Stable and Metastable Structures of Cobalt on Cu(001): An ab initio Study

We report results of density-functional theory calculations on the structural, magnetic, and electronic properties of (1x1)-structures of Co on Cu(001) for coverages up to two monolayers. In particular we discuss the tendency towards phase separation in Co islands and the possibility of segregation of Cu on top of the Co-film. A sandwich structure consisting of a bilayer Co-film covered by 1ML of Cu is found to be the lowest-energy configuration. We also discuss a bilayer c(2x2)-alloy which may form due to kinetic reasons, or be stabilized at strained surface regions. Furthermore, we study the influence of magnetism on the various structures and, e.g., find that Co adlayers induce a weak spin-density wave in the copper substrate.Comment: 11 pages including 4 figures. Related publications can be found at http://www.fhi-berlin.mpg.de/th/paper.htm

Anisotropic susceptibility of ferromagnetic ultrathin Co films on vicinal Cu

We measure the magnetic susceptibility of ultrathin Co films with an in-plane uniaxial magnetic anisotropy grown on a vicinal Cu substrate. Above the Curie temperature the influence of the magnetic anisotropy can be investigated by means of the parallel and transverse susceptibilities along the easy and hard axes. By comparison with a theoretical analysis of the susceptibilities we determine the isotropic exchange interaction and the magnetic anisotropy. These calculations are performed in the framework of a Heisenberg model by means of a many-body Green's function method, since collective magnetic excitations are very important in two-dimensional magnets.Comment: 7 pages, 3 figure