Dynamics of immersed molecules in superfluids

The dynamics of a molecule immersed in a superfluid medium are considered. Results are derived using a classical hydrodynamic approach followed by canonical quantization. The classical model, a rigid body immersed in incompressible fluid, permits a thorough analysis; its effective Hamiltonian generalizes the usual rigid-rotor Hamiltonian. In contrast to the free rigid rotor, the immersed body is shown to have chaotic dynamics. Quantization of the classical model leads to new and experimentally verifiable features. It is shown, for instance, that chiral molecules can behave as "quantum propellers": the rotational-translational coupling induced by the superfluid leads to a nonzero linear momentum in the ground state. Hydrogen peroxide is a strong candidate for experimental detection of this effect. The signature is a characteristic splitting of rotational absorption lines. The 1_{01} --> 1_{10} line in hydrogen peroxide, for example, is predicted to split into three lines separated by as much as 0.01 cm^{-1}, which is about the experimental linewidth.Comment: 10 pages, 3 figure

Interaction between static holes in a quantum dimer model on the kagome lattice

A quantum dimer model (QDM) on the kagome lattice with an extensive ground-state entropy was recently introduced [Phys. Rev. B 67, 214413 (2003)]. The ground-state energy of this QDM in presence of one and two static holes is investigated by means of exact diagonalizations on lattices containing up to 144 kagome sites. The interaction energy between the holes (at distances up to 7 lattice spacings) is evaluated and the results show no indication of confinement at large hole separations.Comment: 6 pages, 3 figures. IOP style files included. To appear in J. Phys.: Condens. Matter, Proceedings of the HFM2003 conference, Grenobl

Scattering-free plasmonic optics with anisotropic metamaterials

We develop an approach to utilize anisotropic metamaterials to solve one of the fundamental problems of modern plasmonics -- parasitic scattering of surface waves into free-space modes, opening the road to truly two-dimensional plasmonic optics. We illustrate the developed formalism on examples of plasmonic refractor and plasmonic crystal, and discuss limitations of the developed technique and its possible applications for sensing and imaging structures, high-performance mode couplers, optical cloaking structures, and dynamically reconfigurable electro-plasmonic circuits

Naturally-phasematched second harmonic generation in a whispering gallery mode resonator

We demonstrate for the first time natural phase matching for optical frequency doubling in a high-Q whispering gallery mode resonator made of Lithium Niobate. A conversion efficiency of 9% is achieved at 30 micro Watt in-coupled continuous wave pump power. The observed saturation pump power of 3.2 mW is almost two orders of magnitude lower than the state-of-the-art. This suggests an application of our frequency doubler as a source of non-classical light requiring only a low-power pump, which easily can be quantum noise limited. Our theoretical analysis of the three-wave mixing in a whispering gallery mode resonator provides the relative conversion efficiencies for frequency doubling in various modes

Rules for Computing Symmetry, Density and Stoichiometry in a Quasi-Unit-Cell Model of Quasicrystals

The quasi-unit cell picture describes the atomic structure of quasicrystals in terms of a single, repeating cluster which overlaps neighbors according to specific overlap rules. In this paper, we discuss the precise relationship between a general atomic decoration in the quasi-unit cell picture atomic decorations in the Penrose tiling and in related tiling pictures. Using these relations, we obtain a simple, practical method for determining the density, stoichiometry and symmetry of a quasicrystal based on the atomic decoration of the quasi-unit cell taking proper account of the sharing of atoms between clusters.Comment: 14 pages, 8 figure

Stability of the hard-sphere icosahedral quasilattice

The stability of the hard-sphere icosahedral quasilattice is analyzed using the differential formulation of the generalized effective liquid approximation. We find that the icosahedral quasilattice is metastable with respect to the hard-sphere crystal structures. Our results agree with recent findings by McCarley and Ashcroft [Phys. Rev. B {\bf 49}, 15600 (1994)] carried out using the modified weighted density approximation.Comment: 15 pages, 2 figures available from authors upon request, (revtex), submitted to Phys. Rev.

Exact Solution of an Octagonal Random Tiling Model

We consider the two-dimensional random tiling model introduced by Cockayne, i.e. the ensemble of all possible coverings of the plane without gaps or overlaps with squares and various hexagons. At the appropriate relative densities the correlations have eight-fold rotational symmetry. We reformulate the model in terms of a random tiling ensemble with identical rectangles and isosceles triangles. The partition function of this model can be calculated by diagonalizing a transfer matrix using the Bethe Ansatz (BA). The BA equations can be solved providing {\em exact} values of the entropy and elastic constants.Comment: 4 pages,3 Postscript figures, uses revte

Hybrid-Entanglement in Continuous Variable Systems

Entanglement is one of the most fascinating features arising from quantum-mechanics and of great importance for quantum information science. Of particular interest are so-called hybrid-entangled states which have the intriguing property that they contain entanglement between different degrees of freedom (DOFs). However, most of the current continuous variable systems only exploit one DOF and therefore do not involve such highly complex states. We break this barrier and demonstrate that one can exploit squeezed cylindrically polarized optical modes to generate continuous variable states exhibiting entanglement between the spatial and polarization DOF. We show an experimental realization of these novel kind of states by quantum squeezing an azimuthally polarized mode with the help of a specially tailored photonic crystal fiber

Magnetic susceptibility and specific heat of the spin-1/2 Heisenberg model on the kagome lattice and experimental data on ZnCu3(OH)6Cl2

We compute the magnetic susceptibility and specific heat of the spin-1/2 Heisenberg model on the kagome lattice with high-temperature expansions and exact diagonalizations. We compare the results with the experimental data on ZnCu3(OH)6Cl2 obtained by Helton et al. [Phys. Rev. Lett. 98, 107204 (2007)]. Down to k_BT/J~0.2, our calculations reproduce accurately the experimental susceptibility, with an exchange interaction J~190K and a contribution of 3.7% of weakly interacting impurity spins. The comparison between our calculations of the specific heat and the experiments indicate that the low-temperature entropy (below ~20K) is smaller in ZnCu3(OH)6Cl2 than in the kagome Heisenberg model, a likely signature of other interactions in the system.Comment: Minor revisions in the text and references. To appear in Eur. Phys. J.