334 research outputs found
Semiconducting-to-metallic photoconductivity crossover and temperature-dependent Drude weight in graphene
We investigated the transient photoconductivity of graphene at various
gate-tuned carrier densities by optical-pump terahertz-probe spectroscopy. We
demonstrated that graphene exhibits semiconducting positive photoconductivity
near zero carrier density, which crosses over to metallic negative
photoconductivity at high carrier density. Our observations are accounted for
by considering the interplay between photo-induced changes of both the Drude
weight and the carrier scattering rate. Notably, we observed multiple sign
changes in the temporal photoconductivity dynamics at low carrier density. This
behavior reflects the non-monotonic temperature dependence of the Drude weight,
a unique property of massless Dirac fermions
Observation of spin Coulomb drag in a two-dimensional electron gas
An electron propagating through a solid carries spin angular momentum in
addition to its mass and charge. Of late there has been considerable interest
in developing electronic devices based on the transport of spin, which offer
potential advantages in dissipation, size, and speed over charge-based devices.
However, these advantages bring with them additional complexity. Because each
electron carries a single, fixed value (-e) of charge, the electrical current
carried by a gas of electrons is simply proportional to its total momentum. A
fundamental consequence is that the charge current is not affected by
interactions that conserve total momentum, notably collisions among the
electrons themselves. In contrast, the electron's spin along a given spatial
direction can take on two values, "up" and "down", so that the spin current and
momentum need not be proportional. Although the transport of spin polarization
is not protected by momentum conservation, it has been widely assumed that,
like the charge current, spin current is unaffected by electron-electron (e-e)
interactions. Here we demonstrate experimentally not only that this assumption
is invalid, but that over a broad range of temperature and electron density,
the flow of spin polarization in a two-dimensional gas of electrons is
controlled by the rate of e-e collisions
Tracking Cooper Pairs in a Cuprate Superconductor by Ultrafast Angle-Resolved Photoemission
In high-temperature superconductivity, the process that leads to the
formation of Cooper pairs, the fundamental charge carriers in any
superconductor, remains mysterious. We use a femtosecond laser pump pulse to
perturb superconducting Bi2Sr2CaCu2O8+{\delta}, and study subsequent dynamics
using time- and angle-resolved photoemission and infrared reflectivity probes.
Gap and quasiparticle population dynamics reveal marked dependencies on both
excitation density and crystal momentum. Close to the d-wave nodes, the
superconducting gap is sensitive to the pump intensity and Cooper pairs
recombine slowly. Far from the nodes pumping affects the gap only weakly and
recombination processes are faster. These results demonstrate a new window into
the dynamical processes that govern quasiparticle recombination and gap
formation in cuprates.Comment: 22 pages, 9 figure
Nodal quasiparticle meltdown in ultra-high resolution pump-probe angle-resolved photoemission
High- cuprate superconductors are characterized by a strong
momentum-dependent anisotropy between the low energy excitations along the
Brillouin zone diagonal (nodal direction) and those along the Brillouin zone
face (antinodal direction). Most obvious is the d-wave superconducting gap,
with the largest magnitude found in the antinodal direction and no gap in the
nodal direction. Additionally, while antinodal quasiparticle excitations appear
only below , superconductivity is thought to be indifferent to nodal
excitations as they are regarded robust and insensitive to . Here we
reveal an unexpected tie between nodal quasiparticles and superconductivity
using high resolution time- and angle-resolved photoemission on optimally doped
BiSrCaCuO. We observe a suppression of the nodal
quasiparticle spectral weight following pump laser excitation and measure its
recovery dynamics. This suppression is dramatically enhanced in the
superconducting state. These results reduce the nodal-antinodal dichotomy and
challenge the conventional view of nodal excitation neutrality in
superconductivity.Comment: 7 pages, 3 figure. To be published in Nature Physic
Observation of suppressed terahertz absorption in photoexcited graphene
When light is absorbed by a semiconductor, photoexcited charge carriers enhance the absorption of far-infrared radiation due to intraband transitions. We observe the opposite behavior in monolayer graphene, a zero-gap semiconductor with linear dispersion. By using time domain terahertz (THz) spectroscopy in conjunction with optical pump excitation, we observe a reduced absorption of THz radiation in photoexcited graphene. The measured spectral shape of the differential optical conductivity exhibits non-Drude behavior. We discuss several possible mechanisms that contribute to the observed low-frequency non-equilibrium optical response of graphene.United States. Dept. of Energy. Office of Basic Energy Sciences (Grant DE-SC0006423)National Science Foundation (U.S.). Graduate Research Fellowship ProgramUnited States. Air Force Office of Scientific ResearchUnited States. Office of Naval Research. Multidisciplinary University Research Initiative. Graphene Approaches to Terahertz ElectronicsNational Science Foundation (U.S.) (Award DMR-0819762)National Science Foundation (U.S.) (Grant ECS-0335765
- …