Polariton-mediated Raman scattering in microcavities: A Green's function approach

We present calculations of the intensity of polariton-mediated inelastic light scattering in semiconductor microcavities within a Green's function framework. In addition to reproducing the strong coupling of light and matter, this method also enables the inclusion of damping mechanisms in a consistent way. Our results show excellent agreement with recent Raman scattering experiments.Comment: 6 pages, 1 figur

Cavity polariton optomechanics: Polariton path to fully resonant dispersive coupling in optomechanical resonators

Resonant photoelastic coupling in semiconductor nanostructures opens new perspectives for strongly enhanced light-sound interaction in optomechanical resonators. One potential problem, however, is the reduction of the cavity Q-factor induced by dissipation when the resonance is approached. We show in this letter that cavity-polariton mediation in the light-matter process overcomes this limitation allowing for a strongly enhanced photon-phonon coupling without significant lifetime reduction in the strongly-coupled regime. Huge optomechanical coupling factors in the PetaHz/nm range are envisaged, three orders of magnitude larger than the backaction produced by the mechanical displacement of the cavity mirrors.Comment: 6 pages, 4 figure

Resonance effects in the Raman scattering of mono- and few layers MoSe2_2

Using resonant Raman scattering spectroscopy with 25 different laser lines, we describe the Raman scattering spectra of mono- and multi-layers 2H-molybdenum diselenide (MoSe$_2$) as well as the different resonances affecting the most pronounced features. For high-energy phonons, both A- and E- symmetry type phonons present resonances with A and B excitons of MoSe$_2$ together with a marked increase of intensity when exciting at higher energy, close to the C exciton energy. We observe symmetry dependent exciton-phonon coupling affecting mainly the low-energy rigid layer phonon modes. The shear mode for multilayer displays a pronounced resonance with the C exciton while the breathing mode has an intensity that grows with the excitation laser energy, indicating a resonance with electronic excitations at energies higher than that of the C exciton.Comment: 9 Figures, 9 page

Dispersion and damping of multi-quantum well polaritons from resonant Brillouin scattering by folded acoustic modes

We report on confined exciton resonances of acoustic and folded acoustic phonon light scattering in a GaAs/AlAs multi-quantum-well. Significant variations of the line shifts and widths are observed across the resonance and quantitatively reproduced in terms of the polariton dispersion. This high resolution Brillouin study brings new unexpectedly detailed informations on the polariton dynamics in confined systems

Uncoupled excitons in semiconductor microcavities detected in resonant Raman scattering

We present an outgoing resonant Raman-scattering study of a GaAs/AlGaAs based microcavity embedded in a p-i-n junction. The p-i-n junction allows the vertical electric field to be varied, permitting control of exciton-photon detuning and quenching of photoluminescence which otherwise obscures the inelastic light scattering signals. Peaks corresponding to the upper and lower polariton branches are observed in the resonant Raman cross sections, along with a third peak at the energy of uncoupled excitons. This third peak, attributed to disorder activated Raman scattering, provides clear evidence for the existence of uncoupled exciton reservoir states in microcavities in the strong-coupling regime

Extension of charge-state-distribution calculations for ion-solid collisions towards low velocities and many-electron ions

Knowledge of the detailed evolution of the whole charge-state distribution of projectile ions colliding with targets is required in several fields of research such as material science and atomic and nuclear physics but also in accelerator physics, and in particular in regard to the several foreseen large-scale facilities. However, there is a lack of data for collisions in the nonperturbative energy domain and that involve many-electron projectiles. Starting from the etacha model we developed [Rozet, Nucl. Instrum. Methods Phys. Res., Sect. B 107, 67 (1996)10.1016/0168-583X(95)00800-4], we present an extension of its validity domain towards lower velocities and larger distortions. Moreover, the system of rate equations is able to take into account ions with up to 60 orbital states of electrons. The computed data from the different new versions of the etacha code are compared to some test collision systems. The improvements made are clearly illustrated by 28.9MeVu-1Pb56+ ions, and laser-generated carbon ion beams of 0.045 to 0.5MeVu-1, passing through carbon or aluminum targets, respectively. Hence, those new developments can efficiently sustain the experimental programs that are currently in progress on the "next-generation" accelerators or laser facilities.Fil: Lamour, E.. Centre National de la Recherche Scientifique; Francia. Universite de Paris; FranciaFil: Fainstein, Pablo Daniel. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina. Comisión Nacional de Energía Atómica. Centro Atómico Bariloche; ArgentinaFil: Galassi, Mariel Elisa. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario. Instituto de Física de Rosario. Universidad Nacional de Rosario. Instituto de Física de Rosario; ArgentinaFil: Prigent, C.. Centre National de la Recherche Scientifique; Francia. Universite de Paris; FranciaFil: Ramirez, C. A.. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario. Instituto de Física de Rosario. Universidad Nacional de Rosario. Instituto de Física de Rosario; ArgentinaFil: Rivarola, Roberto Daniel. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario. Instituto de Física de Rosario. Universidad Nacional de Rosario. Instituto de Física de Rosario; ArgentinaFil: Rozet, J. P.. Centre National de la Recherche Scientifique; Francia. Universite de Paris; FranciaFil: Trassinelli, M.. Centre National de la Recherche Scientifique; Francia. Universite de Paris; FranciaFil: Vernhet, D.. Centre National de la Recherche Scientifique; Francia. Universite de Paris; Franci

Theory of high-order harmonic generation from molecules by intense laser pulses

We show that high-order harmonics generated from molecules by intense laser pulses can be expressed as the product of a returning electron wave packet and the photo-recombination cross section (PRCS) where the electron wave packet can be obtained from simple strong-field approximation (SFA) or from a companion atomic target. Using these wave packets but replacing the PRCS obtained from SFA or from the atomic target by the accurate PRCS from molecules, the resulting HHG spectra are shown to agree well with the benchmark results from direct numerical solution of the time-dependent Schr\"odinger equation, for the case of H$_2^+$ in laser fields. The result illustrates that these powerful theoretical tools can be used for obtaining high-order harmonic spectra from molecules. More importantly, the results imply that the PRCS extracted from laser-induced HHG spectra can be used for time-resolved dynamic chemical imaging of transient molecules with temporal resolutions down to a few femtoseconds.Comment: 10 pages, 5 figure

Phonon Bloch oscillations in acoustic-cavity structures

We describe a semiconductor multilayer structure based in acoustic phonon cavities and achievable with MBE technology, designed to display acoustic phonon Bloch oscillations. We show that forward and backscattering Raman spectra give a direct measure of the created phononic Wannier-Stark ladder. We also discuss the use of femtosecond laser impulsions for the generation and direct probe of the induced phonon Bloch oscillations. We propose a gedanken experiment based in an integrated phonon source-structure-detector device, and we present calculations of pump and probe time dependent optical reflectivity that evidence temporal beatings in agreement with the Wannier-Stark ladder energy splitting.Comment: PDF file including 4 figure