8 research outputs found

    Transiently enhanced interlayer tunneling in optically driven high-Tc superconductors

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    Recent pump-probe experiments reported an enhancement of superconducting transport along the c axis of underdoped YBa2Cu3O6+Ī“ (YBCO), induced by a midinfrared optical pump pulse tuned to a specific lattice vibration. To understand this transient nonequilibrium state, we develop a pump-probe formalism for a stack of Josephson junctions, and we consider the tunneling strengths in the presence of modulation with an ultrashort optical pulse. We demonstrate that a transient enhancement of the Josephson coupling can be obtained for pulsed excitation and that this can be even larger than in a continuously driven steady state. Especially interesting is the conclusion that the effect is largest when the material is parametrically driven at a frequency immediately above the plasma frequency, in agreement with what is found experimentally. For bilayer Josephson junctions, an enhancement similar to that experimentally is predicted below the critical temperature Tc. This model reproduces the essential features of the enhancement measured below Tc. To reproduce the experimental results above Tc, we will explore extensions of this model, such as in-plane and amplitude fluctuations, elsewhere.Deutsche Forschungsgemeinschaft; SFB 925; EXC 1074; Joachim Herz StiftungFirst author draf

    Research on Energy Dissipation in a Discharge Tunnel with a Plug Energy Dissipater

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    Plug energy dissipater, as a kind of effective energy dissipater with economic characteristics, has become very popular. The energy loss coefficient and the minimum wall pressure coefficient of the plug are two important factors in the plug energy dissipater design. In this paper, the two coefficients and relative parameters, such as the contraction ratio of the plug diameter to the flood discharge tunnel diameter, the ratio of the plug thickness to the tunnel diameter, and the Reynolds number of the flow through the plug, were analysed by theoretical considerations, and their relationship expressions were obtained by numerical simulations and were verified by experimental data. It could be concluded that the two coefficients were mainly dominated by the contraction ratio of the plug. The lower contraction ratio of the plug is, the larger are the two coefficients. The research results demonstrate that effects of the Reynolds number on the two coefficients can be neglected when this number is greater than 105; the relative thickness of the plug has little impact on them and can be neglected

    Ultrafast simultaneous manipulation of multiple ferroic orders through nonlinear phonon excitation

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    Recent experimental studies have demonstrated the possibility of utilizing strong terahertz pulses to manipulate individual ferroic orders on pico- and femtosecond timescales. Here, we extend these findings and showcase the simultaneous manipulation of multiple ferroic orders in BiFeO3_3, a material that is both ferroelectric and antiferromagnetic at room temperature. We find a concurrent enhancement of ferroelectric and antiferromagnetic second-harmonic generation (SHG) following the resonant excitation of a high-frequency fully-symmetric phonon mode. Based on first-principles calculations and phenomenological modeling, we ascribe this observation to the inherent coupling of the two ferroic orders to the nonequilibrium distortions induced in the crystal lattice by nonlinearly driven phonons. Our finding highlights the potential of nonlinear phononics as a technique for manipulating multiple ferroic order parameters at once. In addition, this approach provides a promising avenue to studying the dynamical magnetization and polarization behavior, as well as their intrinsic coupling, on ultrashort timescales.Comment: 18 pages, 5 figure

    Structural Property, Immunoreactivity and Gastric Digestion Characteristics of Glycated Parvalbumin from Mandarin Fish (<i>Siniperca chuaisi</i>) during Microwave-Assisted Maillard Reaction

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    This study was aimed to investigate the structural and immunological properties of parvalbumin from mandarin fish during the Maillard reaction. The microwave-assisted the Maillard reaction was optimized by orthogonal designed experiments. The results showed that the type of sugar and heating time had a significant effect on the Maillard reaction (p < 0.05). The SDS-PAGE analysis displayed that the molecular weight of parvalbumin in mandarin fish changed after being glycated with the Maillard reaction. The glycated parvalbumin was analyzed by Nano-LC-MS/MS and eleven glycation sites as well as five glycation groups were identified. By using the indirect competitive ELISA method, it was found that microwave heating gave a higher desensitization ability of mandarin fish parvalbumin than induction cooker did. In vitro gastric digestion experiments showed that microwave-heated parvalbumin was proved to be digested more easily than that cooked by induction cookers. The microwave-assisted Maillard reaction modified the structure of parvalbumin and reduced the immunoreactivity of parvalbumin of mandarin fish

