10,452 research outputs found
Breakpoint lead-lag analysis of the last deglacial climate change andatmospheric CO2 concentration on global and hemispheric scales
Antarctic ice core records show that climate change and atmospheric CO2 concentration (aCO2) are closely related over the past 800 thousand years. However, the interpretation of their sequential, and hence the causal relationship has long been controversial. In this study, we revisit this long-standing scientific issue based on 88 well-dated high-resolution climate proxy records derived from ice cores, marine deposits, and stalagmites. We composite global and hemispheric stacks of the last deglacial climate index (DCI) using a normalization scheme instead of a more conventional area-weighting and mixing scheme to enable a better detection of temporal variations. Rampfit and Breakfit techniques are employed to detect the trend transitions in each composited DCI series and in the recently constructed centennial-scale aCO2 over the period from 22 to 9 thousand years before present. We detect a clear lead of DCI change over aCO2 variation on both global and hemispheric scales at the early stage of the deglaciation, suggesting that the variation of aCO2 is an internal feedback in Earth's climate system rather than an initial trigger of the last deglacial warming. During the periods of the Bølling-Allerød and the Younger Dryas, the climate system appeared to have been constrained by a fast coupling mechanism between climate change and aCO2 with no obvious asynchrony. The northern and southern hemispheric DCI stacks exhibit a seesawing pattern that can be linked to the influences of Atlantic meridional overturning circulation (AMOC) strength, revealing an important role of AMOC in regulating the global climate in the course of the last deglaciation.<br /
Role of stress-assisted martensite in the design of strong ultrafine-grained duplex steels
This work explains the occurrence of transformation-induced plasticity via
stress-assisted martensite, when designing ultrafine-grained duplex steels. It
is found that, when the austenite is reduced to a fine scale of about 300 nm,
the initial deformation-induced microstructure can be dominated by parallel
lamellae of epsilon martensite or mechanical twinning, which cannot efficiently
provide nucleation sites for strain-induced martensite. Hence, alpha martensite
nucleation occurs independently by a stress-assisted process that enhances
transformation-induced plasticity in ultrafine-grained austenite. This
metallurgical principle was validated experimentally by using a combination of
transmission Kikuchi diffraction mapping, transmission electron microscopy, and
atom probe microscopy, and demonstrated theoretically by the thermodynamics
model of stress-assisted martensite.The authors acknowledge the facilities, and the scientific and technical assistance of the
Australian Microscopy & Microanalysis Research Facility (ammrf.org.au) node at
Sydney Microscopy & Microanalysis, at the University of Sydney.This is the accepted manuscript. The final version is available from Elsevier at http://www.sciencedirect.com/science/article/pii/S1359645414006958
The Classical Harmonic Vibrations of the Atomic Centers of Mass with Micro Amplitudes and Low Frequencies Monitored by the Entanglement between the Two Two-level Atoms in a Single mode Cavity
We study the entanglement dynamics of the two two-level atoms coupling with a
single-mode polarized cavity field after incorporating the atomic centers of
mass classical harmonic vibrations with micro amplitudes and low frequencies.
We propose a quantitative vibrant factor to modify the concurrence of the two
atoms states. When the vibrant frequencies are very low, we obtain that: (i)
the factor depends on the relative vibrant displacements and the initial phases
rather than the absolute amplitudes, and reduces the concurrence to three
orders of magnitude; (ii) the concurrence increases with the increase of the
initial phases; (iii) the frequency of the harmonic vibration can be obtained
by measuring the maximal value of the concurrence during a small time. These
results indicate that even the extremely weak classical harmonic vibrations can
be monitored by the entanglement of quantum states.Comment: 10 pages, 3 figure
Large enhancement of the thermopower in NaCoO at high Na doping
Research on the oxide perovskites has uncovered electronic properties that
are strikingly enhanced compared with those in conventional metals. Examples
are the high critical temperatures of the cuprate superconductors and the
colossal magnetoresistance in the manganites. The conducting layered cobaltate
displays several interesting electronic phases as is varied
including water-induced superconductivity and an insulating state that is
destroyed by field. Initial measurements showed that, in the as-grown
composition, displays moderately large thermopower and
conductivity . However, the prospects for thermoelectric cooling
applications faded when the figure of merit was found to be small at this
composition (0.60.7). Here we report that, in the poorly-explored
high-doping region 0.75, undergoes an even steeper enhancement. At the
