajectory profiles in which polyproduct use are predominant patterns of tobacco product use, which predict adverse behavioral outcomes. Prevention and policy addressing polytobacco use (relative to single product use) may be optimal tobacco control strategies for youth, which may in turn prevent other forms of substance use and mental health problems

    Structure and Magnetic Properties of the Pyrochlore Iridate Y2Ir2O7

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    Neutron powder diffraction and inelastic measurements were performed examining the 5d pyrochlore Y2_2Ir2_2O7_7. Temperature dependent measurements were performed between 3.4 K and 290 K, spanning the magnetic transition at 155 K. No sign of any structural or disorder induced phase transition was observed over the entire temperature range. In addition, no sign of magnetic long-range order was observed to within the sensitivity of the instrumentation. These measurements do not rule out long range magnetic order, but the neutron powder diffraction structural refinements do put an upper bound for the ordered iridium moment of ∼\sim 0.2 μB/\mu_B /Ir (for a magnetic structure with wave vector Q≠0Q \neq 0) or ∼\sim 0.5 μB/\mu_B /Ir (for Q = 0).Comment: 5 pages, 8 figure

    A proposed prioritization system for the management of invasive alien plants in South Africa

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    Every country has weed species whose presence conflicts in some way with human management objectives and needs. Resources for research and control are limited, so priority should be given to species that are the biggest problem. The prioritization system described in this article was designed to assess objectively research and control priorities of invasive alien plants at a national scale in South Africa. The evaluation consists of seventeen criteria, grouped into five modules, that assess invasiveness, spatial characteristics, potential impact, potential for control, and conflicts of interest for each plant species under consideration. Total prioritization scores, calculated from criterion and module scores, were used to assess a species' priority. Prioritization scores were calculated by combining independent assessments provided by several experts, thus increasing the reliability of the rankings. The total confidence score, a separate index, indicates the reliability and availability of data used to make an assessment. Candidate species for evaluation were identified and assessed by several experts using the prioritization system. The final ranking was made by combining two separate indices, the total prioritization score and the total confidence score. This approach integrates the plant's perceived priority with an index of data reliability. Of the 61 species assessed, those with the highest ranks (Lantana camara, Chromolaena odorata and Opuntia ficus-indica) had high prioritization and high confidence scores, and are thus of most concern. Those species with the lowest ranks, for example, Harrisia martinii, Opuntia spinulifera and Opuntia exaltata, had low prioritization scores and high confidence scores, and thus are of least concern. Our approach to ranking weeds offers several advantages over existing systems because it is designed for multiple assessors based on the Delphi decision-making technique, the criteria contribute equally to the total score, and the system can accommodate incomplete data on a species. Although the choice of criteria may be criticized and the system has certain limitations, it appears to have delivered credible results

    A proposed prioritization system for the management of invasive alien plants in South Africa

    Get PDF
    Every country has weed species whose presence conflicts in some way with human management objectives and needs. Resources for research and control are limited, so priority should be given to species that are the biggest problem. The prioritization system described in this article was designed to assess objectively research and control priorities of invasive alien plants at a national scale in South Africa. The evaluation consists of seventeen criteria, grouped into five modules, that assess invasiveness, spatial characteristics, potential impact, potential for control, and conflicts of interest for each plant species under consideration. Total prioritization scores, calculated from criterion and module scores, were used to assess a species' priority. Prioritization scores were calculated by combining independent assessments provided by several experts, thus increasing the reliability of the rankings. The total confidence score, a separate index, indicates the reliability and availability of data used to make an assessment. Candidate species for evaluation were identified and assessed by several experts using the prioritization system. The final ranking was made by combining two separate indices, the total prioritization score and the total confidence score. This approach integrates the plant's perceived priority with an index of data reliability. Of the 61 species assessed, those with the highest ranks (Lantana camara, Chromolaena odorata and Opuntia ficus-indica) had high prioritization and high confidence scores, and are thus of most concern. Those species with the lowest ranks, for example, Harrisia martinii, Opuntia spinulifera and Opuntia exaltata, had low prioritization scores and high confidence scores, and thus are of least concern. Our approach to ranking weeds offers several advantages over existing systems because it is designed for multiple assessors based on the Delphi decision-making technique, the criteria contribute equally to the total score, and the system can accommodate incomplete data on a species. Although the choice of criteria may be criticized and the system has certain limitations, it appears to have delivered credible results

    Skyrmion Quantization and the Decay of the Delta

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    We present the complete solution to the so-called ``Yukawa problem'' of the Skyrme model. This refers to the perceived difficulty of reproducing---purely from soliton physics---the usual pseudovector pion-nucleon coupling, echoed by pion coupling to the higher spin/isospin baryons (I=J=3/2,5/2,⋯ ,Nc/2)(I=J=3/2 , 5/2 , \cdots , N_c/2 ) in a manner fixed by large-NcN_c group theory. The solution involves surprisingly elegant interplay between the classical and quantum properties of a new configuration, the ``new improved skyrmion''. This is the near-hedgehog obtained by minimizing the usual skyrmion mass functional augmented by an all-important isorotational kinetic term. The numerics are pleasing: a Δ\Delta decay width within a few MeV of its measured value, and furthermore, the higher-spin baryons (I=J≥5/2)(I=J \ge 5/2 ) with widths so large (Γ>800MeV\Gamma > 800 MeV) that these undesirable large-NcN_c artifacts effectively drop out of the spectrum, and pose no phenomenological problem. Beyond these specific results, we ground the Skyrme model in the Feynman Path Integral, and set up a transparent collective coordinate formalism that makes maximal use of the 1/Nc1/N_c expansion. This approach elucidates the connection between skyrmions on the one hand, and Feynman diagrams in an effective field theory on the other.Comment: This TeX file inputs the macropackage harvmac.tex . Choose the ``b'' (big) option or equations will overrun
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