374,905 research outputs found

    Optical spectroscopy study of Nd(O,F)BiS2 single crystals

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    We present an optical spectroscopy study on F-substituted NdOBiS2_2 superconducting single crystals grown using KCl/LiCl flux method. The measurement reveals a simple metallic response with a relatively low screened plasma edge near 5000 \cm. The plasma frequency is estimated to be 2.1 eV, which is much smaller than the value expected from the first-principles calculations for an electron doping level of x=0.5, but very close to the value based on a doping level of 7%\% of itinerant electrons per Bi site as determined by ARPES experiment. The energy scales of the interband transitions are also well reproduced by the first-principles calculations. The results suggest an absence of correlation effect in the compound, which essentially rules out the exotic pairing mechanism for superconductivity or scenario based on the strong electronic correlation effect. The study also reveals that the system is far from a CDW instability as being widely discussed for a doping level of x=0.5.Comment: 5 pages, 5 figure

    Macroporous materials: microfluidic fabrication, functionalization and applications

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    This article provides an up-to-date highly comprehensive overview (594 references) on the state of the art of the synthesis and design of macroporous materials using microfluidics and their applications in different fields

    Room-Temperature Ferrimagnet with Frustrated Antiferroelectricity: Promising Candidate Toward Multiple State Memory

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    On the basis of first-principles calculations we show that the M-type hexaferrite BaFe12O19 exhibits frustrated antiferroelectricity associated with its trigonal bipyramidal Fe3+ sites. The ferroelectric (FE) state of BaFe12O19, reachable by applying an external electric field to the antiferroelectric (AFE) state, can be made stable at room temperature by appropriate element substitution or strain engineering. Thus M-type hexaferrite, as a new type of multiferoic with coexistence of antiferroelectricity and ferrimagnetism, provide a basis for studying the phenomenon of frustrated antiferroelectricity and realizing multiple state memory devices.Comment: supporting material available via email. arXiv admin note: text overlap with arXiv:1210.7116 by other author

    Semimetallic molecular hydrogen at pressure above 350 GPa

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    According to the theoretical predictions, insulating molecular hydrogen dissociates and transforms to an atomic metal at pressures P~370-500 GPa. In another scenario, the metallization first occurs in the 250-500 GPa pressure range in molecular hydrogen through overlapping of electronic bands. The calculations are not accurate enough to predict which option is realized. Here we show that at a pressure of ~360 GPa and temperatures <200 K the hydrogen starts to conduct, and that temperature dependence of the electrical conductivity is typical of a semimetal. The conductivity, measured up to 440 GPa, increases strongly with pressure. Raman spectra, measured up to 480 GPa, indicate that hydrogen remains a molecular solid at pressures up to 440 GPa, while at higher pressures the Raman signal vanishes, likely indicating further transformation to a good molecular metal or to an atomic state

    Optical properties of TlNi2Se2: Observation of pseudogap formation

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    The quasi-two-dimensional nickel chalcogenides TlNi2Se2TlNi_2Se_2 is a newly discovered superconductor. We have performed optical spectroscopy study on TlNi2Se2TlNi_2Se_2 single crystals over a broad frequency range at various temperatures. The overall optical reflectance spectra are similar to those observed in its isostructure BaNi2As2BaNi_2As_2. Both the suppression in R(ω)R(\omega) and the peaklike feature in σ1(ω)\sigma_1(\omega) suggest the progressive formation of a pseudogap feature in the midinfrared range with decreasing temperatures, which might be originated from the dynamic local fluctuation of charge-density-wave (CDW) instability. We propose that the CDW instability in TlNi2Se2TlNi_2Se_2 is driven by the saddle points mechanism, due to the existence of van Hove singularity very close to the Fermi energy.Comment: 5 pages, 4 figure

    Environmental Dependence of Cold Dark Matter Halo Formation

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    We use a high-resolution NN-body simulation to study how the formation of cold dark matter (CDM) halos is affected by their environments, and how such environmental effects produce the age-dependence of halo clustering observed in recent NN-body simulations. We estimate, for each halo selected at redshift z=0z=0, an `initial' mass MiM_{\rm i} defined to be the mass enclosed by the largest sphere which contains the initial barycenter of the halo particles and within which the mean linear density is equal to the critical value for spherical collapse at z=0z=0. For halos of a given final mass, MhM_{\rm h}, the ratio Mi/MhM_{\rm i}/M_{\rm h} has large scatter, and the scatter is larger for halos of lower final masses. Halos that form earlier on average have larger Mi/MhM_{\rm i}/M_{\rm h}, and so correspond to higher peaks in the initial density field than their final masses imply. Old halos are more strongly clustered than younger ones of the same mass because their initial masses are larger. The age-dependence of clustering for low-mass halos is entirely due to the difference in the initial/final mass ratio. Low-mass old halos are almost always located in the vicinity of big structures, and their old ages are largely due to the fact that their mass accretions are suppressed by the hot environments produced by the tidal fields of the larger structure. The age-dependence of clustering is weaker for more massive halos because the heating by large-scale tidal fields is less important.Comment: 18 pages,19 figures, accepted by MNRA

    Nonlinear parallel momentum transport in strong turbulence

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    Most existing theoretical studies of momentum transport focus on calculating the Reynolds stress based on quasilinear theory, without considering the \emph{nonlinear} momentum flux-. However, a recent experiment on TORPEX found that the nonlinear toroidal momentum flux induced by blobs makes a significant contribution as compared to the Reynolds stress [Labit et al., Phys. Plasmas {\bf 18}, 032308 (2011)]. In this work, the nonlinear parallel momentum flux in strong turbulence is calculated by using three dimensional Hasegawa-Mima equation. It is shown that nonlinear diffusivity is smaller than quasilinear diffusivity from Reynolds stress. However, the leading order nonlinear residual stress can be comparable to the quasilinear residual stress, and so could be important to intrinsic rotation in tokamak edge plasmas. A key difference from the quasilinear residual stress is that parallel fluctuation spectrum asymmetry is not required for nonlinear residual stress
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