critical doping 0.85, (at 80 K) reaches values 40 times
larger than in the as-grown crystals. We discuss prospects for low-temperature
thermoelectric applications.Comment: 6 pages, 7 figure
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Collaborative development of diffraction-limited beamline optical systems at US DOE light sources
An ongoing collaboration among four US Department of Energy (DOE) National Laboratories has demonstrated key technology prototypes and software modeling tools required for new high-coherent flux beamline optical systems. New free electron laser (FEL) and diffraction-limited storage ring (DLSR) light sources demand wavefront preservation from source to sample to achieve and maintain optimal performance. Fine wavefront control was achieved using a novel, roomtemperature cooled mirror system called REAL (resistive element adjustable length) that combines cooling with applied, spatially variable auxiliary heating. Single-grating shearing interferometry (also called Talbot interferometry) and Hartmann wavefront sensors were developed and used for optical characterization and alignment on several beamlines, across a range of photon energies. Demonstrations of non-invasive hard x-ray wavefront sensing were performed using a thin diamond single-crystal as a beamsplitter
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Elucidating the Limit of Li Insertion into the Spinel Li4Ti5O12
In this work, we show that the well-known lithium-ion anode material, Li4Ti5O12, exhibits exceptionally high initial capacity of 310 mAh g-1 when it is discharged to 0.01 V. It maintains a reversible capacity of 230 mAh g-1, far exceeding the "theoretical" capacity of 175 mAh g-1 when this anode is lithiated to the composition Li7Ti5O12. Neutron diffraction analyses identify that additional Li reversibly enters into the Li7Ti5O12 to form Li8Ti5O12. density functional theory (DFT) calculations reveal the average potentials of the Li4Ti5O12 to Li7Ti5O12 step and the Li7Ti5O12 to Li8Ti5O12 step are 1.57 and 0.19 V, respectively, which are in excellent agreement with experimental results. Transmission electron microscopy (TEM) studies confirm that the irreversible capacity of Li4Ti5O12 during its first cycle originates from the formation of a solid electrolyte interface (SEI) layer. This work clarifies the fundamental lithiation mechanism of the Li4Ti5O12, when lithiated to 0.01 V vs Li
Strained graphene structures: from valleytronics to pressure sensing
Due to its strong bonds graphene can stretch up to 25% of its original size
without breaking. Furthermore, mechanical deformations lead to the generation
of pseudo-magnetic fields (PMF) that can exceed 300 T. The generated PMF has
opposite direction for electrons originating from different valleys. We show
that valley-polarized currents can be generated by local straining of
multi-terminal graphene devices. The pseudo-magnetic field created by a
Gaussian-like deformation allows electrons from only one valley to transmit and
a current of electrons from a single valley is generated at the opposite side
of the locally strained region. Furthermore, applying a pressure difference
between the two sides of a graphene membrane causes it to bend/bulge resulting
in a resistance change. We find that the resistance changes linearly with
pressure for bubbles of small radius while the response becomes non-linear for
bubbles that stretch almost to the edges of the sample. This is explained as
due to the strong interference of propagating electronic modes inside the
bubble. Our calculations show that high gauge factors can be obtained in this
way which makes graphene a good candidate for pressure sensing.Comment: to appear in proceedings of the NATO Advanced Research Worksho
The effects of supernovae on the dynamical evolution of binary stars and star clusters
In this chapter I review the effects of supernovae explosions on the
dynamical evolution of (1) binary stars and (2) star clusters.
(1) Supernovae in binaries can drastically alter the orbit of the system,
sometimes disrupting it entirely, and are thought to be partially responsible
for `runaway' massive stars - stars in the Galaxy with large peculiar
velocities. The ejection of the lower-mass secondary component of a binary
occurs often in the event of the more massive primary star exploding as a
supernova. The orbital properties of binaries that contain massive stars mean
that the observed velocities of runaway stars (10s - 100s km s) are
consistent with this scenario.
(2) Star formation is an inherently inefficient process, and much of the
potential in young star clusters remains in the form of gas. Supernovae can in
principle expel this gas, which would drastically alter the dynamics of the
cluster by unbinding the stars from the potential. However, recent numerical
simulations, and observational evidence that gas-free clusters are observed to
be bound, suggest that the effects of supernova explosions on the dynamics of
star clusters are likely to be minimal.Comment: 16 pages, to appear in the 'Handbook of Supernovae', eds. Paul Murdin
and Athem Alsabti. This version replaces an earlier version that contained
several typo
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