553 research outputs found
Neutron knockout of 12Be populating neutron-unbound states in 11Be
Neutron-unbound resonant states of 11Be were populated in neutron knock-out
reactions from 12Be and identified by 10Be-n coincidence measurements. A
resonance in the decay-energy spectrum at 80(2) keV was attributed to a highly
excited unbound state in 11Be at 3.949(2) MeV decaying to the 2+ excited state
in 10Be. A knockout cross section of 15(3) mb was inferred for this 3.949(2)
MeV state suggesting a spectroscopic factor near unity for this 0p3/2- level,
consistent with the detailed shell model calculations.Comment: 5 pages, 2 figures \pacs{29.38.Db, 29.30.Hs, 24.50.+g, 21.10.Pc,
21.10.Hw, 27.20.+n} \keywords{neutron decay spectroscopy, neutron-unbound
states in 11Be
Aqueous U(VI) interaction with magnetic nanoparticles in a mixed flow reactor system: HR-XANES study
The redox variations and changes in local atomic environment of uranium (U) interacted with the magnetite nanoparticles were studied in a proof of principle experiment by the U L3 and M4 edges high energy resolution X-ray absorption near edge structure (HR-XANES) technique. We designed and applied a mixed flow reactor (MFR) set-up to maintain dynamic flow conditions during U-magnetite interactions. Formation of hydrolyzed, bi- and poly-nuclear U species were excluded by slow continuous injection of U(VI) (10-6 M) and pH control integrated in the MFR set-up. The applied U HR-XANES technique is more sensitive to minor changes in the U redox states and bonding compared to the conventional XANES method. Major U(VI) contribution in uranyl type of bonding is found in the magnetite nanoparticles after three days operation time of the MFR. Indications for shortening of the U-Oaxial bond length for the magnetite compared to the maghemite system are present too
XAS signatures of Am(III) adsorbed onto magnetite and maghemite
Trivalent americium was adsorbed on magnetite and maghemite under similar chemical conditions and the local environment probed by EXAFS spectroscopy. In both samples, partially hydrated Am(III) binds the surface but slightly different surface complexes were identified. On Fe3O4, Am(III) forms monomeric tridentate surface complexes similar to that reported for Pu(III) at the (111) surface. In contrast, the lower number of detected Fe atoms may suggest that Am(III) forms monomeric bidentate surface complexes on Îł-Fe2O3. Alternatively, the lower Fe coordination number can also be due to the presence of vacancies in maghemite. XPS data imply very similar binding environments for Am at both Fe oxide surfaces
Spectroscopy of neutron-unbound F
The ground state of F has been observed as an unbound resonance
keV above the ground state of F. Comparison of this
result with USDA/USDB shell model predictions leads to the conclusion that the
F ground state is primarily dominated by -shell configurations. Here
we present a detailed report on the experiment in which the ground state
resonance of F was first observed. Additionally, we report the first
observation of a neutron-unbound excited state in F at an excitation
energy of keV.Comment: 10 pages, 11 figures, Accepted for publication in Phys. Rev.
Observation of a low-lying neutron-unbound state in 19C
Proton removal reactions from a secondary 22N beam were utilized to populate
unbound states in neutron-rich carbon isotopes. Neutrons were measured with the
Modular Neutron Array (MoNA) in coincidence with carbon fragments. A resonance
with a decay energy of 76(14) keV was observed in the system 18C+n
corresponding to a state in 19C at an excitation energy of 653(95)keV. This
resonance could correspond to the first 5/2+ state which was recently
speculated to be unbound in order to describe 1n and 2n removal cross section
measurements from 20C.Comment: accepted for publication in Nucl. Phys.
Two-Neutron Sequential Decay of O
A two-neutron unbound excited state of O was populated through a
(d,d') reaction at 83.4 MeV/nucleon. A state at (stat) (sys) keV with a width of MeV was observed above the
two-neutron separation energy placing it at 7.65 0.2 MeV with respect to
the ground state. Three-body correlations for the decay of O
O + show clear evidence for a sequential decay
through an intermediate state in O. Neither a di-neutron nor phase-space
model for the three-body breakup were able to describe these correlations
Exploring the Low- Shore of the Island of Inversion at
The technique of invariant mass spectroscopy has been used to measure, for
the first time, the ground state energy of neutron-unbound
determined to be a resonance in the continuum at
keV. States in were
populated by the reactions of a 62 MeV/u beam impinging on a
288 beryllium target. The measured ground
state energy is in good agreement with USDA/USDB shell model predictions,
indicating that shell intruder configurations play only a small role in
the ground state structure of and establishing a low-
boundary of the island of inversion for N=19 isotones.Comment: 5 pages, 4 figures, to be published in Phys. Rev. Let
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