109 research outputs found
Spin-wave spectrum of copper metaborate in the commensurate phase 10K<T<21K
We have investigated the spin-wave spectrum of copper metaborate,
CuBO, by means of inelastic neutron scattering in the commensurate
magnetic phase. We have found two branches of spin-wave excitations associated
with the two magnetic sublattices Cu(A) and Cu(B), respectively. In the
temperature regime , where only the Cu(A) magnetic moments
are ordered, the interaction between the two sublattices is found to be
negligible. With this approximation we have determined the `easy plane'
exchange parameters of the Cu(A) subsystem within standard spin-wave theory.Comment: 4 figure
Spin–glass magnetism in RFeTi2O7 (R=Lu and Tb) compounds
20th International Conference on Magnetism.The compounds RFeTi2O7 (R=Lu and Tb) crystallize at room temperature in centrosymmetric orthorhombic space group Pcnb. There are five non-equivalent positions of the iron ions: the two positions, Fe’ and Fe”, in the octahedron consisting of the Fe’ tetrahedron and Fe” five-vertex polyhedron and the three positions, Fe1, Fe2 and Fe3 in the mixed Fe-Ti octahedra [1]. The populations of the mixed Fe-Ti sites are different. The crystal structure features lead to atomic disorder in the distribution of the magnetic ions in this compound. From low temperature heat capacity, magnetization and frequency dependent ac susceptibility we conclude that both compounds undergo a spin glass transition at TSG=4.5 and 6 K for R =Lu and Tb, respectively. Since Lu is not magnetic, in RFeTi2O7 the spin glass behavior is caused by the disordered distribution of the magnetic Fe3+ ions in the different crystallographic positions. The substitution of the magnetic and highly anisotropic Tb ion instead of Lu increases TSG because of the additional Tb-Fe exchange interaction, while the critical exponent of the frequency dependence on temperature hardly varies. The spin glass behavior in these crystalline compounds is caused by the presence of competitive interactions that lead to frustration.The financial support of the Spanish MINECO MAT2011-23791, MAT2014-53921-R and Aragonese DGA-IMANA E34 projects is acknowledged.Peer Reviewe
A single chain analysis of doped quasi one dimensional spin 1 compounds: paramagnetic versus spin 1/2 doping
We present a numerical study of single chain models of doped spin 1
compounds. We use low energy effective one-dimensional models for both the
cases of paramagnetic and spin-1/2 doping. In the case of paramagnetic doping,
the effective model is equivalent to the bond disordered spin-1/2 chain model
recently analyzed by means of real space renormalization group by Hyman and
Yang. By means of exact diagonalizations in the XX limit, we confirm the
stability of the Haldane phase for weak disorder. Above a critical amount of
disorder, the effective model flows to the so called random singlet fixed
point. In the case of spin-1/2 doping, we argue that the Haldane phase should
be destabilized even for weak disorder. This picture is not in contradiction
with existing experimental data. We also discuss the possible occurrence of
(unobserved) antiferromagnetically ordered phases.Comment: 13 pages, 7 included figure
Spin dynamics in copper metaborate studied by muon spin relaxation
Copper metaborate CuBO was studied by muon spin relaxation
measurements in order to clarify its static and dynamic magnetic properties.
The time spectra of muon spin depolarization suggest that the local fields at
the muon site contain both static and fluctuating components in all ordered
phases down to 0.3 K. In the weak ferromagnetic phase (20 K~~9.3 K), the
static component is dominant. On the other hand, upon cooling the fluctuating
component becomes dominant in the incommensurate helix phase (9.3K > T > 1.4K).
The dynamical fluctuations of the local fields persist down to 0.3K, where a
new incommensurate phase (T < 1.4K) is expected to appear. This result suggests
that spins fluctuate even at T \to 0. We propose two possible origins of the
remnant dynamical spin fluctuations: frustration of the exchange interactions
and the dynamic behavior of the soliton lattice
Conductivity, weak ferromagnetism and charge instability in single crystal
The temperature dependence of resistivity, magnetization and electron-spin
resonance of the single crystal were measured in temperature
range of . Magnetization hysteresis in applied magnetic field
up to 0.7 T at , irreversible temperature behavior of
magnetization and resistivity were found . The obtained data were explained in
terms of degenerate tight binding model using random phase approximation. The
contribution of holes in and bands of manganese ions to the
conductivity, optical absorbtion spectra and charge instability in were studied. Charge susceptibility maxima resulted from the competition of
the on-site Coulomb interaction between the holes in different orbitals and
small hybridization of sub-bands were calculated at .Comment: 6 pages, 12 figure
Resonant inelastic x-ray scattering in electronically quasi-zero-dimensional CuB2O4
We explore the general phenomenology of resonant inelastic scattering (RIXS)
using CuB2O4, a network of CuO4 plaquettes electronically isolated by B+3 ions.
Spectra show a small number of well-separated features, and we exploit the
simple electronic structure to explore RIXS phenomenology by developing a
calculation which allows for intermediate-state effects ignored in standard
approaches. These effects are found to be non-negligible and good
correspondence between our model and experiment leads to a simple picture of
such phenomenology as the genesis of d-d excitations at the K edge and
intermediate-state interference effects.Comment: Phys. Rev. B 80, 092509 (2009
Spin-Glass State in
Magnetic susceptibility, magnetization, specific heat and positive muon spin
relaxation (\musr) measurements have been used to characterize the magnetic
ground-state of the spinel compound . We observe a spin-glass
transition of the S=1/2 spins below characterized
by a cusp in the susceptibility curve which suppressed when a magnetic field is
applied. We show that the magnetization of depends on the
magnetic histo Well below , the muon signal resembles the dynamical
Kubo-Toyabe expression reflecting that the spin freezing process in results Gaussian distribution of the magnetic moments. By means of
Monte-Carlo simulati we obtain the relevant exchange integrals between the spins in this compound.Comment: 6 pages, 16 figure
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