508 research outputs found
Structural and Magnetic Properties of Pyrochlore Solid Solutions (Y,Lu)2Ti2-x(Nb,Ta)xO7+/-y
The synthesis and characterization of the pyrochlore solid solutions,
Y2Ti2-xNbxO7-y, Lu2Ti2-xNbxO7-y, Y2Ti2-xTaxO7-y and Lu2TiTaO7-y (-0.4<y<0.5),
is described. Synthesis at 1600 C, and 10-5 Torr yields oxygen deficiency in
all systems. All compounds are found to be paramagnetic and semiconducting,
with the size of the local moments being less, in some cases substantially
less, than the expected value for the number of nominally unpaired electrons
present. Thermogravimetric analysis (TGA) shows that all compounds can be fully
oxidized while retaining the pyrochlore structure, yielding oxygen rich
pyrochlores as white powders. Powder neutron diffraction of Y2TiNbO7-based
samples was done. Refinement of the data for oxygen deficient Y2TiNbO6.76
indicates the presence of a distribution of oxygen over the 8b and 48f sites.
Refinement of the data for oxygen rich Y2TiNbO7.5 shows these sites to be
completely filled, with an additional half filling of the 8a site. The magnetic
and TGA data strongly suggest a preference for a Ti3+/(Nb,Ta)5+ combination, as
opposed to Ti4+/(Nb,Ta)4+, in this pyrochlore family. In addition, the evidence
clearly points to Ti3+ as the source of the localized moments, with no evidence
for localized Nb4+ moments.Comment: Accepted to Journal of Solid State Chemistr
Neutrino oscillations in the early universe: How large lepton asymmetry can be generated?
The lepton asymmetry that could be generated in the early universe through
oscillations of active to sterile neutrinos is calculated (almost) analytically
for small mixing angles, sin 2\theta < 10^{-2}. It is shown that for a mass
squared difference, \delta m^2=-1 eV^2 it may rise at most by 6 orders of
magnitude from the initial ``normal'' value of 10^{-10}, since the
back-reaction from the refraction index terminates this rise while the
asymmetry is still small. Only for very large mass differences, \delta m^2
about 10^9 eV^2, the lepton asymmetry could reach a significant magnitude
exceeding 0.1.Comment: 25 pages, LaTeX (5 graphs
Controlling laser spectra in a phaseonium photonic crystal using maser
We study the control of quantum resonances in photonic crystals with
electromagnetically induced transparency driven by microwave field. In addition
to the control laser, the intensity and phase of the maser can alter the
transmission and reflection spectra in interesting ways, producing hyperfine
resonances through the combined effects of multiple scattering in the
superstructure.Comment: 7 pages, 4 figure
Randomly dilute Ising model: A nonperturbative approach
The N-vector cubic model relevant, among others, to the physics of the
randomly dilute Ising model is analyzed in arbitrary dimension by means of an
exact renormalization-group equation. This study provides a unified picture of
its critical physics between two and four dimensions. We give the critical
exponents for the three-dimensional randomly dilute Ising model which are in
good agreement with experimental and numerical data. The relevance of the cubic
anisotropy in the O(N) model is also treated.Comment: 4 pages, published versio
Predicted Infrared and Raman Spectra for Neutral Ti_8C_12 Isomers
Using a density-functional based algorithm, the full IR and Raman spectra are
calculated for the neutral Ti_8C_12 cluster assuming geometries of Th, Td, D2d
and C3v symmetry. The Th pentagonal dodecahedron is found to be dynamically
unstable. The calculated properties of the relaxed structure having C3v
symmetry are found to be in excellent agreement with experimental gas phase
infrared results, ionization potential and electron affinity measurements.
Consequently, the results presented may be used as a reference for further
experimental characterization using vibrational spectroscopy.Comment: 6 pages, 5 figures. Physical Review A, 2002 (in press
Single Photons on Pseudo-Demand from Stored Parametric Down-Conversion
We describe the results of a parametric down-conversion experiment in which
the detection of one photon of a pair causes the other photon to be switched
into a storage loop. The stored photon can then be switched out of the loop at
a later time chosen by the user, providing a single photon for potential use in
a variety of quantum information processing applications. Although the stored
single photon is only available at periodic time intervals, those times can be
chosen to match the cycle time of a quantum computer by using pulsed
down-conversion. The potential use of the storage loop as a photonic quantum
memory device is also discussed.Comment: 8 pages, 7 Figs., RevTe
Microscopic mechanisms of spin-dependent electric polarization in 3d oxides
We present a short critical overview of different microscopic models for
nonrelativistic and relativistic magnetoelectric coupling including the
so-called "spin current scenario", ab-initio calculations, and several recent
microscopic approaches to a spin-dependent electric polarization in 3d oxides.Comment: 8 pages, 3 figure
Selective quantum evolution of a qubit state due to continuous measurement
We consider a two-level quantum system (qubit) which is continuously measured
by a detector. The information provided by the detector is taken into account
to describe the evolution during a particular realization of measurement
process. We discuss the Bayesian formalism for such ``selective'' evolution of
an individual qubit and apply it to several solid-state setups. In particular,
we show how to suppress the qubit decoherence using continuous measurement and
the feedback loop.Comment: 15 pages (including 9 figures
The Harris-Luck criterion for random lattices
The Harris-Luck criterion judges the relevance of (potentially) spatially
correlated, quenched disorder induced by, e.g., random bonds, randomly diluted
sites or a quasi-periodicity of the lattice, for altering the critical behavior
of a coupled matter system. We investigate the applicability of this type of
criterion to the case of spin variables coupled to random lattices. Their
aptitude to alter critical behavior depends on the degree of spatial
correlations present, which is quantified by a wandering exponent. We consider
the cases of Poissonian random graphs resulting from the Voronoi-Delaunay
construction and of planar, ``fat'' Feynman diagrams and precisely
determine their wandering exponents. The resulting predictions are compared to
various exact and numerical results for the Potts model coupled to these
quenched ensembles of random graphs.Comment: 13 pages, 9 figures, 2 tables, REVTeX 4. Version as published, one
figure added for clarification, minor re-wordings and typo cleanu
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