56 research outputs found
Local breaking of four-fold rotational symmetry by short-range magnetic order in heavily overdoped Ba(FeCu)As
We investigate Cu-doped Ba(FeCu)As with transport,
magnetic susceptibility, and elastic neutron scattering measurements. In the
heavily Cu-doped regime where long-range stripe-type antiferromagnetic order in
BaFeAs is suppressed, Ba(FeCu)As (0.145 0.553) samples exhibit spin-glass-like behavior in magnetic
susceptibility and insulating-like temperature dependence in electrical
transport. Using elastic neutron scattering, we find stripe-type short-range
magnetic order in the spin-glass region identified by susceptibility
measurements. The persistence of short-range magnetic order over a large doping
range in Ba(FeCu)As likely arises from local arrangements
of Fe and Cu that favor magnetic order, with Cu acting as vacancies relieving
magnetic frustration and degeneracy. These results indicate locally broken
four-fold rotational symmetry, suggesting that stripe-type magnetism is
ubiquitous in iron pnictides.Comment: accepted by Physical Review B Rapid Communication
Strict limit on in-plane ordered magnetic dipole moment in URu2Si2
Neutron diffraction is used to examine the polarization of weak static
antiferromagnetism in high quality single crystalline URu2Si2. As previously
documented, elastic Bragg-like diffraction develops for temperature T<T_{HO}=
17.5 K at q=(100) but not at wave vector transfer q=(001). The peak width
indicates correlation lengths \xi_c=230(12) \AA \ and \xi_a=240(15) \AA. The
integrated intensity of the T-dependent peaks corresponds to a sample averaged
c-oriented staggered moment of \mu_{c}=0.022(1) \mu_B at T=1.7 K. The absence
of T-dependent diffraction at q=(001) places a limit \mu_{\perp}<0.0011 \mu_B
on an f- or d-orbital based in-plane staggered magnetic dipole moment, which is
associated with multipolar orders proposed for URu_2Si_2.Comment: 9 pages, 7 figure
Temperature dependence of the resonance and low energy spin excitations in superconducting FeTeSe
We use inelastic neutron scattering to study the temperature dependence of
the low-energy spin excitations in single crystals of superconducting
FeTeSe ( K). In the low-temperature superconducting
state, the imaginary part of the dynamic susceptibility at the electron and
hole Fermi surfaces nesting wave vector ,
, has a small spin gap, a two-dimensional
neutron spin resonance above the spin gap, and increases linearly with
increasing for energies above the resonance. While the intensity
of the resonance decreases like an order parameter with increasing temperature
and disappears at temperature slightly above , the energy of the mode is
weakly temperature dependent and vanishes concurrently above . This
suggests that in spite of its similarities with the resonance in electron-doped
superconducting BaFe(Co,Ni)As, the mode in
FeTeSe is not directly associated with the superconducting
electronic gap.Comment: 7 pages, 6 figure
Short-range cluster spin glass near optimal superconductivity in BaFeNiAs
High-temperature superconductivity in iron pnictides occurs when electrons
are doped into their antiferromagnetic (AF) parent compounds. In addition to
inducing superconductivity, electron-doping also changes the static
commensurate AF order in the undoped parent compounds into short-range
incommensurate AF order near optimal superconductivity. Here we use neutron
scattering to demonstrate that the incommensurate AF order in
BaFeNiAs is not a spin-density-wave arising from the
itinerant electrons in nested Fermi surfaces, but consistent with a cluster
spin glass in the matrix of the superconducting phase. Therefore, optimal
superconductivity in iron pnictides coexists and competes with a mesoscopically
separated cluster spin glass phase, much different from the homogeneous
coexisting AF and superconducting phases in the underdoped regime.Comment: 4 figure
Electron doping evolution of the neutron spin resonance in NaFeCoAs
Neutron spin resonance, a collective magnetic excitation coupled to
superconductivity, is one of the most prominent features shared by a broad
family of unconventional superconductors including copper oxides, iron
pnictides, and heavy fermions. In this work, we study the doping evolution of
the resonances in NaFeCoAs covering the entire superconducting
dome. For the underdoped compositions, two resonance modes coexist. As doping
increases, the low-energy resonance gradually loses its spectral weight to the
high-energy one but remains at the same energy. By contrast, in the overdoped
regime we only find one single resonance, which acquires a broader width in
both energy and momentum, but retains approximately the same peak position even
when drops by nearly a half compared to optimal doping. These results
suggest that the energy of the resonance in electron overdoped
NaFeCoAs is neither simply proportional to nor the
superconducting gap, but is controlled by the multi-orbital character of the
system and doped impurity scattering effect.Comment: accepted by PR
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