24 research outputs found
Fragmentation of Nuclei at Intermediate and High Energies in Modified Cascade Model
The process of nuclear multifragmentation has been implemented, together with
evaporation and fission channels of the disintegration of excited remnants in
nucleus-nucleus collisions using percolation theory and the intranuclear
cascade model. Colliding nuclei are treated as face--centered--cubic lattices
with nucleons occupying the nodes of the lattice. The site--bond percolation
model is used. The code can be applied for calculation of the fragmentation of
nuclei in spallation and multifragmentation reactions.Comment: 19 pages, 10 figure
Unified description of magic numbers of metal clusters in terms of the 3-dimensional q-deformed harmonic oscillator
Magic numbers predicted by a 3-dimensional q-deformed harmonic oscillator
with Uq(3)>SOq(3) symmetry are compared to experimental data for atomic
clusters of alkali metals (Li, Na, K, Rb, Cs), noble metals (Cu, Ag, Au),
divalent metals (Zn, Cd), and trivalent metals (Al, In), as well as to
theoretical predictions of jellium models, Woods-Saxon and wine bottle
potentials, and to the classification scheme using the 3n+l pseudo quantum
number. In alkali metal clusters and noble metal clusters the 3-dimensional
q-deformed harmonic oscillator correctly predicts all experimentally observed
magic numbers up to 1500 (which is the expected limit of validity for theories
based on the filling of electronic shells), while in addition it gives
satisfactory results for the magic numbers of clusters of divalent metals and
trivalent metals, thus indicating that Uq(3), which is a nonlinear extension of
the U(3) symmetry of the spherical (3-dimensional isotropic) harmonic
oscillator, is a good candidate for being the symmetry of systems of several
metal clusters. The Taylor expansions of angular momentum dependent potentials
approximately producing the same spectrum as the 3-dimensional q-deformed
harmonic oscillator are found to be similar to the Taylor expansions of the
symmetrized Woods-Saxon and wine-bottle symmetrized Woods-Saxon potentials,
which are known to provide successful fits of the Ekardt potentials.Comment: 23 pages including 7 table
Atomic structure and segregation in alkali-metal heteroclusters
The ground-state atomic and electronic distributions in NamCsn clusters with composition m=n and m=2n have been calculated by minimizing the total cluster energy using the density-functional formalism. The approximation is made by replacing the total external potential of the ions by its spherical average around the cluster center during the iterative process of solving the Kohn-Sham equations for each geometry tested. In the size range studied here (up to 90 atoms per cluster), the cluster is composed of well-separated homoatomic Na and Cs shells, the external one always being a Cs shell. We have also found that the cohesive energy goes rapidly to the bulk limit. An analysis of the geometries shows strong cluster reconstruction with increasing size. By comparing the geometry of pure Nan with that of the Nan core in NanCsn for clusters formed by only an inner Na layer and an outer Cs layer, we have observed that the Nan core adopts a geometry different in most cases from that of the free Nan cluster, and such that the number of faces of the polyhedron formed by the Nan core is as close as possible to the number of external Cs atoms, in order to accomodate these Cs atoms on top of the faces of the polyhedron