304 research outputs found
Tension dynamics and viscoelasticity of extensible wormlike chains
The dynamic response of prestressed semiflexible biopolymers is characterized
by the propagation and relaxation of tension, which arises due to the near
inextensibility of a stiff backbone. It is coupled to the dynamics of contour
length stored in thermal undulations, but also to the local relaxation of
elongational strain. We present a systematic theory of tension dynamics for
stiff yet extensible wormlike chains. Our results show that even moderate
prestress gives rise to distinct Rouse-like extensibility signatures in the
high-frequency viscoelastic response.Comment: 4 pages, 1 figure; corrected typo
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Relaxation Dynamics of Semiflexible Polymers
We study the relaxation dynamics of a semiflexible chain by introducing a time-dependent tension. The chain has one of its ends attached to a large bead, and the other end is fixed. We focus on the initial relaxation of the chain that is initially strongly stretched. Using a tension that is self-consistently determined, we obtain the evolution of the end-to-end distance with no free parameters. Our results are in good agreement with single molecule experiments on double stranded DNA
Generalized model for dynamic percolation
We study the dynamics of a carrier, which performs a biased motion under the
influence of an external field E, in an environment which is modeled by dynamic
percolation and created by hard-core particles. The particles move randomly on
a simple cubic lattice, constrained by hard-core exclusion, and they
spontaneously annihilate and re-appear at some prescribed rates. Using
decoupling of the third-order correlation functions into the product of the
pairwise carrier-particle correlations we determine the density profiles of the
"environment" particles, as seen from the stationary moving carrier, and
calculate its terminal velocity, V_c, as the function of the applied field and
other system parameters. We find that for sufficiently small driving forces the
force exerted on the carrier by the "environment" particles shows a
viscous-like behavior. An analog Stokes formula for such dynamic percolative
environments and the corresponding friction coefficient are derived. We show
that the density profile of the environment particles is strongly
inhomogeneous: In front of the stationary moving carrier the density is higher
than the average density, , and approaches the average value as an
exponential function of the distance from the carrier. Past the carrier the
local density is lower than and the relaxation towards may
proceed differently depending on whether the particles number is or is not
explicitly conserved.Comment: Latex, 32 pages, 4 ps-figures, submitted to PR
Diffusion with rearranging traps
A model for diffusion on a cubic lattice with a random distribution of traps
is developed. The traps are redistributed at certain time intervals. Such
models are useful for describing systems showing dynamic disorder, such as
ion-conducting polymers. In the present model the traps are infinite, unlike an
earlier version with finite traps, this model has a percolation threshold. For
the infinite trap version a simple analytical calculation is possible and the
results agree qualitatively with simulation.Comment: Latex, five figure
Random Walks on a Fluctuating Lattice: A Renormalization Group Approach Applied in One Dimension
We study the problem of a random walk on a lattice in which bonds connecting
nearest neighbor sites open and close randomly in time, a situation often
encountered in fluctuating media. We present a simple renormalization group
technique to solve for the effective diffusive behavior at long times. For
one-dimensional lattices we obtain better quantitative agreement with
simulation data than earlier effective medium results. Our technique works in
principle in any dimension, although the amount of computation required rises
with dimensionality of the lattice.Comment: PostScript file including 2 figures, total 15 pages, 8 other figures
obtainable by mail from D.L. Stei
Anomalous fluctuations of active polar filaments
Using a simple model, we study the fluctuating dynamics of inextensible,
semiflexible polar filaments interacting with active and directed force
generating centres such as molecular motors. Taking into account the fact that
the activity occurs on time-scales comparable to the filament relaxation time,
we obtain some unexpected differences between both the steady-state and
dynamical behaviour of active as compared to passive filaments. For the
statics, the filaments have a {novel} length-scale dependent rigidity.
Dynamically, we find strongly enhanced anomalous diffusion.Comment: 5 pages, 3 figure
Pearling and Pinching: Propagation of Rayleigh Instabilities
A new category of front propagation problems is proposed in which a spreading
instability evolves through a singular configuration before saturating. We
examine the nature of this front for the viscous Rayleigh instability of a
column of one fluid immersed in another, using the marginal stability criterion
to estimate the front velocity, front width, and the selected wavelength in
terms of the surface tension and viscosity contrast. Experiments are suggested
on systems that may display this phenomenon, including droplets elongated in
extensional flows, capillary bridges, liquid crystal tethers, and viscoelastic
fluids. The related problem of propagation in Rayleigh-like systems that do not
fission is also considered.Comment: Revtex, 7 pages, 4 ps figs, PR
Ultra-Slow Vacancy-Mediated Tracer Diffusion in Two Dimensions: The Einstein Relation Verified
We study the dynamics of a charged tracer particle (TP) on a two-dimensional
lattice all sites of which except one (a vacancy) are filled with identical
neutral, hard-core particles. The particles move randomly by exchanging their
positions with the vacancy, subject to the hard-core exclusion. In case when
the charged TP experiences a bias due to external electric field ,
(which favors its jumps in the preferential direction), we determine exactly
the limiting probability distribution of the TP position in terms of
appropriate scaling variables and the leading large-N ( being the discrete
time) behavior of the TP mean displacement ; the latter is
shown to obey an anomalous, logarithmic law . On comparing our results with earlier predictions by Brummelhuis
and Hilhorst (J. Stat. Phys. {\bf 53}, 249 (1988)) for the TP diffusivity
in the unbiased case, we infer that the Einstein relation
between the TP diffusivity and the mobility holds in the leading in order, despite
the fact that both and are not constant but vanish as . We also generalize our approach to the situation with very small but
finite vacancy concentration , in which case we find a ballistic-type law
. We demonstrate that here,
again, both and , calculated in the linear in
approximation, do obey the Einstein relation.Comment: 25 pages, one figure, TeX, submitted to J. Stat. Phy
Dynamics of viscoelastic membranes
We determine both the in-plane and out-of-plane dynamics of viscoelastic
membranes separating two viscous fluids in order to understand microrheological
studies of such membranes. We demonstrate the general viscoelastic signatures
in the dynamics of shear, bending, and compression modes. We also find a
screening of the otherwise two-dimensional character of the response to point
forces due to the presence of solvent. Finally, we show that there is a linear,
hydrodynamic coupling between the in-plane compression modes of the membrane
and the out-of-plane bending modes in the case where the membrane separates two
different fluids or environments
Intracellular microrheology of motile Amoeba proteus
The motility of motile Amoeba proteus was examined using the technique of
passive particle tracking microrheology, with the aid of newly-developed
particle tracking software, a fast digital camera and an optical microscope. We
tracked large numbers of endogeneous particles in the amoebae, which displayed
subdiffusive motion at short time scales, corresponding to thermal motion in a
viscoelastic medium, and superdiffusive motion at long time scales due to the
convection of the cytoplasm. Subdiffusive motion was characterised by a
rheological scaling exponent of 3/4 in the cortex, indicative of the
semiflexible dynamics of the actin fibres. We observed shear-thinning in the
flowing endoplasm, where exponents increased with increasing flow rate; i.e.
the endoplasm became more fluid-like. The rheology of the cortex is found to be
isotropic, reflecting an isotropic actin gel. A clear difference was seen
between cortical and endoplasmic layers in terms of both viscoelasticity and
flow velocity, where the profile of the latter is close to a Poiseuille flow
for a Newtonian fluid
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