94 research outputs found
Problems of atomic reactor-lasers
The preliminary directions to be pursued in correcting and implementing basic atomic reactor-laser concepts are outlined. The basic measures to be followed in implementing such systems are discussed
Thermalization of coupled atom-light states in the presence of optical collisions
The interaction of a two-level atomic ensemble with a quantized single mode
electromagnetic field in the presence of optical collisions (OC) is
investigated both theoretically and experimentally. The main accent is made on
achieving thermal equilibrium for coupled atom-light states (in particular
dressed states). We propose a model of atomic dressed state thermalization that
accounts for the evolution of the pseudo-spin Bloch vector components and
characterize the essential role of the spontaneous emission rate in the
thermalization process. Our model shows that the time of thermalization of the
coupled atom-light states strictly depends on the ratio of the detuning and the
resonant Rabi frequency. The predicted time of thermalization is in the
nanosecond domain and about ten times shorter than the natural lifetime at full
optical power in our experiment. Experimentally we are investigating the
interaction of the optical field with rubidium atoms in an ultra-high pressure
buffer gas cell under the condition of large atom-field detuning comparable to
the thermal energy in frequency units. In particular, an observed detuning
dependence of the saturated lineshape is interpreted as evidence for thermal
equilibrium of coupled atom-light states. A significant modification of
sideband intensity weights is predicted and obtained in this case as well.Comment: 14 pages, 12 figures; the content was edite
Laser assisted charge transfer reactions in slow ionâatom collisions: Coupled dressed quasimolecularâstates approach
This is the published version, also available here: http://dx.doi.org/10.1063/1.447712.Semiclassical coupled dressed quasimolecular states (DQMS) approaches are presented for the nonperturbative treatment of charge transferreactions at low collision velocities and high laser intensities. The DQMS are first obtained via the Floquet theory. The laser assisted collision process can then be treated as the electronic transitions among the DQMS driven by the nuclear motion only. The expansion of the total electronic wave function in a truncated DQMS basis results in a set of coupled a d i a b a t i c equations. The adiabatic DQMS and their associated quasienergies (depending parametrically upon the internuclear separation R) exhibit regions of avoided crossings, where the electronic transition probabilities are large due to strong radial couplings induced by the nuclear movement. By further transforming the a d i a b a t i c DQMS into an appropriate d i a b a t i c DQMS representation, defined via the vanishing of the aforementioned radial couplings, we obtain a new set of coupled d i a b a t i c equations which offer computational advantage. The method is illustrated by a case study of the laser assisted charge exchange process He+ ++H(1s)+âÏâHe+(n=2)+H+, in a twoâstate approximation, for the velocity range from 1.5Ă105 to 2Ă107 cm/s and for the laser intensity in the range of 0.4 to 4.0 TW/cm2. Results of exact coupled diabatic DQMS calculations are presented along with several approximation calculations, using first order perturbation theory, the Magnus approximation, and the average cross section
On the Indirect Detection of Sodium in the Atmosphere of the Planetary Companion to HD 209458
Using a self-consistent atmosphere code, we construct a new model of the
atmosphere of the transiting extrasolar giant planet HD 209458b to investigate
the disparity between the observed strength of the sodium absorption feature at
589 nm and the predictions of previous models. For the atmospheric
temperature-pressure profile we derive, silicate and iron clouds reside at a
pressure of several mbar in the planet's atmosphere. These clouds have
significant vertical extent and optical depth due to our slant viewing geometry
and lead to increased absorption in bands directly adjacent to the sodium line
core. Using a non-LTE sodium ionization model that includes photoionization by
stellar UV flux, collisional processes with H_2, and radiative recombination,
we show that the ionization depth in the planet's atmosphere reaches ~1/2 mbar
at the day/night terminator. Ionization leads to a slight weakening of the
sodium feature. We present our baseline model, including ionization and clouds,
which falls near the observational error bars. The sensitivity of our
conclusions to the derived atmospheric temperature-pressure profile is
discussed.Comment: 15 pages, 9 figures -- Accepted to The Astrophysical Journal -- The
paper is significantly revised and expande
The influence of coordinative tartrate and malatogermanate compounds on the activity of α-L-rhamnosidase preparations from Penicillium tardum, Eupenicillium erubescens and Cryptococcus albidus
Recently enzyme preparations of microbial origin become increasingly important in different industries. Preparations of α-L-rhamnosidase are used in the pharmaceutical industry as well as in scientific work as a tool for analytical research. We have obtained purified α-L-rhamnosidase preparations from Penicillium tardum, Eupenicillium erubescens and Cryptococcus albidus microorganism strains which are effective enzyme producers. The aim of the study was to estimate the ability of germanium coordination compounds to enhance enzyme catalytic activity. The effects of 11 heterometal mixed ligand tartrate (malate-)germanate compounds at 0.01 and 0.1% concentration on the activity of α-L-rhamnosidase preparations from Penicillium tardum IMV F-100074, Eupenicillium erubescens and Cryptococcus albidus 1001 were studied at 0.5 and 24 h exposition. The inhibitory effect of [Ni(bipy)3]4[{Ge2(OH)2(Tart)2}3Cl2]·15H2 on P. tardum α-L-rhamnosidase was revealed. All studied compounds except [CuCl(phen)2][Ge(OH)(HMal)2] were shown to increase activity of P. tardum α-L-rhamnosidase at a longer term of exposition. Activity of E. erubescens α-L-rhamnosidase was shown to be stimulated by d-metal cation-free compounds. C. albidus α-L-rhamnosidase occurred to be insensitive to all compounds studied
UV continuum emission and diagnostics of hydrogen-containing non-equilibrium plasmas
For the first time the emission of the radiative dissociation continuum of
the hydrogen molecule ( electronic
transition) is proposed to be used as a source of information for the
spectroscopic diagnostics of non-equilibrium plasmas. The detailed analysis of
excitation-deactivation kinetics, rate constants of various collisional and
radiative transitions and fitting procedures made it possible to develop two
new methods of diagnostics of: (1) the ground state
vibrational temperature from the relative intensity
distribution, and (2) the rate of electron impact dissociation
(d[\mbox{H_{2}}]/dt)_{\text{diss}} from the absolute intensity of the
continuum. A known method of determination of from relative
intensities of Fulcher- bands was seriously corrected and simplified
due to the revision of transition probabilities and cross sections of
electron impact excitation. General considerations are illustrated
with examples of experiments in pure hydrogen capillary-arc and H+Ar
microwave discharges.Comment: REVTeX, 25 pages + 12 figures + 9 tables. Phys. Rev. E, eprint
replaced because of resubmission to journal after referee's 2nd repor
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