On the mechanism of irradiation enhanced exchange bias

By means of layer resolved ion irradiation the mechanisms involved in the irradiation driven modifications of the exchange bias effect in NiFe/FeMn bilayers have been investigated. It is shown that not only the locations of the defects but also the magnetic coupling between both layers during the irradiation process is of crucial importance. This requires an extension of current models accounting for defects in exchange bias systems.Comment: 3 pages, 3 figures, revised version, added results from further structural characterization by TEM, submitted to Europhysics Letter

Lorentz TEM imaging of stripe structures embedded in a soft magnetic matrix

N\'eel walls in soft magnetic NiFe/NiFeGa hybrid stripe structures surrounded by a NiFe film are investigated by high resolution Lorentz transmission electron microscopic imaging. An anti-parallel orientation of magnetization in 1000 nm wide neighboring unirradiated-irradiated stripes is observed by forming high angle domain walls during magnetization reversal. Upon downscaling the stripe structure size from 1000 nm to 200 nm a transition from a discrete domain pattern to an effective magnetic medium is observed for external magnetic field reversal. This transition is associated with vanishing ability of hosting high angle domain walls between adjacent stripes. The investigation also demonstrated the potentiality of Lorentz microscopy to image periodic stripe structures well under micron length-scale.Comment: 7 pages, 6 figure

Origin of magnetic moments in defective TiO2 single crystals

In this paper we show that ferromagnetism can be induced in pure TiO2 single crystals by oxygen ion irradiation. By combining x-ray diffraction, Raman-scattering, and electron spin resonance spectroscopy, a defect complex, \emph{i.e.} Ti$^{3+}$ ions on the substitutional sites accompanied by oxygen vacancies, has been identified in irradiated TiO2. This kind of defect complex results in a local (TiO$_{6-x}$) stretching Raman mode. We elucidate that Ti$^{3+}$ ions with one unpaired 3d electron provide the local magnetic moments.Comment: 4 pages, 4 figures, to be published at Phys. Rev.

The reversal of the SF-density relation in a massive, X-ray selected galaxy cluster at z=1.58: results from Herschel

Dusty, star-forming galaxies have a critical role in the formation and evolution of massive galaxies in the Universe. Using deep far-infrared imaging in the range 100-500um obtained with the Herschel telescope, we investigate the dust-obscured star formation in the galaxy cluster XDCP J0044.0-2033 at z=1.58, the most massive cluster at z >1.5, with a measured mass M200= 4.7x10$^{14}$ Msun. We perform an analysis of the spectral energy distributions (SEDs) of 12 cluster members (5 spectroscopically confirmed) detected with >3$\sigma$ significance in the PACS maps, all ULIRGs. The individual star formation rates (SFRs) lie in the range 155-824 Ms/yr, with dust temperatures of 24$\pm$35 K. We measure a strikingly high amount of star formation (SF) in the cluster core, SFR ( 1875$\pm$158 Ms/yr, 4x higher than the amount of star formation in the cluster outskirts. This scenario is unprecedented in a galaxy cluster, showing for the first time a reversal of the SF-density relation at z~1.6 in a massive cluster.Comment: Letter accepted for publication in MNRAS, ESA Press Release on 18 December 201

Control of interlayer exchange coupling in Fe/Cr/Fe trilayers by ion beam irradiation

The manipulation of the antiferromagnetic interlayer coupling in the epitaxial Fe/Cr/Fe(001) trilayer system by moderate 5 keV He ion beam irradiation has been investigated experimentally. It is shown that even for irradiation with very low fluences (10^14 ions/cm^2) a drastic change in strength of the coupling appears. For thin Cr-spacers (below 0.6 - 0.7 nm) the coupling strength decreases with fluence, becoming ferromagnetic for fluences above (2x10^14 ions/cm^2). The effect is connected with the creation of magnetic bridges in the layered system due to atomic exchange events caused by the bombardment. For thicker Cr spacers (0.8 - 1.2 nm) an enhancement of the antiferromagnetic coupling strength is found. A possible explanation of the enhancement effect is given.Comment: Submitted to PR

Evidence for Kosterlitz-Thouless type orientational ordering of CF3_3Br monolayers physisorbed on graphite

Monolayers of the halomethane CF$_3$Br adsorbed on graphite have been investigated by x-ray diffraction. The layers crystallize in a commensurate triangular lattice. On cooling they approach a three-sublattice antiferroelectric pattern of the in-plane components of the dipole moments. The ordering is not consistent with a conventional phase transition, but points to Kosterlitz-Thouless behavior. It is argued that the transition is described by a 6-state clock model on a triangular lattice with antiferromagnetic nearest neighbor interactions which is studied with Monte-Carlo simulations. A finite-size scaling analysis shows that the ordering transition is indeed in the KT universality class.Comment: 4 pages, 5 figure

Crystallographically oriented magnetic ZnFe2O4 nanoparticles synthesized by Fe implantation into ZnO

In this paper, a correlation between structural and magnetic properties of Fe implanted ZnO is presented. High fluence Fe^+ implantation into ZnO leads to the formation of superparamagnetic alpha-Fe nanoparticles. High vacuum annealing at 823 K results in the growth of alpha-Fe particles, but the annealing at 1073 K oxidized the majority of the Fe nanoparticles. After a long term annealing at 1073 K, crystallographically oriented ZnFe2O4 nanoparticles were formed inside ZnO with the orientation relationship of ZnFe2O4(111)[110]//ZnO(0001)[1120]. These ZnFe2O4 nanoparticles show a hysteretic behavior upon magnetization reversal at 5 K.Comment: 21 pages, 7 figures, accepted by J. Phys. D: Appl. Phy

Spinel ferrite nanocrystals embedded inside ZnO: magnetic, electronic and magneto-transport properties

In this paper we show that spinel ferrite nanocrystals (NiFe2O4, and CoFe2O4) can be texturally embedded inside a ZnO matrix by ion implantation and post-annealing. The two kinds of ferrites show different magnetic properties, e.g. coercivity and magnetization. Anomalous Hall effect and positive magnetoresistance have been observed. Our study suggests a ferrimagnet/semiconductor hybrid system for potential applications in magneto-electronics. This hybrid system can be tuned by selecting different transition metal ions (from Mn to Zn) to obtain various magnetic and electronic properties.Comment: 12 pages, 14 figs. accepted for publication at PR