Precision spectral manipulation of optical pulses using a coherent photon echo memory

Photon echo schemes are excellent candidates for high efficiency coherent optical memory. They are capable of high-bandwidth multi-pulse storage, pulse resequencing and have been shown theoretically to be compatible with quantum information applications. One particular photon echo scheme is the gradient echo memory (GEM). In this system, an atomic frequency gradient is induced in the direction of light propagation leading to a Fourier decomposition of the optical spectrum along the length of the storage medium. This Fourier encoding allows precision spectral manipulation of the stored light. In this letter, we show frequency shifting, spectral compression, spectral splitting, and fine dispersion control of optical pulses using GEM

QED with a spherical mirror

We investigate the Quantum-Electro-Dynamic properties of an atomic electron close to the focus of a spherical mirror. We first show that the spontaneous emission and excited state level shift of the atom can be fully suppressed with mirror-atom distances of many wavelengths. A three-dimensional theory predicts that the spectral density of vacuum fluctuations can indeed vanish within a volume $\lambda^3$ around the atom, with the use of a far distant mirror covering only half of the atomic emission solid angle. The modification of these QED atomic properties is also computed as a function of the mirror size and large effects are found for only moderate numerical apertures. We also evaluate the long distance ground state energy shift (Casimir-Polder shift) and find that it scales as $(\lambda/R)^2$ at the focus of a hemi-spherical mirror of radius $R$, as opposed to the well known $(\lambda/R)^4$ scaling law for an atom at a distance $R$ from an infinite plane mirror. Our results are relevant for investigations of QED effects, and also free space coupling to single atoms using high-numerical aperture lenses.Comment: 12 pages, 4 figure

Electromagnetically Induced Transparency from a Single Atom in Free Space

We report an absorption spectroscopy experiment and the observation of electromagnetically induced transparency from a single trapped atom. We focus a weak and narrowband Gaussian light beam onto an optically cooled Barium ion using a high numerical aperture lens. Extinction of this beam is observed with measured values of up to 1.3 %. We demonstrate electromagnetically induced transparency of the ion by tuning a strong control beam over a two-photon resonance in a three-level lambda-type system. The probe beam extinction is inhibited by more than 75 % due to population trapping.Comment: 4 pages, 3 figure

Coherent population trapping of a single nuclear spin under ambient conditions

Coherent control of quantum systems has far-reaching implications in quantum engineering. In this context, coherent population trapping (CPT) involving dark resonances has played a prominent role, leading to a wealth of major applications including laser cooling of atoms and molecules, optical magnetometry, light storage and highly precise atomic clocks. Extending CPT methods to individual solid-state quantum systems has been only achieved in cryogenic environments for electron spin impurities and superconducting circuits. Here, we demonstrate efficient CPT of a single nuclear spin in a room temperature solid. To this end, we make use of a three-level system with a $\Lambda$-configuration in the microwave domain, which consists of nuclear spin states addressed through their hyperfine coupling to the electron spin of a single nitrogen-vacancy defect in diamond. Dark state pumping requires a relaxation mechanism which, in atomic systems, is simply provided by spontaneous emission. In this work, the relaxation process is externally controlled through incoherent optical pumping and separated in time from consecutive coherent microwave excitations of the nuclear spin $\Lambda$-system. Such a pumping scheme with controlled relaxation allows us (i) to monitor the sequential accumulation of population into the dark state and (ii) to reach a new regime of CPT dynamics for which periodic arrays of dark resonances can be observed, owing to multiple constructive interferences. This work offers new prospects for quantum state preparation, information storage in hybrid quantum systems and metrology.Comment: 13 pages including supplementary information, links to figures correcte

Analytic treatment of CRIB Quantum Memories for Light using Two-level Atoms

It has recently been discovered that the optical analogue of a gradient echo in an optically thick material could form the basis of a optical memory that is both completely efficient and noise free. Here we present analytical calculation showing this is the case. There is close analogy between the operation of the memory and an optical system with two beam splitters. We can use this analogy to calculate efficiencies as a function of optical depth for a number of quantum memory schemes based on controlled inhomogeneous broadening. In particular we show that multiple switching leads to a net 100% retrieval efficiency for the optical gradient echo even in the optically thin case.Comment: 10 page

An AC Stark Gradient Echo Memory in Cold Atoms

The burgeoning fields of quantum computing and quantum key distribution have created a demand for a quantum memory. The gradient echo memory scheme is a quantum memory candidate for light storage that can boast efficiencies approaching unity, as well as the flexibility to work with either two or three level atoms. The key to this scheme is the frequency gradient that is placed across the memory. Currently the three level implementation uses a Zeeman gradient and warm atoms. In this paper we model a new gradient creation mechanism - the ac Stark effect - to provide an improvement in the flexibility of gradient creation and field switching times. We propose this scheme in concert with a move to cold atoms (~1 mK). These temperatures would increase the storage times possible, and the small ensemble volumes would enable large ac Stark shifts with reasonable laser power. We find that memory bandwidths on the order of MHz can be produced with experimentally achievable laser powers and trapping volumes, with high precision in gradient creation and switching times on the order of nanoseconds possible. By looking at the different decoherence mechanisms present in this system we determine that coherence times on the order of 10s of milliseconds are possible, as are delay-bandwidth products of approximately 50 and efficiencies over 90%

Gradient Echo Quantum Memory for Light using Two-level Atoms

We propose a quantum memory for light that is analogous to the NMR gradient echo. Our proposal is ideally perfectly efficient and provides simplifications to current 3-level quantum memory schemes based on controlled inhomogeneous broadening. Our scheme does not require auxiliary light fields. Instead the input optical pulse interacts only with two-level atoms that have linearly increasing Stark shifts. By simply reversing the sign of the atomic Stark shifts, the pulse is retrieved in the forward direction. We present analytical, numerical and experimental results of this scheme. We report experimental efficiencies of up to 15% and suggest simple realizable improvements to significantly increase the efficiency.Comment: 4 pages, 4 figure