Quantum Monte Carlo and exact diagonalization study of a dynamic Hubbard model

A one-dimensional model of electrons locally coupled to spin-1/2 degrees of freedom is studied by numerical techniques. The model is one in the class of $dynamic$ $Hubbard$ $models$ that describe the relaxation of an atomic orbital upon double electron occupancy due to electron-electron interactions. We study the parameter regime where pairing occurs in this model by exact diagonalization of small clusters. World line quantum Monte Carlo simulations support the results of exact diagonalization for larger systems and show that kinetic energy is lowered when pairing occurs. The qualitative physics of this model and others in its class, obtained through approximate analytic calculations, is that superconductivity occurs through hole undressing even in parameter regimes where the effective on-site interaction is strongly repulsive. Our numerical results confirm the expected qualitative behavior, and show that pairing will occur in a substantially larger parameter regime than predicted by the approximate low energy effective Hamiltonian.Comment: Some changes made in response to referees comments. To be published in Phys.Rev.

Correcting 100 years of misunderstanding: electric fields in superconductors, hole superconductivity, and the Meissner effect

From the outset of superconductivity research it was assumed that no electrostatic fields could exist inside superconductors, and this assumption was incorporated into conventional London electrodynamics. Yet the London brothers themselves initially (in 1935) had proposed an electrodynamic theory of superconductors that allowed for static electric fields in their interior, which they unfortunately discarded a year later. I argue that the Meissner effect in superconductors necessitates the existence of an electrostatic field in their interior, originating in the expulsion of negative charge from the interior to the surface when a metal becomes superconducting. The theory of hole superconductivity predicts this physics, and associated with it a macroscopic spin current in the ground state of superconductors ("Spin Meissner effect"), qualitatively different from what is predicted by conventional BCS-London theory. A new London-like electrodynamic description of superconductors is proposed to describe this physics. Within this theory superconductivity is driven by lowering of quantum kinetic energy, the fact that the Coulomb repulsion strongly depends on the character of the charge carriers, namely whether electron- or hole-like, and the spin-orbit interaction. The electron-phonon interaction does not play a significant role, yet the existence of an isotope effect in many superconductors is easily understood. In the strong coupling regime the theory appears to favor local charge inhomogeneity. The theory is proposed to apply to all superconducting materials, from the elements to the high $T_c$ cuprates and pnictides, is highly falsifiable, and explains a wide variety of experimental observations.Comment: Proceedings of the conference "Quantum phenomena in complex matter 2011 - Stripes 2011", Rome, 10 July -16 July 2011, to be published in J. Supercond. Nov. Mag

Meissner effect, Spin Meissner effect and charge expulsion in superconductors

The Meissner effect and the Spin Meissner effect are the spontaneous generation of charge and spin current respectively near the surface of a metal making a transition to the superconducting state. The Meissner effect is well known but, I argue, not explained by the conventional theory, the Spin Meissner effect has yet to be detected. I propose that both effects take place in all superconductors, the first one in the presence of an applied magnetostatic field, the second one even in the absence of applied external fields. Both effects can be understood under the assumption that electrons expand their orbits and thereby lower their quantum kinetic energy in the transition to superconductivity. Associated with this process, the metal expels negative charge from the interior to the surface and an electric field is generated in the interior. The resulting charge current can be understood as arising from the magnetic Lorentz force on radially outgoing electrons, and the resulting spin current can be understood as arising from a spin Hall effect originating in the Rashba-like coupling of the electron magnetic moment to the internal electric field. The associated electrodynamics is qualitatively different from London electrodynamics, yet can be described by a small modification of the conventional London equations. The stability of the superconducting state and its macroscopic phase coherence hinge on the fact that the orbital angular momentum of the carriers of the spin current is found to be exactly $\hbar/2$, indicating a topological origin. The simplicity and universality of our theory argue for its validity, and the occurrence of superconductivity in many classes of materials can be understood within our theory.Comment: Submitted to SLAFES XX Proceeding

Quasiparticle undressing in a dynamic Hubbard model: exact diagonalization study

Dynamic Hubbard models have been proposed as extensions of the conventional Hubbard model to describe the orbital relaxation that occurs upon double occupancy of an atomic orbital. These models give rise to pairing of holes and superconductivity in certain parameter ranges. Here we explore the changes in carrier effective mass and quasiparticle weight and in one- and two-particle spectral functions that occur in a dynamic Hubbard model upon pairing, by exact diagonalization of small systems. It is found that pairing is associated with lowering of effective mass and increase of quasiparticle weight, manifested in transfer of spectral weight from high to low frequencies in one- and two-particle spectral functions. This 'undressing' phenomenology resembles observations in transport, photoemission and optical experiments in high T_c cuprates. This behavior is contrasted with that of a conventional electron-hole symmetric Holstein-like model with attractive on-site interaction, where pairing is associated with 'dressing' instead of 'undressing'

