789 research outputs found
Bottlenecks in Two-Hop Ad Hoc Networks - Dividing Radio Capacity in a Smart Way
In two-hop ad hoc networks the available radio capacity tends to be equally shard among the contending stations, which may lead to bottleneck situations in case of unbalanced traffic routing. We propose a generic model for evaluating adaptive capacity sharing strategies. We use infinite-state stochastic Petri nets for modeling the system and use the logic CSRL for specifying the measures of interest
Bond disproportionation and dynamical charge fluctuations in the perovskite rare earth nickelates
We present a theory describing the local electronic properties of the
perovskite rare earth nickelates--materials which have negative charge transfer
energies, strong O -- Ni covalence, and breathing mode lattice
distortions at the origin of highly studied metal-insulator and
antiferromagnetic ordering transitions. Utilizing a full orbital, full
correlation double cluster approach, we find strong charge fluctuations in
agreement with a bond disproportionation interpretation. The unique double
cluster formulation permits the inclusion of necessary orbital degeneracies and
Coulomb interactions to calculate resonant x-ray spectral responses, with which
we find excellent agreement with well-established experimental results. This
previously absent, crucial link between theory and experiment provides
validation of the recently proposed bond disproportionation theory, and
provides an analysis methodology for spectroscopic studies of engineered phases
of nickelates and other high valence transition metal compounds
Symmetry analysis of magneto-optical effects: The case of x-ray diffraction and x-ray absorption at the transition metal L23 edge
A general symmetry analysis of the optical conductivity or scattering tensor
is used to rewrite the conductivity tensor as a sum of fundamental spectra
multiplied by simple functions depending on the local magnetization direction.
Using this formalism, we present several numerical examples at the transition
metal L23 edge. From these numerical calculations we can conclude that large
deviations from the magneto-optical effects in spherical symmetry are found.
These findings are in particular important for resonant x-ray diffraction
experiments where the polarization dependence and azimuthal dependence of the
scattered Bragg intensity is used to determine the local ordered magnetization
direction
Bands, resonances, edge singularities and excitons in core level spectroscopy investigated within the dynamical mean field theory
Using a recently developed impurity solver we exemplify how dynamical mean
field theory captures band excitations, resonances, edge singularities and
excitons in core level x-ray absorption (XAS) and core level photo electron
spectroscopy (cPES) on metals, correlated metals and Mott insulators. Comparing
XAS at different values of the core-valence interaction shows how the
quasiparticle peak in the absence of core-valence interactions evolves into a
resonance of similar shape, but different origin. Whereas XAS is rather
insensitive to the metal insulator transition, cPES can be used, due to
nonlocal screening, to measure the amount of local charge fluctuation
Strong spin-orbit coupling effects on the Fermi surface of Sr2RuO4 and Sr2RhO4
We present a first-principle study of spin-orbit coupling effects on the
Fermi surface of Sr2RuO4 and Sr2RhO4. For nearly degenerate bands, spin-orbit
coupling leads to a dramatic change of the Fermi surface with respect to
non-relativistic calculations; as evidenced by the comparison with experiments
on Sr2RhO4, it cannot be disregarded. For Sr2RuO4, the Fermi surface
modifications are more subtle but equally dramatic in the detail: spin-orbit
coupling induces a strong momentum dependence, normal to the RuO2 planes, for
both orbital and spin character of the low-energy electronic states. These
findings have profound implications for the understanding of unconventional
superconductivity in Sr2RuO4.Comment: A high-resolution version can be found at
http://www.physics.ubc.ca/~quantmat/ARPES/PUBLICATIONS/Articles/SO_Sr2RuO4.pd
Spin-state transition in LaCoO3: direct neutron spectroscopic evidence of excited magnetic states
A gradual spin-state transition occurs in LaCoO3 around T~80-120 K, whose
detailed nature remains controversial. We studied this transition by means of
inelastic neutron scattering (INS), and found that with increasing temperature
an excitation at ~0.6 meV appears, whose intensity increases with temperature,
following the bulk magnetization. Within a model including crystal field
interaction and spin-orbit coupling we interpret this excitation as originating
from a transition between thermally excited states located about 120 K above
the ground state. We further discuss the nature of the magnetic excited state
in terms of intermediate-spin (IS, S=1) vs. high-spin (HS, S=2) states. Since
the g-factor obtained from the field dependence of the INS is g~3, the second
interpretation looks more plausible.Comment: 10 pages, 4 figure
High multipole transitions in NIXS: valence and hybridization in 4f systems
Momentum-transfer (q) dependent non-resonant inelastic x-ray scattering
measurements were made at the N4,5 edges for several rare earth compounds. With
increasing q, giant dipole resonances diminish, to be replaced by strong
multiplet lines at lower energy transfer. These multiplets result from two
different orders of multipole scattering and are distinct for systems with
simple 4f^0 and 4f^1 initial states. A many-body theoretical treatment of the
multiplets agrees well with the experimental data on ionic La and Ce phosphate
reference compounds. Comparing measurements on CeO2 and CeRh3 to the theory and
the phosphates indicates sensitivity to hybridization as observed by a
broadening of 4f^0-related multiplet features. We expect such strong, nondipole
features to be generic for NIXS from f-electron systems
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