Validity of the linear coupling approximation in heavy-ion fusion reactions at sub barrier energies

The role of higher order coupling of surface vibrations to the relative motion in heavy-ion fusion reactions at near-barrier energies is investigated. The coupled channels equations are solved to all orders, and also in the linear and the quadratic coupling approximations. Taking $^{64}$Ni + $^{92,96}$Zr reactions as examples, it is shown that all order couplings lead to considerably improved agreement with the experimentally measured fusion cross sections and average angular momenta of the compound nucleus for such heavy nearly symmetric systems. The importance of higher order coupling is also examined for asymmetric systems like $^{16}$O + $^{112}$Cd, $^{144}$Sm, for which previous calculations of the fusion cross section seemed to indicate that the linear coupling approximation was adequate. It is shown that the shape of the barrier distributions and the energy dependence of the average angular momentum can change significantly when the higher order couplings are included, even for systems where measured fusion cross sections may seem to be well reproduced by the linear coupling approximation.Comment: Latex file, 15 pages, 6 figure

Suppression of complete fusion due to breakup in the reactions 10,11^{10,11}B + 209^{209}Bi

Above-barrier cross sections of $\alpha$-active heavy reaction products, as well as fission, were measured for the reactions of $^{10,11}$B with $^{209}$Bi. Detailed analysis showed that the heavy products include components from incomplete fusion as well as complete fusion (CF), but fission originates almost exclusively from CF. Compared with fusion calculations without breakup, the CF cross sections are suppressed by 15% for $^{10}$B and 7% for $^{11}$B. A consistent and systematic variation of the suppression of CF for reactions of the weakly bound nuclei $^{6,7}$Li, $^{9}$Be, $^{10,11}$B on targets of $^{208}$Pb and $^{209}$Bi is found as a function of the breakup threshold energy

Relating breakup and incomplete fusion of weakly-bound nuclei through a classical trajectory model with stochastic breakup

A classical dynamical model that treats break-up stochastically is presented for low energy reactions of weakly-bound nuclei. The three-dimensional model allows a consistent calculation of breakup, incomplete and complete fusion cross sections. The model is assessed by comparing the breakup observables with CDCC quantum mechanical predictions, which are found to be in reasonable agreement. Through the model, it is demonstrated that the breakup probability of the projectile as a function of its distance from the target is of primary importance for understanding complete and incomplete fusion at energies near the Coulomb barrier.Comment: Accepted in Physical Review Letter

Importance of Non-Linear Couplings in Fusion Barrier Distributions and Mean Angular Momenta

The effects of higher order coupling of surface vibrations to the relative motion on heavy-ion fusion reactions at near-barrier energies are investigated. The coupled channels equations are solved to all orders, and also in the linear and the quadratic coupling approximations. It is shown that the shape of fusion barrier distributions and the energy dependence of the average angular momentum of the compound nucleus can significantly change when the higher order couplings are included. The role of octupole vibrational excitation of ^{16}O in the ^{16}O + ^{144}Sm fusion reaction is also discussed using the all order coupled-channels equations.Comment: 8 pages, 6 figures, To be published in the Proceedings of the FUSION 97 Conference, South Durras, Australia, March 1997 (J. Phys. G

Novel insights into transfer processes in the reaction 16O+208Pb at sub-barrier energies

The collision of the doubly-magic nuclei $^{16}$O+$^{208}$Pb is a benchmark in nuclear reaction studies. Our new measurements of back-scattered projectile-like fragments at sub-barrier energies show show that transfer of 2 protons ($2p$) is much more probable than $\alpha$-particle transfer. $2p$ transfer probabilities are strongly enhanced compared to expectations for the sequential transfer of two uncorrelated protons; at energies around the fusion barrier absolute probabilities for two proton transfer are similar to those for one proton transfer. This strong enhancement indicates strong $2p$ pairing correlations in $^{16}$O, and suggests evidence for the occurrence of a nuclear supercurrent of two-proton Cooper pairs in this reaction, already at energies well below the fusion barrier.Comment: 5 pages, 3 figure

Atomic spectral-product representations of molecular electronic structure: metric matrices and atomic-product composition of molecular eigenfunctions

