Electrically Driven Light Emission from Individual CdSe Nanowires

We report electroluminescence (EL) measurements carried out on three-terminal devices incorporating individual n-type CdSe nanowires. Simultaneous optical and electrical measurements reveal that EL occurs near the contact between the nanowire and a positively biased electrode or drain. The surface potential profile, obtained by using Kelvin probe microscopy, shows an abrupt potential drop near the position of the EL spot, while the band profile obtained from scanning photocurrent microscopy indicates the existence of an n-type Schottky barrier at the interface. These observations indicate that light emission occurs through a hole leakage or an inelastic scattering induced by the rapid potential drop at the nanowire-electrode interface.Comment: 12 pages, 4 figure

Growth and Transport Properties of Complementary Germanium Nanowire Field Effect Transistors

n- and p-type Ge nanowires were synthesized by a multistep process in which axial elongation, via vapor–liquid–solid (VLS) growth, and doping were accomplished in separate chemical vapor deposition steps. Intrinsic, single-crystal, Ge nanowires prepared by Au nanocluster-mediated VLS growth were surface-doped in situ using diborane or phosphine, and then radial growth of an epitaxial Ge shell was used to cap the dopant layer. Field-effect transistors prepared from these Ge nanowires exhibited on currents and transconductances up to 850 µA/µm and 4.9 µA/V, respectively, with device yields of \u3e85%

An Ab Initio Approach to the Solar Coronal Heating Problem

We present an ab initio approach to the solar coronal heating problem by modelling a small part of the solar corona in a computational box using a 3D MHD code including realistic physics. The observed solar granular velocity pattern and its amplitude and vorticity power spectra, as reproduced by a weighted Voronoi tessellation method, are used as a boundary condition that generates a Poynting flux in the presence of a magnetic field. The initial magnetic field is a potential extrapolation of a SOHO/MDI high resolution magnetogram, and a standard stratified atmosphere is used as a thermal initial condition. Except for the chromospheric temperature structure, which is kept fixed, the initial conditions are quickly forgotten because the included Spitzer conductivity and radiative cooling function have typical timescales much shorter than the time span of the simulation. After a short initial start up period, the magnetic field is able to dissipate 3-4 10^6 ergs cm^{-2} s^{-1} in a highly intermittent corona, maintaining an average temperature of $\sim 10^6$ K, at coronal density values for which emulated images of the Transition Region And Coronal Explorer(TRACE) 171 and 195 pass bands reproduce observed photon count rates.Comment: 12 pages, 14 figures. Submitted to Ap

Temperature dependent fluorescence in disordered Frenkel chains: interplay of equilibration and local band-edge level structure

We model the optical dynamics in linear Frenkel exciton systems governed by scattering on static disorder and lattice vibrations, and calculate the temperature dependent fluorescence spectrum and lifetime. The fluorescence Stokes shift shows a nonmonotonic behavior with temperature, which derives from the interplay of the local band-edge level structure and thermal equilibration. The model yields excellent fits to experiments performed on linear dye aggregates.Comment: 4 pages, 3 figure

Many-Body Effects on Tunneling of Electrons in Magnetic-Field-Induced Quasi One-Dimensional Electron Systems in Semiconductor Nanowhiskers

Effects of the electron-electron interaction on tunneling in a semiconductor nanowhisker are studied in a magnetic quantum limit. We consider the system with which bulk and edge states coexist. In bulk states, the temperature dependence of the transmission probability is qualitatively similar to that of a one-dimensional electron system. We investigate contributions of edge states on transmission probability in bulk states. Those contributions can be neglected within our approximation which takes into account only most divergent terms at low temperatures.Comment: 9 pages, 6 figure

Heat conduction in a 1D harmonic chain with three dimensional vibrations

We study vibrational energy transport in a quasi 1-D harmonic chain with both longitudinal and transverse vibrations. We demonstrate via both numerical simulation and theoretic analysis that for 1-D atomic chain connected by 3D harmonic springs, the coefficient of heat conduction changes it continuously with its lattice constant, indicating the qualitative difference from the corresponding 1-D case where the coefficient is independent of the lattice constant.Comment: 4 pages, 4 figure

Atomistic simulations of self-trapped exciton formation in silicon nanostructures: The transition from quantum dots to nanowires

Using an approximate time-dependent density functional theory method, we calculate the absorption and luminescence spectra for hydrogen passivated silicon nanoscale structures with large aspect ratio. The effect of electron confinement in axial and radial directions is systematically investigated. Excited state relaxation leads to significant Stokes shifts for short nanorods with lengths less than 2 nm, but has little effect on the luminescence intensity. The formation of self-trapped excitons is likewise observed for short nanostructures only; longer wires exhibit fully delocalized excitons with neglible geometrical distortion at the excited state minimum.Comment: 10 pages, 4 figure

Profiles of heating in turbulent coronal magnetic loops

Context: The location of coronal heating in magnetic loops has been the subject of a long-lasting controversy: does it occur mostly at the loop footpoints, at the top, is it random, or is the average profile uniform? Aims: We try to address this question in model loops with MHD turbulence and a profile of density and/or magnetic field along the loop. Methods: We use the ShellAtm MHD turbulent heating model described in Buchlin & Velli (2006), with a static mass density stratification obtained by the HydRad model (Bradshaw & Mason 2003). This assumes the absence of any flow or heat conduction subsequent to the dynamic heating. Results: The average profile of heating is quasi-uniform, unless there is an expansion of the flux tube (non-uniform axial magnetic field) or the variation of the kinetic and magnetic diffusion coefficients with temperature is taken into account: in the first case the heating is enhanced at footpoints, whereas in the second case it is enhanced where the dominant diffusion coefficient is enhanced. Conclusions: These simulations shed light on the consequences on heating profiles of the complex interactions between physical effects involved in a non-uniform turbulent coronal loop.Comment: 9 pages, 8 figure

Structure of nanoparticles embedded in micellar polycrystals

We investigate by scattering techniques the structure of water-based soft composite materials comprising a crystal made of Pluronic block-copolymer micelles arranged in a face-centered cubic lattice and a small amount (at most 2% by volume) of silica nanoparticles, of size comparable to that of the micelles. The copolymer is thermosensitive: it is hydrophilic and fully dissolved in water at low temperature (T ~ 0{\deg}C), and self-assembles into micelles at room temperature, where the block-copolymer is amphiphilic. We use contrast matching small-angle neuron scattering experiments to probe independently the structure of the nanoparticles and that of the polymer. We find that the nanoparticles do not perturb the crystalline order. In addition, a structure peak is measured for the silica nanoparticles dispersed in the polycrystalline samples. This implies that the samples are spatially heterogeneous and comprise, without macroscopic phase separation, silica-poor and silica-rich regions. We show that the nanoparticle concentration in the silica-rich regions is about tenfold the average concentration. These regions are grain boundaries between crystallites, where nanoparticles concentrate, as shown by static light scattering and by light microscopy imaging of the samples. We show that the temperature rate at which the sample is prepared strongly influence the segregation of the nanoparticles in the grain-boundaries.Comment: accepted for publication in Langmui