Electromotive forces and the Meissner effect puzzle

In a voltaic cell, positive (negative) ions flow from the low (high) potential electrode to the high (low) potential electrode, driven by an `electromotive force' which points in opposite direction and overcomes the electric force. Similarly in a superconductor charge flows in direction opposite to that dictated by the Faraday electric field as the magnetic field is expelled in the Meissner effect. The puzzle is the same in both cases: what drives electric charges against electromagnetic forces? I propose that the answer is also the same in both cases: kinetic energy lowering, or `quantum pressure'

Electronic dynamic Hubbard model: exact diagonalization study

A model to describe electronic correlations in energy bands is considered. The model is a generalization of the conventional Hubbard model that allows for the fact that the wavefunction for two electrons occupying the same Wannier orbital is different from the product of single electron wavefunctions. We diagonalize the Hamiltonian exactly on a four-site cluster and study its properties as function of band filling. The quasiparticle weight is found to decrease and the quasiparticle effective mass to increase as the electronic band filling increases, and spectral weight in one- and two-particle spectral functions is transfered from low to high frequencies as the band filling increases. Quasiparticles at the Fermi energy are found to be more 'dressed' when the Fermi level is in the upper half of the band (hole carriers) than when it is in the lower half of the band (electron carriers). The effective interaction between carriers is found to be strongly dependent on band filling becoming less repulsive as the band filling increases, and attractive near the top of the band in certain parameter ranges. The effective interaction is most attractive when the single hole carriers are most heavily dressed, and in the parameter regime where the effective interaction is attractive, hole carriers are found to 'undress', hence become more like electrons, when they pair. It is proposed that these are generic properties of electronic energy bands in solids that reflect a fundamental electron-hole asymmetry of condensed matter. The relation of these results to the understanding of superconductivity in solids is discussed.Comment: Small changes following referee's comment

Consequences of charge imbalance in superconductors within the theory of hole superconductivity

The theory of hole superconductivity proposes that the fundamental asymmetry between electrons and holes in solids is responsible for superconductivity. Here we point out a remarkable consequence of this theory: a tendency for negative charge to be expelled from the bulk of the superconductor towards the surface. Experimentally observable consequences of this physics are discussed

Metallic ferromagnetism without exchange splitting

In the band theory of ferromagnetism there is a relative shift in the position of majority and minority spin bands due to the self-consistent field due to opposite spin electrons. In the simplest realization, the Stoner model, the majority and minority spin bands are rigidly shifted with respect to each other. Here we consider models at the opposite extreme, where there is no overall shift of the energy bands. Instead, upon spin polarization one of the bands broadens relative to the other. Ferromagnetism is driven by the resulting gain in kinetic energy. A signature of this class of mechanisms is that a transfer of spectral weight in optical absorption from high to low frequencies occurs upon spin polarization. We show that such models arise from generalized tight binding models that include off-diagonal matrix elements of the Coulomb interaction. For certain parameter ranges it is also found that reentrant ferromagnetism occurs. We examine properties of these models at zero and finite temperatures, and discuss their possible relevance to real materials

Spontaneous spinning of a magnet levitating over a superconductor

A permanent magnet levitating over a superconductor is found to spontaneously spin, overcoming resistance to air friction. We explain the physics behind this remarkable effect.Comment: See http://physics.ucsd.edu/~jorge/spinning.html for movie clips of the effec

Optical sum rule violation, superfluid weight and condensation energy in the cuprates

The model of hole superconductivity predicts that the superfluid weight in the zero-frequency $\delta$-function in the optical conductivity has an anomalous contribution from high frequencies, due to lowering of the system's kinetic energy upon entering the superconducting state. The lowering of kinetic energy, mainly in-plane in origin, accounts for both the condensation energy of the superconductor as well as an increased potential energy due to larger Coulomb repulsion in the paired state. It leads to an apparent violation of the conductivity sum rule, which in the clean limit we predict to be substantially larger for in-plane than for c-axis conductivity. However, because cuprates are in the dirty limit for c-axis transport, the sum rule violation is found to be greatly enhanced in the c-direction. The model predicts the sum rule violation to be largest in the underdoped regime and to decrease with doping, more rapidly in the c-direction that in the plane. So far, experiments have detected sum rule violation in c-axis transport in several cuprates, as well as a decrease and disappearance of this violation for increasing doping, but no violation in-plane. We explore the predictions of the model for a wide range of parameters, both in the absence and in the presence of disorder, and the relation with current experimental knowledge.Comment: submitted to Phys.Rev.