Recent progress is reported in development of ab initio computational methods for the electronic structures of molecules employing the many-electron eigenstates of constituent atoms in spectral-product forms. The approach provides a universal atomic-product description of the electronic structure of matter as an alternative to more commonly employed valence-bond- or molecular-orbital-based representations. The Hamiltonian matrix in this representation is seen to comprise a sum over atomic energies and a pairwise sum over Coulombic interaction terms that depend only on the separations of the individual atomic pairs. Overall electron antisymmetry can be enforced by unitary transformation when appropriate, rather than as a possibly encumbering or unnecessary global constraint. The matrix representative of the antisymmetrizer in the spectral-product basis, which is equivalent to the metric matrix of the corresponding explicitly antisymmetric basis, provides the required transformation to antisymmetric or linearly independent states after Hamiltonian evaluation. Particular attention is focused in the present report on properties of the metric matrix and on the atomic-product compositions of molecular eigenstates as described in the spectral-product representations. Illustrative calculations are reported for simple but prototypically important diatomic (H_2, CH) and triatomic (H_3, CH_2) molecules employing algorithms and computer codes devised recently for this purpose. This particular implementation of the approach combines Slater-orbital-based one- and two-electron integral evaluations, valence-bond constructions of standard tableau functions and matrices, and transformations to atomic eigenstate-product representations. The calculated metric matrices and corresponding potential energy surfaces obtained in this way elucidate a number of aspects of the spectral-product development, including the nature of closure in the representation, the general redundancy or linear dependence of its explicitly antisymmetrized form, the convergence of the apparently disparate atomic-product and explicitly antisymmetrized atomic-product forms to a common invariant subspace, and the nature of a chemical bonding descriptor provided by the atomic-product compositions of molecular eigenstates. Concluding remarks indicate additional studies in progress and the prognosis for performing atomic spectral-product calculations more generally and efficiently

Evidence of Double Phonon Excitations in ^{16}O + ^{208}Pb Reaction

The fusion cross-sections for ^{16}O + ^{208}Pb, measured to high precision, enable the extraction of the distribution of fusion barriers. This shows a structure markedly different from the single-barrier which might be expected for fusion of two doubly-closed shell nuclei. The results of exact coupled channel calculations performed to understand the observations are presented. These calculations indicate that coupling to a double octupole phonon excited state in ^{208}Pb is necessary to explain the experimental barrier distributions.Comment: 6 pages, 2 figures, To be published in the Proceedings of the FUSION 97 Conference, South Durras, Australia, March 1997 (J. Phys. G

An evaporation-based model of thermal neutron induced ternary fission of plutonium

Ternary fission probabilities for thermal neutron induced fission of plutonium are analyzed within the framework of an evaporation-based model where the complexity of time-varying potentials, associated with the neck collapse, are included in a simplistic fashion. If the nuclear temperature at scission and the fission-neck-collapse time are assumed to be ~1.2 MeV and ~10^-22 s, respectively, then calculated relative probabilities of ternary-fission light-charged-particle emission follow the trends seen in the experimental data. The ability of this model to reproduce ternary fission probabilities spanning seven orders of magnitude for a wide range of light-particle charges and masses implies that ternary fission is caused by the coupling of an evaporation-like process with the rapid re-arrangement of the nuclear fluid following scission.Comment: 25 pages, 12 figures, accepted for publication in IJMP

Effects of Nuclear Structure on Quasi-fission

The quasi-fission mechanism hinders fusion of heavy systems because of a mass flow between the reactants, leading to a re-separation of more symmetric fragments in the exit channel. A good understanding of the competition between fusion and quasi-fission mechanisms is expected to be of great help to optimize the formation and study of heavy and superheavy nuclei. Quantum microscopic models, such as the time-dependent Hartree-Fock approach, allow for a treatment of all degrees of freedom associated to the dynamics of each nucleon. This provides a description of the complex reaction mechanisms, such as quasi-fission, with no parameter adjusted on reaction mechanisms. In particular, the role of the deformation and orientation of a heavy target, as well as the entrance channel magicity and isospin are investigated with theoretical and experimental approaches.Comment: Invited talk to NSRT12. To be published in Eur. Phys. J. Web of Con