Random projections and the optimization of an algorithm for phase retrieval

Iterative phase retrieval algorithms typically employ projections onto constraint subspaces to recover the unknown phases in the Fourier transform of an image, or, in the case of x-ray crystallography, the electron density of a molecule. For a general class of algorithms, where the basic iteration is specified by the difference map, solutions are associated with fixed points of the map, the attractive character of which determines the effectiveness of the algorithm. The behavior of the difference map near fixed points is controlled by the relative orientation of the tangent spaces of the two constraint subspaces employed by the map. Since the dimensionalities involved are always large in practical applications, it is appropriate to use random matrix theory ideas to analyze the average-case convergence at fixed points. Optimal values of the gamma parameters of the difference map are found which differ somewhat from the values previously obtained on the assumption of orthogonal tangent spaces.Comment: 15 page

Dynamics of immersed molecules in superfluids

The dynamics of a molecule immersed in a superfluid medium are considered. Results are derived using a classical hydrodynamic approach followed by canonical quantization. The classical model, a rigid body immersed in incompressible fluid, permits a thorough analysis; its effective Hamiltonian generalizes the usual rigid-rotor Hamiltonian. In contrast to the free rigid rotor, the immersed body is shown to have chaotic dynamics. Quantization of the classical model leads to new and experimentally verifiable features. It is shown, for instance, that chiral molecules can behave as "quantum propellers": the rotational-translational coupling induced by the superfluid leads to a nonzero linear momentum in the ground state. Hydrogen peroxide is a strong candidate for experimental detection of this effect. The signature is a characteristic splitting of rotational absorption lines. The 1_{01} --> 1_{10} line in hydrogen peroxide, for example, is predicted to split into three lines separated by as much as 0.01 cm^{-1}, which is about the experimental linewidth.Comment: 10 pages, 3 figure

Scattering-free plasmonic optics with anisotropic metamaterials

We develop an approach to utilize anisotropic metamaterials to solve one of the fundamental problems of modern plasmonics -- parasitic scattering of surface waves into free-space modes, opening the road to truly two-dimensional plasmonic optics. We illustrate the developed formalism on examples of plasmonic refractor and plasmonic crystal, and discuss limitations of the developed technique and its possible applications for sensing and imaging structures, high-performance mode couplers, optical cloaking structures, and dynamically reconfigurable electro-plasmonic circuits

A method for dense packing discovery

The problem of packing a system of particles as densely as possible is foundational in the field of discrete geometry and is a powerful model in the material and biological sciences. As packing problems retreat from the reach of solution by analytic constructions, the importance of an efficient numerical method for conducting \textit{de novo} (from-scratch) searches for dense packings becomes crucial. In this paper, we use the \textit{divide and concur} framework to develop a general search method for the solution of periodic constraint problems, and we apply it to the discovery of dense periodic packings. An important feature of the method is the integration of the unit cell parameters with the other packing variables in the definition of the configuration space. The method we present led to improvements in the densest-known tetrahedron packing which are reported in [arXiv:0910.5226]. Here, we use the method to reproduce the densest known lattice sphere packings and the best known lattice kissing arrangements in up to 14 and 11 dimensions respectively (the first such numerical evidence for their optimality in some of these dimensions). For non-spherical particles, we report a new dense packing of regular four-dimensional simplices with density $\phi=128/219\approx0.5845$ and with a similar structure to the densest known tetrahedron packing.Comment: 15 pages, 5 figure

Stability of the hard-sphere icosahedral quasilattice

The stability of the hard-sphere icosahedral quasilattice is analyzed using the differential formulation of the generalized effective liquid approximation. We find that the icosahedral quasilattice is metastable with respect to the hard-sphere crystal structures. Our results agree with recent findings by McCarley and Ashcroft [Phys. Rev. B {\bf 49}, 15600 (1994)] carried out using the modified weighted density approximation.Comment: 15 pages, 2 figures available from authors upon request, (revtex), submitted to Phys. Rev.

Device calibration impacts security of quantum key distribution

Characterizing the physical channel and calibrating the cryptosystem hardware are prerequisites for establishing a quantum channel for quantum key distribution (QKD). Moreover, an inappropriately implemented calibration routine can open a fatal security loophole. We propose and experimentally demonstrate a method to induce a large temporal detector efficiency mismatch in a commercial QKD system by deceiving a channel length calibration routine. We then devise an optimal and realistic strategy using faked states to break the security of the cryptosystem. A fix for this loophole is also suggested.Comment: 4 pages + 1 page of supplementary information. Considerable modification of Eve's attack strategy and QBER minimization technique. All figures have also been improve

Highly Confined Optical Modes in Nanoscale Metal-Dielectric Multilayers

We show that a stack of metal-dielectric nanolayers, in addition to the long- and short-range plasmons, guides also an entire family of modes strongly confined within the multilayer - the bulk plasmon modes. We propose the classification scheme that reflects specific properties of these modes. We report experimental verification of the bulk plasmon modes by measuring modal indices in a structure made of three pairs of silica(29nm)/gold(25nm) layers.Comment: 4 pages, 4 figure

Magnetic Properties of Undoped C60C_{60}

The Heisenberg antiferromagnet, which arises from the large $U$ Hubbard model, is investigated on the $C_{60}$ molecule and other fullerenes. The connectivity of $C_{60}$ leads to an exotic classical ground state with nontrivial topology. We argue that there is no phase transition in the Hubbard model as a function of $U/t$, and thus the large $U$ solution is relevant for the physical case of intermediate coupling. The system undergoes a first order metamagnetic phase transition. We also consider the S=1/2 case using perturbation theory. Experimental tests are suggested.Comment: 12 pages, 3 figures (included

Rules for Computing Symmetry, Density and Stoichiometry in a Quasi-Unit-Cell Model of Quasicrystals

The quasi-unit cell picture describes the atomic structure of quasicrystals in terms of a single, repeating cluster which overlaps neighbors according to specific overlap rules. In this paper, we discuss the precise relationship between a general atomic decoration in the quasi-unit cell picture atomic decorations in the Penrose tiling and in related tiling pictures. Using these relations, we obtain a simple, practical method for determining the density, stoichiometry and symmetry of a quasicrystal based on the atomic decoration of the quasi-unit cell taking proper account of the sharing of atoms between clusters.Comment: 14 pages, 8 figure

Proliferation of anomalous symmetries in colloidal monolayers subjected to quasiperiodic light fields

Quasicrystals provide a fascinating class of materials with intriguing properties. Despite a strong potential for numerous technical applications, the conditions under which quasicrystals form are still poorly understood. Currently, it is not clear why most quasicrystals hold 5- or 10-fold symmetry but no single example with 7 or 9-fold symmetry has ever been observed. Here we report on geometrical constraints which impede the formation of quasicrystals with certain symmetries in a colloidal model system. Experimentally, colloidal quasicrystals are created by subjecting micron-sized particles to two-dimensional quasiperiodic potential landscapes created by n=5 or seven laser beams. Our results clearly demonstrate that quasicrystalline order is much easier established for n = 5 compared to n = 7. With increasing laser intensity we observe that the colloids first adopt quasiperiodic order at local areas which then laterally grow until an extended quasicrystalline layer forms. As nucleation sites where quasiperiodicity originates, we identify highly symmetric motifs in the laser pattern. We find that their density strongly varies with n and surprisingly is smallest exactly for those quasicrystalline symmetries which have never been observed in atomic systems. Since such high symmetry motifs also exist in atomic quasicrystals where they act as preferential adsorption sites, this suggests that it is indeed the deficiency of such motifs which accounts for the absence of materials with e.g. 7-fold symmetry