    Transiently enhanced interlayer tunneling in optically driven high- T

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    Recent pump-probe experiments reported an enhancement of superconducting transport along the cc-axis of underdoped YBa2_2Cu3_3O6+Ī“_{6+\delta} (YBCO), induced by a mid-infrared optical pump pulse tuned to a specific lattice vibration. To understand this transient non-equilibrium state, we develop a pump-probe formalism for a stack of Josephson junctions, and we consider the tunneling strengths in presence of modulation with an ultrashort optical pulse. We demonstrate that a transient enhancement of the Josephson coupling can be obtained for pulsed excitation and that this can be even larger than in a continuously driven steady-state. Especially interesting is the conclusion that the effect is largest when the material is parametrically driven at a frequency immediately above the plasma frequency, in agreement with what is found experimentally. For bilayer Josephson junctions, an enhancement similar to that experimentally is predicted below the critical temperature TcT_c. This model reproduces the essential features of the enhancement measured below TcT_c. To reproduce the experimental results above TcT_c, we will explore extensions of this model, such as in-plane and amplitude fluctuations, elsewhere.Comment: 7 pages, 8 figure

    Pressure-Induced Phase Transitions and Correlation between Structure and Superconductivity in Iron-Based Superconductor Ce(O<sub>0.84</sub>F<sub>0.16</sub>)FeAs

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    High-pressure angle-dispersive X-ray diffraction experiments on iron-based superconductor CeĀ­(O<sub>0.84</sub>F<sub>0.16</sub>)Ā­FeAs were performed up to 54.9 GPa at room temperature. A tetragonal to tetragonal isostructural phase transition starts at about 13.9 GPa, and a new high-pressure phase has been found above 33.8 GPa. At pressures above 19.9 GPa, CeĀ­(O<sub>0.84</sub>F<sub>0.16</sub>)Ā­FeAs completely transforms to a high-pressure tetragonal phase, which remains in the same tetragonal structure with a larger <i>a</i>-axis and smaller <i>c</i>-axis than those of the low-pressure tetragonal phase. The structure analysis shows a discontinuity in the pressure dependences of the Feā€“As and Ceā€“(O, F) bond distances, as well as the Asā€“Feā€“As and Ceā€“(O, F)ā€“Ce bond angles in the transition region, which correlates with the change in <i>T</i><sub>c</sub> of this compound upon compression. The isostructural phase transition in CeĀ­(O<sub>0.84</sub>F<sub>0.16</sub>)Ā­FeAs leads to a drastic drop in the superconducting transition temperature <i>T</i><sub>c</sub> and restricts the superconductivity at low temperature. For the 1111-type iron-based superconductors, the structure evolution and following superconductivity changes under compression are related to the radius of lanthanide cations in the charge reservoir layer

    Enhanced photo-Fenton-like process over Z-scheme CoFe2O4/g-C3N4 Heterostructures under natural indoor light

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    Low-cost catalysts with high activity and stability toward producing strongly oxidative species are extremely desirable, but their development still remains a big challenge. Here, we report a novel strategy for the synthesis of a magnetic CoFe2O4/C3N4 hybrid via a simple self-assembly method. The CoFe2O4/C3N4 was utilized as a photo-Fenton-like catalyst for degradation of organic dyes in the presence of H2O2 under natural indoor light irradiation, a green and energy-saving approach for environmental cleaning. It was found the CoFe2O4/C3N4 hybrid with a CoFe2O4: g-C3N4 mass ratio of 2:1 can completely degrade Rhodamine B nearly 100 % within 210 min under room-light irradiation. The effects of the amount of H2O2 (0.01ā€“0.5 M), initial dye concentration (5ā€“20 mg/L), solution pH (3.08-10.09), fulvic acid concentration (5ā€“50 mg/L), different dyes and catalyst stability on the organic dye degradation were investigated. The introduction of CoFe2O4 on g-C3N4 produced an enhanced separation efficiency of photogenerated electron - hole pairs by a Z-scheme mechanism between the interfaces of g-C3N4 and CoFe2O4, leading to an excellent activity as compared with either g-C3N4 or CoFe2O4 and their mixture. This study demonstrates an efficient way to construct the low-cost magnetic CoFe2O4/C3N4 heterojunction as a typical Z-scheme system in environmental remediation
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