Light generation via quantum interaction of electrons with periodic nanostructures

The Smith-Purcell effect is a hallmark of light-matter interactions in periodic structures, resulting in light emission with distinct spectral and angular distribution. We find yet undiscovered effects in Smith-Purcell radiation that arise due to the quantum nature of light and matter, through an approach based on exact energy and momentum conservation. The effects include emission cutoff, convergence of emission orders, and a possible second photoemission process, appearing predominantly in structures with nanoscale periodicities (a few tens of nanometers or less), accessible by recent nanofabrication advances. We further present ways to manipulate the effects by varying the geometry or by accounting for a refractive index. Our derivation emphasizes the fundamental relation between Smith-Purcell radiation and Čerenkov radiation, and paves the way to alternative kinds of light sources wherein nonrelativistic electrons create Smith-Purcell radiation in nanoscale, on-chip devices. Finally, the path towards experimental realizations of these effects is discussed

Inverse design of broadband, strongly-coupled plexcitonic nonlinear metasurfaces

Hybrid photonic structures of plasmonic metasurfaces coupled to atomically thin semiconductors have emerged as a versatile platform for strong light-matter interaction, supporting both strong coupling and parametric nonlinearities. However, designing optimized nonlinear hybrid metasurfaces is a complex task, as the multiple parameters' contribution to the nonlinear response is elusive. Here we present a simple yet powerful strategy for maximizing the nonlinear response of the hybrid structures based on evolutionary inverse design of the metasurface's near-field enhancement around the excitonic frequency. We show that the strong coupling greatly enhances the nonlinear signal, and that its magnitude is mainly determined by the Rabi splitting, making it robust to geometrical variations of the metasurface. Furthermore, the large Rabi splitting attained by these hybrid structures enables broadband operation over the frequencies of the hybridized modes. Our results constitute a significant step towards achieving flexible nonlinear control, which can benefit applications in nonlinear frequency conversion, all-optical switching, and phase-controlled nonlinear metasurfaces

Finite element simulation of a perturbed axial-symmetric whispering-gallery mode and its use for intensity enhancement with a nanoparticle coupled to a microtoroid

We present an optical mode solver for a whispering gallery resonator coupled to an adjacent arbitrary shaped nano-particle that breaks the axial symmetry of the resonator. Such a hybrid resonator-nanoparticle is similar to what was recently used for bio-detection and for field enhancement. We demonstrate our solver by parametrically studying a toroid-nanoplasmonic device and get the optimal nano-plasmonic size for maximal enhancement. We investigate cases near a plasmonic resonance as well as far from a plasmonic resonance. Unlike common plasmons that typically benefit from working near their resonance, here working far from plasmonic resonance provides comparable performance. This is because the plasmonic resonance enhancement is accompanied by cavity quality degradation through plasmonic absorption.Comment: Supplementary COMSOL script, see http://www.quantumchaos.de/Media/comsol2013/Supplement_Script_for_Fig.3_Comsol_4.3a.mp

Incoherent white-light solitons in nonlinear periodic lattices

We predict the existence of lattice solitons made of incoherent white light: lattice solitons made of light originating from an ordinary incandescent light bulb. We find that the intensity structure and spatial power spectra associated with different temporal frequency constituents of incoherent white-light lattice solitons (IWLLSs) arrange themselves in a characteristic fashion, with the intensity structure more localized at higher frequencies, and the spatial power spectrum more localized at lower frequencies; the spatial correlation distance is larger at lower frequency constituents of IWLLSs. This characteristic shape of incoherent white-light lattice solitons reflects the fact that diffraction is stronger for lower temporal frequency constituents, while higher frequencies experience stronger effective nonlinearity and deeper lattice structure

Observation of 2nd band vortex solitons in 2D photonic lattices

We demonstrate second-band bright vortex-array solitons in photonic lattices. This constitutes the first experimental observation of higher-band solitons in any 2D periodic system. These solitons possess complex intensity and phase structures, yet they can be excited by a simple highly-localized vortex-ring beam. Finally, we show that the linear diffraction of such beams exhibits preferential transport along the lattice axes