9,668 research outputs found
Optical signature of the pressure-induced dimerization in the honeycomb iridate -LiIrO
We studied the effect of external pressure on the electrodynamic properties
of -LiIrO single crystals in the frequency range of the phonon
modes and the Ir - transitions. The abrupt hardening of several phonon
modes under pressure supports the onset of the dimerized phase at the critical
pressure =3.8 GPa. With increasing pressure an overall decrease in
spectral weight of the Ir - transitions is found up to . Above
, the local (on-site) - excitations gain spectral weight with
increasing pressure, which hints at a pressure-induced increase in the
octahedral distortions. The non-local (intersite) Ir - transitions show a
monotonic blue-shift and decrease in spectral weight. The changes observed for
the non-local excitations are most prominent well above , namely for
pressures 12 GPa, and only small changes occur for pressures close to
. The profile of the optical conductivity at high pressures (20 GPa)
appears to be indicative for the dimerized state in iridates.Comment: 10 pages, 6 figures; accepted for publication in Phys. Rev.
Electron tunneling into a quantum wire in the Fabry-Perot regime
We study a gated quantum wire contacted to source and drain electrodes in the
Fabry-Perot regime. The wire is also coupled to a third terminal (tip), and we
allow for an asymmetry of the tip tunneling amplitudes of right and left moving
electrons. We analyze configurations where the tip acts as an electron injector
or as a voltage-probe, and show that the transport properties of this
three-terminal set-up exhibit very rich physical behavior. For a
non-interacting wire we find that a tip in the voltage-probe configuration
affects the source-drain transport in different ways, namely by suppressing the
conductance, by modulating the Fabry-Perot oscillations, and by reducing their
visibility. The combined effect of electron electron interaction and finite
length of the wire, accounted for by the inhomogeneous Luttinger liquid model,
leads to significantly modified predictions as compared to models based on
infinite wires. We show that when the tip injects electrons asymmetrically the
charge fractionalization induced by interaction cannot be inferred from the
asymmetry of the currents flowing in source and drain. Nevertheless interaction
effects are visible as oscillations in the non-linear tip-source and tip-drain
conductances. Important differences with respect to a two-terminal set-up
emerge, suggesting new strategies for the experimental investigation of
Luttinger liquid behavior.Comment: 27 pages, 10 figure
Noise in Electron Devices
Contains research objectives.Joint Services Electronics Programs (U. S. Army, U.S. Navy, and U.S. Air Force) under Contract DA 36-039-AMC-03200(E
Classical and quantum dynamics of a spin-1/2
We reply to a comment on `Semiclassical dynamics of a spin-1/2 in an
arbitrary magnetic field'.Comment: 4 pages, submitted to Journal of Physics
Computer simulation of crystallization kinetics with non-Poisson distributed nuclei
The influence of non-uniform distribution of nuclei on crystallization
kinetics of amorphous materials is investigated. This case cannot be described
by the well-known Johnson-Mehl-Avrami (JMA) equation, which is only valid under
the assumption of a spatially homogeneous nucleation probability. The results
of computer simulations of crystallization kinetics with nuclei distributed
according to a cluster and a hardcore distribution are compared with JMA
kinetics. The effects of the different distributions on the so-called Avrami
exponent are shown. Furthermore, we calculate the small-angle scattering
curves of the simulated structures which can be used to distinguish
experimentally between the three nucleation models under consideration.Comment: 14 pages including 7 postscript figures, uses epsf.sty and
ioplppt.st
High-pressure versus isoelectronic doping effect on the honeycomb iridate NaIrO
We study the effect of isoelectronic doping and external pressure in tuning
the ground state of the honeycomb iridate NaIrO by combining optical
spectroscopy with synchrotron x-ray diffraction measurements on single
crystals. The obtained optical conductivity of NaIrO is discussed in
terms of a Mott insulating picture versus the formation of quasimolecular
orbitals and in terms of Kitaev-interactions. With increasing Li content ,
(NaLi)IrO moves deeper into the Mott insulating regime and
there are indications that up to a doping level of 24\% the compound comes
closer to the Kitaev-limit. The optical conductivity spectrum of single
crystalline -LiIrO does not follow the trends observed for the
series up to . There are strong indications that -LiIrO
is less close to the Kitaev-limit compared to NaIrO and closer to the
quasimolecular orbital picture. Except for the pressure-induced hardening of
the phonon modes, the optical properties of NaIrO seem to be robust
against external pressure. Possible explanations of the unexpected evolution of
the optical conductivity with isolectronic doping and the drastic change
between and are given by comparing the pressure-induced changes
of lattice parameters and the optical conductivity with the corresponding
changes induced by doping.Comment: 12 pages, 6 figures, accepted for publication in Phys. Rev.
Tunneling Density of States of the Interacting Two-Dimensional Electron Gas
We investigate the influence of electron--electron interactions on the
density of states of a ballistic two--dimensional electron gas. The density of
states is determined nonperturbatively by means of path integral techniques
allowing for reliable results near the Fermi surface, where perturbation theory
breaks down. We find that the density of states is suppressed at the Fermi
level to a finite value. This suppression factor grows with decreasing electron
density and is weakened by the presence of gates.Comment: 4 pages, 2 figures; slightly shortened version published in PR
The convergence of the ab-initio many-body expansion for the cohesive energy of solid mercury
A many-body expansion for mercury clusters of the form E = \sum_{i<j}\Delta
\epsilon_{ij} + \sum_{i<j<k}\Delta \epsilon_{ijk} + ... \quad, does not
converge smoothly with increasing cluster size towards the solid state. Even
for smaller cluster sizes (up to n=6), where van der Waals forces still
dominate, one observes bad convergence behaviour. For solid mercury the
convergence of the many-body expansion can dramatically be improved by an
incremental procedure within an embedded cluster approach. Here one adds the
coupled cluster many-body electron correlation contributions of the embedded
cluster to the bulk HF energy. In this way we obtain a cohesive energy (not
corrected for zero-point vibration) of 0.79 eV in perfect agreement with the
experimental value.Comment: 10 pages, 3 figures, accepted PR
Jahn-Teller Distortions and the Supershell Effect in Metal Nanowires
A stability analysis of metal nanowires shows that a Jahn-Teller deformation
breaking cylindrical symmetry can be energetically favorable, leading to stable
nanowires with elliptic cross sections. The sequence of stable cylindrical and
elliptical nanowires allows for a consistent interpretation of experimental
conductance histograms for alkali metals, including both the shell and
supershell structures. It is predicted that for gold, elliptical nanowires are
even more likely to form since their eccentricity is smaller than for alkali
metals. The existence of certain metastable ``superdeformed'' nanowires is also
predicted
Electrodynamics of Media
Contains reports on two research projects.Joint Services Electronics Programs (U. S. Army, U. S. Navy, and U. S. Air Force) under Contract DA 28-043-AMC-02536(E
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